非线性手性介质中的光参量放大和振荡。

IF 3.1 2区 化学 Q3 CHEMISTRY, PHYSICAL Journal of Chemical Physics Pub Date : 2024-11-14 DOI:10.1063/5.0231374
Christos Flytzanis, Fredrik Jonsson, Govind P Agrawal
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引用次数: 0

摘要

我们讨论了手性晶体内部光参量放大的非线性过程。我们的研究表明,手性诱导的圆双折射会导致两种不同的非线性过程,它们的相位匹配条件各不相同,并与相反的圆偏振态相关联。只有当入射泵浦光束和信号光束的偏振态均为圆形且正交时,才会发生单一的非线性过程。当这些光束最初为线性偏振时,由于两个相互竞争的非线性过程并行发生,它们的偏振状态会以椭圆的方式演变。我们还讨论了通过在光腔内放置手性非线性晶体而制成的单谐振和双谐振光参量振荡器的特性。
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Optical parametric amplification and oscillation in nonlinear chiral media.

We discuss the nonlinear process of optical parametric amplification inside a chiral crystal. We show that circular birefringence, induced by chirality, leads to two different nonlinear processes with different phase-matching conditions that are associated with the opposite states of circular polarizations. A single nonlinear process occurs only when the states of polarization of the incident pump and signal beams are both circular and orthogonal. When these beams are linearly polarized initially, their state of polarization evolves in an elliptical fashion because of the two competing nonlinear processes taking place in parallel. We also discuss the properties of singly and doubly resonant optical parametric oscillators made by placing a chiral nonlinear crystal inside an optical cavity.

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来源期刊
Journal of Chemical Physics
Journal of Chemical Physics 物理-物理:原子、分子和化学物理
CiteScore
7.40
自引率
15.90%
发文量
1615
审稿时长
2 months
期刊介绍: The Journal of Chemical Physics publishes quantitative and rigorous science of long-lasting value in methods and applications of chemical physics. The Journal also publishes brief Communications of significant new findings, Perspectives on the latest advances in the field, and Special Topic issues. The Journal focuses on innovative research in experimental and theoretical areas of chemical physics, including spectroscopy, dynamics, kinetics, statistical mechanics, and quantum mechanics. In addition, topical areas such as polymers, soft matter, materials, surfaces/interfaces, and systems of biological relevance are of increasing importance. Topical coverage includes: Theoretical Methods and Algorithms Advanced Experimental Techniques Atoms, Molecules, and Clusters Liquids, Glasses, and Crystals Surfaces, Interfaces, and Materials Polymers and Soft Matter Biological Molecules and Networks.
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