合成低声子能量的 SrZnOSe 晶体以增强近红外机械发光能力

IF 27.4 1区 材料科学 Q1 CHEMISTRY, MULTIDISCIPLINARY Advanced Materials Pub Date : 2024-11-12 DOI:10.1002/adma.202406899
Yanze Wang, Biyun Ren, Weilin Zheng, Dengfeng Peng, Feng Wang
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引用次数: 0

摘要

近红外(NIR)光具有穿透能力强、抗环境辐射干扰的特点,因此在生物成像和信息技术领域大有可为。本文开发了一类新型掺杂镧系元素的 SrZnOSe 晶体,可在机械激励下自持地产生近红外辐射。拉曼光谱证实,由于硒化物宿主的声子能量较低,SrZnOSe 晶体的近红外发射强度是成熟的 CaZnOS 晶体的 5 倍。这种晶体的潜在用途通过与护齿的集成得到了证明,护齿可以通过咬合力产生明亮的近红外辐射,从而在环境中通过厚组织(最厚达 8 毫米)传输加密的光学信号。这些发现为自恢复机械发光材料的工具箱提供了强有力的补充,并为应用研究开辟了新的可能性。
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Synthesis of SrZnOSe Crystals with Low Phonon Energy for Enhancing Near-Infrared Mechanoluminescence
Near-infrared (NIR) light is promising for bioimaging and information technology due to its high penetration ability and resistance to interference with environmental radiation. Here, a new class of lanthanide-doped SrZnOSe crystals are developed for the self-sustainable generation of NIR emissions under mechanical excitation. It is shown that the SrZnOSe crystals render ≈5-fold stronger NIR emissions than the well-established CaZnOS due to the low phonon energies of the selenide host, as confirmed by Raman spectroscopy. The potential utility of the crystals is demonstrated by integration with a mouthguard, which can generate bright NIR emissions by bite force to transmit encrypted optical signals through thick tissues (up to 8 mm) in ambient environments. The findings provide a powerful addition to the toolbox of self-recovery mechanoluminescent materials and open new possibilities for applied research.
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来源期刊
Advanced Materials
Advanced Materials 工程技术-材料科学:综合
CiteScore
43.00
自引率
4.10%
发文量
2182
审稿时长
2 months
期刊介绍: Advanced Materials, one of the world's most prestigious journals and the foundation of the Advanced portfolio, is the home of choice for best-in-class materials science for more than 30 years. Following this fast-growing and interdisciplinary field, we are considering and publishing the most important discoveries on any and all materials from materials scientists, chemists, physicists, engineers as well as health and life scientists and bringing you the latest results and trends in modern materials-related research every week.
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