甲烷和煤尘混合物爆炸中 OH* 发射光谱特征和瞬态点火动力学实验研究

IF 6.9 2区 环境科学与生态学 Q1 ENGINEERING, CHEMICAL Process Safety and Environmental Protection Pub Date : 2024-10-22 DOI:10.1016/j.psep.2024.10.068
Siyu Tian , Botao Qin , Yanwei Zhang , Dong Ma , Jingde Xu
{"title":"甲烷和煤尘混合物爆炸中 OH* 发射光谱特征和瞬态点火动力学实验研究","authors":"Siyu Tian ,&nbsp;Botao Qin ,&nbsp;Yanwei Zhang ,&nbsp;Dong Ma ,&nbsp;Jingde Xu","doi":"10.1016/j.psep.2024.10.068","DOIUrl":null,"url":null,"abstract":"<div><div>Combustible gases, dusts and their mixtures are widely present in human production and life,and the fire and explosion disasters caused by them pose a serious threat to the field of energy security applications. Studying the ignition process of mixtures is essential for disaster risk assessment and safety protection. In this work, the explosion characteristics and OH* emission spectra of the mixtures were experimentally tested by varying the fuel equivalence ratio ( ER ≈ 0.79 ∼ 1.71), and the evolution of the transient flow field structure during the ignition process was quantitatively analyzed using the schlieren image velocimetry method. The results indicate that the emission spectrum of OH* is closely correlated with the maximum explosion pressure, and the spectral intensity of OH* at 306.4 nm is consistent with the maximum rate of explosion pressure rise. The flow field during the ignition process of the mixtures shows that a small amount of coal dust (concentration≤30 g/m<sup>3</sup>) can significantly promote flame acceleration and instability as the methane concentration is in lean combustion or stoichiometric ratio. However, when the concentration of coal dust increases (concentration≥40 g/m<sup>3</sup>), coal dust will suppress flame acceleration and instability. For methane concentration in fuel-rich combustion state, coal dust always suppresses flame acceleration and instability. The experimental results contribute to a further understanding of gas and coal dust mixed explosions and provide a verification database for the construction of chemical kinetic mechanisms.</div></div>","PeriodicalId":20743,"journal":{"name":"Process Safety and Environmental Protection","volume":"192 ","pages":"Pages 669-679"},"PeriodicalIF":6.9000,"publicationDate":"2024-10-22","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Experimental investigation of OH* emission spectrum characteristics and transient ignition dynamics in methane and coal dust mixtures explosions\",\"authors\":\"Siyu Tian ,&nbsp;Botao Qin ,&nbsp;Yanwei Zhang ,&nbsp;Dong Ma ,&nbsp;Jingde Xu\",\"doi\":\"10.1016/j.psep.2024.10.068\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<div><div>Combustible gases, dusts and their mixtures are widely present in human production and life,and the fire and explosion disasters caused by them pose a serious threat to the field of energy security applications. Studying the ignition process of mixtures is essential for disaster risk assessment and safety protection. In this work, the explosion characteristics and OH* emission spectra of the mixtures were experimentally tested by varying the fuel equivalence ratio ( ER ≈ 0.79 ∼ 1.71), and the evolution of the transient flow field structure during the ignition process was quantitatively analyzed using the schlieren image velocimetry method. The results indicate that the emission spectrum of OH* is closely correlated with the maximum explosion pressure, and the spectral intensity of OH* at 306.4 nm is consistent with the maximum rate of explosion pressure rise. The flow field during the ignition process of the mixtures shows that a small amount of coal dust (concentration≤30 g/m<sup>3</sup>) can significantly promote flame acceleration and instability as the methane concentration is in lean combustion or stoichiometric ratio. However, when the concentration of coal dust increases (concentration≥40 g/m<sup>3</sup>), coal dust will suppress flame acceleration and instability. For methane concentration in fuel-rich combustion state, coal dust always suppresses flame acceleration and instability. The experimental results contribute to a further understanding of gas and coal dust mixed explosions and provide a verification database for the construction of chemical kinetic mechanisms.</div></div>\",\"PeriodicalId\":20743,\"journal\":{\"name\":\"Process Safety and Environmental Protection\",\"volume\":\"192 \",\"pages\":\"Pages 669-679\"},\"PeriodicalIF\":6.9000,\"publicationDate\":\"2024-10-22\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Process Safety and Environmental Protection\",\"FirstCategoryId\":\"93\",\"ListUrlMain\":\"https://www.sciencedirect.com/science/article/pii/S0957582024013508\",\"RegionNum\":2,\"RegionCategory\":\"环境科学与生态学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q1\",\"JCRName\":\"ENGINEERING, CHEMICAL\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Process Safety and Environmental Protection","FirstCategoryId":"93","ListUrlMain":"https://www.sciencedirect.com/science/article/pii/S0957582024013508","RegionNum":2,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"ENGINEERING, CHEMICAL","Score":null,"Total":0}
引用次数: 0

摘要

可燃气体、粉尘及其混合物广泛存在于人类的生产和生活中,其引发的火灾和爆炸灾害对能源安全应用领域构成严重威胁。研究混合物的燃烧过程对于灾害风险评估和安全防护至关重要。本研究通过改变燃料当量比(ER ≈ 0.79 ∼ 1.71),对混合物的爆炸特性和 OH* 发射光谱进行了实验测试,并利用 Schlieren 图像速度测量法定量分析了点火过程中瞬态流场结构的演变。结果表明,OH*的发射光谱与最大爆炸压力密切相关,OH*在306.4 nm处的光谱强度与最大爆炸压力上升速率一致。混合物点火过程中的流场表明,当甲烷浓度处于贫燃或化学计量比时,少量煤粉(浓度≤30 g/m3)可显著促进火焰加速和不稳定。但当煤粉浓度增加时(浓度≥40 g/m3),煤粉会抑制火焰加速和不稳定。对于富燃料燃烧状态下的甲烷浓度,煤粉始终抑制火焰加速和不稳定。实验结果有助于进一步理解瓦斯和煤粉混合爆炸,并为构建化学动力学机制提供了验证数据库。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
查看原文
分享 分享
微信好友 朋友圈 QQ好友 复制链接
本刊更多论文
Experimental investigation of OH* emission spectrum characteristics and transient ignition dynamics in methane and coal dust mixtures explosions
Combustible gases, dusts and their mixtures are widely present in human production and life,and the fire and explosion disasters caused by them pose a serious threat to the field of energy security applications. Studying the ignition process of mixtures is essential for disaster risk assessment and safety protection. In this work, the explosion characteristics and OH* emission spectra of the mixtures were experimentally tested by varying the fuel equivalence ratio ( ER ≈ 0.79 ∼ 1.71), and the evolution of the transient flow field structure during the ignition process was quantitatively analyzed using the schlieren image velocimetry method. The results indicate that the emission spectrum of OH* is closely correlated with the maximum explosion pressure, and the spectral intensity of OH* at 306.4 nm is consistent with the maximum rate of explosion pressure rise. The flow field during the ignition process of the mixtures shows that a small amount of coal dust (concentration≤30 g/m3) can significantly promote flame acceleration and instability as the methane concentration is in lean combustion or stoichiometric ratio. However, when the concentration of coal dust increases (concentration≥40 g/m3), coal dust will suppress flame acceleration and instability. For methane concentration in fuel-rich combustion state, coal dust always suppresses flame acceleration and instability. The experimental results contribute to a further understanding of gas and coal dust mixed explosions and provide a verification database for the construction of chemical kinetic mechanisms.
求助全文
通过发布文献求助,成功后即可免费获取论文全文。 去求助
来源期刊
Process Safety and Environmental Protection
Process Safety and Environmental Protection 环境科学-工程:化工
CiteScore
11.40
自引率
15.40%
发文量
929
审稿时长
8.0 months
期刊介绍: The Process Safety and Environmental Protection (PSEP) journal is a leading international publication that focuses on the publication of high-quality, original research papers in the field of engineering, specifically those related to the safety of industrial processes and environmental protection. The journal encourages submissions that present new developments in safety and environmental aspects, particularly those that show how research findings can be applied in process engineering design and practice. PSEP is particularly interested in research that brings fresh perspectives to established engineering principles, identifies unsolved problems, or suggests directions for future research. The journal also values contributions that push the boundaries of traditional engineering and welcomes multidisciplinary papers. PSEP's articles are abstracted and indexed by a range of databases and services, which helps to ensure that the journal's research is accessible and recognized in the academic and professional communities. These databases include ANTE, Chemical Abstracts, Chemical Hazards in Industry, Current Contents, Elsevier Engineering Information database, Pascal Francis, Web of Science, Scopus, Engineering Information Database EnCompass LIT (Elsevier), and INSPEC. This wide coverage facilitates the dissemination of the journal's content to a global audience interested in process safety and environmental engineering.
期刊最新文献
Investigations on the reactivity removal and leaching behavior of secondary aluminum dross through the thermal oxidation Pollution Analysis of Metals in the Sediments of Lagoon Lakes in Türkiye: Toxicological Risk Assessment and Source Insights Efficient and low-emission approaches for cost-effective hydrogen, power, and heat production based on chemical looping combustion Semi-supervised convolutional generative adversarial networks for dynamic fault classification with manifold regularization Experimental treatment of pickled vegetable wastewater by electrofenton method based on modified PbO2 electrode
×
引用
GB/T 7714-2015
复制
MLA
复制
APA
复制
导出至
BibTeX EndNote RefMan NoteFirst NoteExpress
×
×
提示
您的信息不完整,为了账户安全,请先补充。
现在去补充
×
提示
您因"违规操作"
具体请查看互助需知
我知道了
×
提示
现在去查看 取消
×
提示
确定
0
微信
客服QQ
Book学术公众号 扫码关注我们
反馈
×
意见反馈
请填写您的意见或建议
请填写您的手机或邮箱
已复制链接
已复制链接
快去分享给好友吧!
我知道了
×
扫码分享
扫码分享
Book学术官方微信
Book学术文献互助
Book学术文献互助群
群 号:481959085
Book学术
文献互助 智能选刊 最新文献 互助须知 联系我们:info@booksci.cn
Book学术提供免费学术资源搜索服务,方便国内外学者检索中英文文献。致力于提供最便捷和优质的服务体验。
Copyright © 2023 Book学术 All rights reserved.
ghs 京公网安备 11010802042870号 京ICP备2023020795号-1