{"title":"燃烧合成 TiO2/C 复合材料，提高光催化 H2O2 产率和太阳能蒸汽蒸发效率","authors":"Yunyun Gong, Yali Cao, Yuanyuan Feng, Wenmiao Zhu, Qinying Li, Meichao Gao","doi":"10.1016/j.matlet.2024.137617","DOIUrl":null,"url":null,"abstract":"<div><div>In this work, a simple combustion method was proposed for the controllable synthesis of TiO<sub>2</sub>/C composites, which can achieve both the efficient solar water evaporation at the interface and photocatalytic H<sub>2</sub>O<sub>2</sub> production. Structural and morphological characteristic indicated the co-existence of carbon quantum dots and amorphous carbon, which were well distributed on the surface of the TiO<sub>2</sub>. TiO<sub>2</sub>/C composites displayed the enhanced visible light absorption and the rapid separation of photogenerated electron-hole pairs. TiO<sub>2</sub>/C-10 exhibited an excellent photocatalytic H<sub>2</sub>O<sub>2</sub> production activity of 3068.46 μmol/g/h under the simulated solar irradiation. Besides, its water evaporation rate reached up to 5.81 kg·m<sup>−2</sup>·h<sup>−1</sup> under the simulated solar irradiation.</div></div>","PeriodicalId":384,"journal":{"name":"Materials Letters","volume":"379 ","pages":"Article 137617"},"PeriodicalIF":2.7000,"publicationDate":"2024-10-28","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Combustion synthesis of TiO2/C composites for enhanced photocatalytic H2O2 production and solar steam evaporation efficiency\",\"authors\":\"Yunyun Gong, Yali Cao, Yuanyuan Feng, Wenmiao Zhu, Qinying Li, Meichao Gao\",\"doi\":\"10.1016/j.matlet.2024.137617\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<div><div>In this work, a simple combustion method was proposed for the controllable synthesis of TiO<sub>2</sub>/C composites, which can achieve both the efficient solar water evaporation at the interface and photocatalytic H<sub>2</sub>O<sub>2</sub> production. Structural and morphological characteristic indicated the co-existence of carbon quantum dots and amorphous carbon, which were well distributed on the surface of the TiO<sub>2</sub>. TiO<sub>2</sub>/C composites displayed the enhanced visible light absorption and the rapid separation of photogenerated electron-hole pairs. TiO<sub>2</sub>/C-10 exhibited an excellent photocatalytic H<sub>2</sub>O<sub>2</sub> production activity of 3068.46 μmol/g/h under the simulated solar irradiation. Besides, its water evaporation rate reached up to 5.81 kg·m<sup>−2</sup>·h<sup>−1</sup> under the simulated solar irradiation.</div></div>\",\"PeriodicalId\":384,\"journal\":{\"name\":\"Materials Letters\",\"volume\":\"379 \",\"pages\":\"Article 137617\"},\"PeriodicalIF\":2.7000,\"publicationDate\":\"2024-10-28\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Materials Letters\",\"FirstCategoryId\":\"88\",\"ListUrlMain\":\"https://www.sciencedirect.com/science/article/pii/S0167577X24017579\",\"RegionNum\":4,\"RegionCategory\":\"材料科学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q3\",\"JCRName\":\"MATERIALS SCIENCE, MULTIDISCIPLINARY\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Materials Letters","FirstCategoryId":"88","ListUrlMain":"https://www.sciencedirect.com/science/article/pii/S0167577X24017579","RegionNum":4,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q3","JCRName":"MATERIALS SCIENCE, MULTIDISCIPLINARY","Score":null,"Total":0}
Combustion synthesis of TiO2/C composites for enhanced photocatalytic H2O2 production and solar steam evaporation efficiency
In this work, a simple combustion method was proposed for the controllable synthesis of TiO2/C composites, which can achieve both the efficient solar water evaporation at the interface and photocatalytic H2O2 production. Structural and morphological characteristic indicated the co-existence of carbon quantum dots and amorphous carbon, which were well distributed on the surface of the TiO2. TiO2/C composites displayed the enhanced visible light absorption and the rapid separation of photogenerated electron-hole pairs. TiO2/C-10 exhibited an excellent photocatalytic H2O2 production activity of 3068.46 μmol/g/h under the simulated solar irradiation. Besides, its water evaporation rate reached up to 5.81 kg·m−2·h−1 under the simulated solar irradiation.
期刊介绍：
Materials Letters has an open access mirror journal Materials Letters: X, sharing the same aims and scope, editorial team, submission system and rigorous peer review.
Materials Letters is dedicated to publishing novel, cutting edge reports of broad interest to the materials community. The journal provides a forum for materials scientists and engineers, physicists, and chemists to rapidly communicate on the most important topics in the field of materials.
Contributions include, but are not limited to, a variety of topics such as:
• Materials - Metals and alloys, amorphous solids, ceramics, composites, polymers, semiconductors
• Applications - Structural, opto-electronic, magnetic, medical, MEMS, sensors, smart
• Characterization - Analytical, microscopy, scanning probes, nanoscopic, optical, electrical, magnetic, acoustic, spectroscopic, diffraction
• Novel Materials - Micro and nanostructures (nanowires, nanotubes, nanoparticles), nanocomposites, thin films, superlattices, quantum dots.
• Processing - Crystal growth, thin film processing, sol-gel processing, mechanical processing, assembly, nanocrystalline processing.
• Properties - Mechanical, magnetic, optical, electrical, ferroelectric, thermal, interfacial, transport, thermodynamic
• Synthesis - Quenching, solid state, solidification, solution synthesis, vapor deposition, high pressure, explosive
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