{"title":"用于绿色制氢的增值电解材料","authors":"Endalkachew Asefa Moges, Keseven Lakshmanan, Chia-Yu Chang, Wei-Sheng Liao, Fikiru Temesgen Angerasa, Woldesenbet Bafe Dilebo, Habib Gemechu Edao, Kirubel Teshome Tadele, Dessalew Dagnew Alemayehu, Baru Debtera Bejena, Chemeda Barasa Guta, Chun-Chi Chang, Meng-Che Tsai, Wei-Nien Su* and Bing Joe Hwang*, ","doi":"10.1021/acsmaterialslett.4c0117310.1021/acsmaterialslett.4c01173","DOIUrl":null,"url":null,"abstract":"<p >The increasing energy consumption and resulting environmental pollution present a major challenge for society. This has led to a global demand for ultrapure energy and valuable chemical products. Therefore, a sustainable and ecofriendly approach to green energy production is essential. Recently, combining anodic oxidation reactions with hydrogen evolution reactions has shown potential in transforming low-grade molecules such as alcohols (such as ethanol, methanol, ethylene glycol, and glycerol), iodide, and biomass-derived compounds. This method could replace the sluggish oxygen evolution reaction in sustainable electrochemical energy systems. This review summarizes electro-oxidation reactions that produce green hydrogen with low electricity consumption and valuable chemicals from inexpensive small-molecule oxidants. It also explores rational design approaches for catalysts, including late transition metals on carbon-based supports, metal oxides, surface engineering, and interface engineering. Finally, the current challenges and future perspectives for developing material catalysts for value-added electrolysis technologies (power-to-green hydrogen production).</p>","PeriodicalId":9,"journal":{"name":"ACS Catalysis ","volume":null,"pages":null},"PeriodicalIF":11.3000,"publicationDate":"2024-10-03","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://pubs.acs.org/doi/epdf/10.1021/acsmaterialslett.4c01173","citationCount":"0","resultStr":"{\"title\":\"Materials of Value-Added Electrolysis for Green Hydrogen Production\",\"authors\":\"Endalkachew Asefa Moges, Keseven Lakshmanan, Chia-Yu Chang, Wei-Sheng Liao, Fikiru Temesgen Angerasa, Woldesenbet Bafe Dilebo, Habib Gemechu Edao, Kirubel Teshome Tadele, Dessalew Dagnew Alemayehu, Baru Debtera Bejena, Chemeda Barasa Guta, Chun-Chi Chang, Meng-Che Tsai, Wei-Nien Su* and Bing Joe Hwang*, \",\"doi\":\"10.1021/acsmaterialslett.4c0117310.1021/acsmaterialslett.4c01173\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<p >The increasing energy consumption and resulting environmental pollution present a major challenge for society. This has led to a global demand for ultrapure energy and valuable chemical products. Therefore, a sustainable and ecofriendly approach to green energy production is essential. Recently, combining anodic oxidation reactions with hydrogen evolution reactions has shown potential in transforming low-grade molecules such as alcohols (such as ethanol, methanol, ethylene glycol, and glycerol), iodide, and biomass-derived compounds. This method could replace the sluggish oxygen evolution reaction in sustainable electrochemical energy systems. This review summarizes electro-oxidation reactions that produce green hydrogen with low electricity consumption and valuable chemicals from inexpensive small-molecule oxidants. It also explores rational design approaches for catalysts, including late transition metals on carbon-based supports, metal oxides, surface engineering, and interface engineering. Finally, the current challenges and future perspectives for developing material catalysts for value-added electrolysis technologies (power-to-green hydrogen production).</p>\",\"PeriodicalId\":9,\"journal\":{\"name\":\"ACS Catalysis \",\"volume\":null,\"pages\":null},\"PeriodicalIF\":11.3000,\"publicationDate\":\"2024-10-03\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"https://pubs.acs.org/doi/epdf/10.1021/acsmaterialslett.4c01173\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"ACS Catalysis \",\"FirstCategoryId\":\"92\",\"ListUrlMain\":\"https://pubs.acs.org/doi/10.1021/acsmaterialslett.4c01173\",\"RegionNum\":1,\"RegionCategory\":\"化学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q1\",\"JCRName\":\"CHEMISTRY, PHYSICAL\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"ACS Catalysis ","FirstCategoryId":"92","ListUrlMain":"https://pubs.acs.org/doi/10.1021/acsmaterialslett.4c01173","RegionNum":1,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"CHEMISTRY, PHYSICAL","Score":null,"Total":0}
Materials of Value-Added Electrolysis for Green Hydrogen Production
The increasing energy consumption and resulting environmental pollution present a major challenge for society. This has led to a global demand for ultrapure energy and valuable chemical products. Therefore, a sustainable and ecofriendly approach to green energy production is essential. Recently, combining anodic oxidation reactions with hydrogen evolution reactions has shown potential in transforming low-grade molecules such as alcohols (such as ethanol, methanol, ethylene glycol, and glycerol), iodide, and biomass-derived compounds. This method could replace the sluggish oxygen evolution reaction in sustainable electrochemical energy systems. This review summarizes electro-oxidation reactions that produce green hydrogen with low electricity consumption and valuable chemicals from inexpensive small-molecule oxidants. It also explores rational design approaches for catalysts, including late transition metals on carbon-based supports, metal oxides, surface engineering, and interface engineering. Finally, the current challenges and future perspectives for developing material catalysts for value-added electrolysis technologies (power-to-green hydrogen production).
期刊介绍：
ACS Catalysis is an esteemed journal that publishes original research in the fields of heterogeneous catalysis, molecular catalysis, and biocatalysis. It offers broad coverage across diverse areas such as life sciences, organometallics and synthesis, photochemistry and electrochemistry, drug discovery and synthesis, materials science, environmental protection, polymer discovery and synthesis, and energy and fuels.
The scope of the journal is to showcase innovative work in various aspects of catalysis. This includes new reactions and novel synthetic approaches utilizing known catalysts, the discovery or modification of new catalysts, elucidation of catalytic mechanisms through cutting-edge investigations, practical enhancements of existing processes, as well as conceptual advances in the field. Contributions to ACS Catalysis can encompass both experimental and theoretical research focused on catalytic molecules, macromolecules, and materials that exhibit catalytic turnover.
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