Zhonghang Chen, Peiyu Fang, Jiangnan Li, Xue Han, Wenhao Huang, Wenyue Cui, Zhiwei Liu, Mark R Warren, David Allan, Peng Cheng, Sihai Yang, Wei Shi
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引用次数: 0
摘要
由于苯和环己烷的沸点几乎相同,目前从环己烷中萃取痕量苯是通过高能耗的萃取蒸馏法进行的。多孔材料对它们的吸附分离因其尺寸相似而受到阻碍。具有多种孔隙环境的金属有机框架(MOFs)能够进行分子分辨,但液相中痕量底物的分离仍然极具挑战性。在此,我们报告了一种具有冠醚装饰的三角形通道的坚固 MOF(NKU-300),它可以从环己烷中分辨出痕量苯,对苯/环己烷混合物(v/v = 1/1000)的选择性高达 8615(10),这是前所未有的。值得注意的是,NKU-300 在 0.1%-50% 的广泛浓度范围内从环己烷中萃取苯时表现出卓越的选择性、超快的吸附动力学和出色的稳定性。单晶 X 射线衍射和计算建模显示,多种超分子相互作用协同固定了三角形通道中的苯分子,从而实现了卓越的分离性能。这项研究将促进具有定制结合位点的先进吸附剂在具有挑战性的工业分离中的应用。
Rapid extraction of trace benzene by a crown-ether-based metal-organic framework.
Due to almost identical boiling points of benzene and cyclohexane, the extraction of trace benzene from cyclohexane is currently performed via the energy-intensive extractive distillation method. Their adsorptive separation by porous materials is hampered by their similar dimensions. Metal-organic frameworks (MOFs) with versatile pore environments are capable of molecular discrimination, but the separation of trace substrates in liquid-phase remains extremely challenging. Herein, we report a robust MOF (NKU-300) with triangular channels decorated with crown ether that can discriminate trace benzene from cyclohexane, exhibiting an unprecedented selectivity of 8615(10) for the mixture of benzene/cyclohexane (v/v = 1/1000). Remarkably, NKU-300 demonstrates exceptional selectivities for the extraction of benzene from cyclohexane over a wide range of concentrations of 0.1%-50% with ultrafast sorption kinetics and excellent stability. Single-crystal X-ray diffraction and computational modelling reveal that multiple supramolecular interactions cooperatively immobilise benzene molecules in the triangular channel, enabling superior separation performance. This study will promote the application of advanced sorbents with tailored binding sites for challenging industrial separations.
期刊介绍:
National Science Review (NSR; ISSN abbreviation: Natl. Sci. Rev.) is an English-language peer-reviewed multidisciplinary open-access scientific journal published by Oxford University Press under the auspices of the Chinese Academy of Sciences.According to Journal Citation Reports, its 2021 impact factor was 23.178.
National Science Review publishes both review articles and perspectives as well as original research in the form of brief communications and research articles.