人工孢子作为多功能生物催化剂执行生物合成级联（功能材料学进展 45/2024）

IF 18.5 1区材料科学 Q1 CHEMISTRY, MULTIDISCIPLINARY Advanced Functional Materials Pub Date : 2024-11-04 DOI:10.1002/adfm.202470261

Maialen Iturralde, Magdalena Ripoll, Desiré di Silvio, Marta Gallego, Daniel A. Grajales-Hernández, Xabier López, Lorena Betancor, Fernando López-Gallego

{"title":"人工孢子作为多功能生物催化剂执行生物合成级联（功能材料学进展 45/2024）","authors":"Maialen Iturralde, Magdalena Ripoll, Desiré di Silvio, Marta Gallego, Daniel A. Grajales-Hernández, Xabier López, Lorena Betancor, Fernando López-Gallego","doi":"10.1002/adfm.202470261","DOIUrl":null,"url":null,"abstract":"<p><b>Enzyme Immobilization</b></p><p>In article number 2406097, Fernando López-Gallego and co-workers develop a universal method for encapsulating single gram-negative microbes with polymeric coatings to fabricate synthetic spores that selectively bind His-tagged enzymes. These synthetic spores serve as biocatalytic materials for the one-pot oxidative amination of diols into amino alcohols, facilitated by the cooperative catalysis between intracellular and extracellular enzymes that maintain their performance in consecutive batch cycles.\n\n <figure>\n <div><picture>\n <source></source></picture><p></p>\n </div>\n </figure></p>","PeriodicalId":112,"journal":{"name":"Advanced Functional Materials","volume":"34 45","pages":""},"PeriodicalIF":18.5000,"publicationDate":"2024-11-04","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/adfm.202470261","citationCount":"0","resultStr":"{\"title\":\"Artificial Spores as Multi-Functional Biocatalysts to Perform Biosynthetic Cascades (Adv. Funct. Mater. 45/2024)\",\"authors\":\"Maialen Iturralde, Magdalena Ripoll, Desiré di Silvio, Marta Gallego, Daniel A. Grajales-Hernández, Xabier López, Lorena Betancor, Fernando López-Gallego\",\"doi\":\"10.1002/adfm.202470261\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<p><b>Enzyme Immobilization</b></p><p>In article number 2406097, Fernando López-Gallego and co-workers develop a universal method for encapsulating single gram-negative microbes with polymeric coatings to fabricate synthetic spores that selectively bind His-tagged enzymes. These synthetic spores serve as biocatalytic materials for the one-pot oxidative amination of diols into amino alcohols, facilitated by the cooperative catalysis between intracellular and extracellular enzymes that maintain their performance in consecutive batch cycles.\\n\\n <figure>\\n <div><picture>\\n <source></source></picture><p></p>\\n </div>\\n </figure></p>\",\"PeriodicalId\":112,\"journal\":{\"name\":\"Advanced Functional Materials\",\"volume\":\"34 45\",\"pages\":\"\"},\"PeriodicalIF\":18.5000,\"publicationDate\":\"2024-11-04\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"https://onlinelibrary.wiley.com/doi/epdf/10.1002/adfm.202470261\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Advanced Functional Materials\",\"FirstCategoryId\":\"88\",\"ListUrlMain\":\"https://onlinelibrary.wiley.com/doi/10.1002/adfm.202470261\",\"RegionNum\":1,\"RegionCategory\":\"材料科学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q1\",\"JCRName\":\"CHEMISTRY, MULTIDISCIPLINARY\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Advanced Functional Materials","FirstCategoryId":"88","ListUrlMain":"https://onlinelibrary.wiley.com/doi/10.1002/adfm.202470261","RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"CHEMISTRY, MULTIDISCIPLINARY","Score":null,"Total":0}

引用次数: 0

摘要

酶固定化在文章编号 2406097 中，Fernando López-Gallego 及其合作者开发了一种通用方法，用聚合物涂层包裹单个革兰氏阴性微生物，从而制造出可选择性结合 His 标记酶的合成孢子。这些合成孢子可作为生物催化材料，用于将二元醇氧化胺化为氨基醇的一锅式反应，细胞内和细胞外酶之间的协同催化作用促进了这种反应，使其在连续的批处理循环中保持性能。

本文章由计算机程序翻译，如有差异，请以英文原文为准。

摘要图片

查看原文

微信好友朋友圈 QQ好友复制链接

本刊更多论文

Artificial Spores as Multi-Functional Biocatalysts to Perform Biosynthetic Cascades (Adv. Funct. Mater. 45/2024)

Enzyme Immobilization

In article number 2406097, Fernando López-Gallego and co-workers develop a universal method for encapsulating single gram-negative microbes with polymeric coatings to fabricate synthetic spores that selectively bind His-tagged enzymes. These synthetic spores serve as biocatalytic materials for the one-pot oxidative amination of diols into amino alcohols, facilitated by the cooperative catalysis between intracellular and extracellular enzymes that maintain their performance in consecutive batch cycles.

求助全文

通过发布文献求助，成功后即可免费获取论文全文。去求助

来源期刊

Advanced Functional Materials 工程技术-材料科学：综合

CiteScore

29.50

自引率

4.20%

发文量

2086

审稿时长

2.1 months

期刊介绍： Firmly established as a top-tier materials science journal, Advanced Functional Materials reports breakthrough research in all aspects of materials science, including nanotechnology, chemistry, physics, and biology every week. Advanced Functional Materials is known for its rapid and fair peer review, quality content, and high impact, making it the first choice of the international materials science community.