金红石氧化物 RuO_{2} 中不存在异磁自旋分裂特性。

IF 8.1 1区 物理与天体物理 Q1 PHYSICS, MULTIDISCIPLINARY Physical review letters Pub Date : 2024-10-25 DOI:10.1103/PhysRevLett.133.176401
Jiayu Liu, Jie Zhan, Tongrui Li, Jishan Liu, Shufan Cheng, Yuming Shi, Liwei Deng, Meng Zhang, Chihao Li, Jianyang Ding, Qi Jiang, Mao Ye, Zhengtai Liu, Zhicheng Jiang, Siyu Wang, Qian Li, Yanwu Xie, Yilin Wang, Shan Qiao, Jinsheng Wen, Yan Sun, Dawei Shen
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引用次数: 0

摘要

金红石 RuO_{2} 已被认为是一种潜在的 d 波改磁候选物质,据预测,其显著的自旋分裂可达 1.4 eV。尽管理论预测和输运测量不断积累,但对自旋分裂的直接光谱观测却始终难以实现。在这里,我们采用自旋和角度分辨光发射光谱来研究薄膜和单晶 RuO_{2} 的能带结构和自旋极化。与对反磁性的预期相反,我们的分析表明 RuO_{2} 的电子结构与在非磁性条件下预测的电子结构一致,没有表现出假设的自旋分裂。此外,我们还观察到低洼的体带有明显的面内自旋极化现象,这种现象与高对称面是反对称的,并且与变磁性中时间反转对称破缺导致的 d 波自旋纹理相反。这些发现明确地挑战了之前提出的金红石 RuO_{2} 的反磁性顺序,促使人们重新评估其磁性能。
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Absence of Altermagnetic Spin Splitting Character in Rutile Oxide RuO_{2}.

Rutile RuO_{2} has been posited as a potential d-wave altermagnetism candidate, with a predicted significant spin splitting up to 1.4 eV. Despite accumulating theoretical predictions and transport measurements, direct spectroscopic observation of spin splitting has remained elusive. Here, we employ spin- and angle-resolved photoemission spectroscopy to investigate the band structures and spin polarization of thin-film and single-crystal RuO_{2}. Contrary to expectations of altermagnetism, our analysis indicates that RuO_{2}'s electronic structure aligns with those predicted under nonmagnetic conditions, exhibiting no evidence of the hypothesized spin splitting. Additionally, we observe significant in-plane spin polarization of the low-lying bulk bands, which is antisymmetric about the high-symmetry plane and contrary to the d-wave spin texture due to time-reversal symmetry breaking in altermagnetism. These findings definitively challenge the altermagnetic order previously proposed for rutile RuO_{2}, prompting a reevaluation of its magnetic properties.

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来源期刊
Physical review letters
Physical review letters 物理-物理:综合
CiteScore
16.50
自引率
7.00%
发文量
2673
审稿时长
2.2 months
期刊介绍: Physical review letters(PRL)covers the full range of applied, fundamental, and interdisciplinary physics research topics: General physics, including statistical and quantum mechanics and quantum information Gravitation, astrophysics, and cosmology Elementary particles and fields Nuclear physics Atomic, molecular, and optical physics Nonlinear dynamics, fluid dynamics, and classical optics Plasma and beam physics Condensed matter and materials physics Polymers, soft matter, biological, climate and interdisciplinary physics, including networks
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