{"title":"具有可调节的电催化二氧化碳还原产物的纯相 IB 族 Sn 基合金的通用合成方法","authors":"Luyao Yang, Wenqing Zhang, Ximei Lv, Qianqian Zhao, Xiaojing Liu, Shulin Zhao, Yuhui Chen","doi":"10.1039/d4cc05317f","DOIUrl":null,"url":null,"abstract":"We present a universal method for synthesizing a range of pure-phase IB-group Sn-based alloy catalysts (Cu3Sn, Ag4Sn, and AuSn) for electrochemical reduction of CO2 to C1 product. The selectivity can be widely adjusted based on the change in metal composition and applied potential. This study contribute to a better understanding of the structure-activity relationship between components and properties in various Sn-based alloys.","PeriodicalId":67,"journal":{"name":"Chemical Communications","volume":null,"pages":null},"PeriodicalIF":4.3000,"publicationDate":"2024-10-22","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Universal synthesis of pure-phase IB-group Sn-based alloys with modulable electrocatalytic CO2 reduction products\",\"authors\":\"Luyao Yang, Wenqing Zhang, Ximei Lv, Qianqian Zhao, Xiaojing Liu, Shulin Zhao, Yuhui Chen\",\"doi\":\"10.1039/d4cc05317f\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"We present a universal method for synthesizing a range of pure-phase IB-group Sn-based alloy catalysts (Cu3Sn, Ag4Sn, and AuSn) for electrochemical reduction of CO2 to C1 product. The selectivity can be widely adjusted based on the change in metal composition and applied potential. This study contribute to a better understanding of the structure-activity relationship between components and properties in various Sn-based alloys.\",\"PeriodicalId\":67,\"journal\":{\"name\":\"Chemical Communications\",\"volume\":null,\"pages\":null},\"PeriodicalIF\":4.3000,\"publicationDate\":\"2024-10-22\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Chemical Communications\",\"FirstCategoryId\":\"92\",\"ListUrlMain\":\"https://doi.org/10.1039/d4cc05317f\",\"RegionNum\":2,\"RegionCategory\":\"化学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q2\",\"JCRName\":\"CHEMISTRY, MULTIDISCIPLINARY\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Chemical Communications","FirstCategoryId":"92","ListUrlMain":"https://doi.org/10.1039/d4cc05317f","RegionNum":2,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q2","JCRName":"CHEMISTRY, MULTIDISCIPLINARY","Score":null,"Total":0}
引用次数: 0
摘要
我们提出了一种合成一系列纯相 IB 族锡基合金催化剂（Cu3Sn、Ag4Sn 和 AuSn）的通用方法，用于将 CO2 电化学还原为 C1 产物。根据金属成分和应用电位的变化，选择性可进行广泛调整。这项研究有助于更好地理解各种锡基合金中成分与性能之间的结构-活性关系。
Universal synthesis of pure-phase IB-group Sn-based alloys with modulable electrocatalytic CO2 reduction products
We present a universal method for synthesizing a range of pure-phase IB-group Sn-based alloy catalysts (Cu3Sn, Ag4Sn, and AuSn) for electrochemical reduction of CO2 to C1 product. The selectivity can be widely adjusted based on the change in metal composition and applied potential. This study contribute to a better understanding of the structure-activity relationship between components and properties in various Sn-based alloys.
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