电催化微环境调节的最新进展。

IF 16.3 1区 综合性期刊 Q1 MULTIDISCIPLINARY SCIENCES National Science Review Pub Date : 2024-09-19 eCollection Date: 2024-12-01 DOI:10.1093/nsr/nwae315
Zhiyuan Xu, Xin Tan, Chang Chen, Xingdong Wang, Rui Sui, Zhongbin Zhuang, Chao Zhang, Chen Chen
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引用次数: 0

摘要

高效电催化可作为连接可再生能源技术、氢经济和碳捕获/利用的桥梁,为人类带来可持续发展的未来。因此,探索可行的策略来调节相关电催化反应并优化设备性能,从而促进其大规模实际应用,具有极其重要的意义。催化界面的微环境调节已被证明能够有效提高反应速率并改善特定产物的选择性。在这篇综述中,我们总结了典型电催化过程(包括水电解、氢氧燃料电池和二氧化碳还原)中微环境调节的最新进展,以及相关的原位/操作表征技术和理论模拟方法。文章最后,我们对发展趋势和未来可能的发展方向进行了展望。
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Recent advances in microenvironment regulation for electrocatalysis.

High-efficiency electrocatalysis could serve as the bridge that connects renewable energy technologies, hydrogen economy and carbon capture/utilization, promising a sustainable future for humankind. It is therefore of paramount significance to explore feasible strategies to modulate the relevant electrocatalytic reactions and optimize device performances so as to promote their large-scale practical applications. Microenvironment regulation at the catalytic interface has been demonstrated to be capable of effectively enhancing the reaction rates and improving the selectivities for specific products. In this review we summarize the latest advances in microenvironment regulation in typical electrocatalytic processes (including water electrolysis, hydrogen-oxygen fuel cells, and carbon dioxide reduction) and the related in situ/operando characterization techniques and theoretical simulation methods. At the end of this article, we present an outlook on development trends and possible future directions.

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来源期刊
National Science Review
National Science Review MULTIDISCIPLINARY SCIENCES-
CiteScore
24.10
自引率
1.90%
发文量
249
审稿时长
13 weeks
期刊介绍: National Science Review (NSR; ISSN abbreviation: Natl. Sci. Rev.) is an English-language peer-reviewed multidisciplinary open-access scientific journal published by Oxford University Press under the auspices of the Chinese Academy of Sciences.According to Journal Citation Reports, its 2021 impact factor was 23.178. National Science Review publishes both review articles and perspectives as well as original research in the form of brief communications and research articles.
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