Chao Zhang , Guofu Liu , Xin Zhang , Angang Song , Dan Xu , Xiaowu Jiang , Chenghong Gong , Xiaobo Zhou , Qiuping Gong , Dekui Shen
{"title":"基于选择性催化还原系统实时氮氧化物通量分布特征的分区动态喷氨策略","authors":"Chao Zhang , Guofu Liu , Xin Zhang , Angang Song , Dan Xu , Xiaowu Jiang , Chenghong Gong , Xiaobo Zhou , Qiuping Gong , Dekui Shen","doi":"10.1016/j.fuel.2024.133711","DOIUrl":null,"url":null,"abstract":"<div><div>To optimize the NO<sub>x</sub>/NH<sub>3</sub> (Nitrogen Oxides/Ammonia) matching ratio for a SCR (Selective Catalytic Reduction) system, dynamic NH<sub>3</sub> injection was achieved on the basis of the constructed control rules for critical AIG (Ammonia Injection Grid) branch-pipe valves via the determination of the basic NH<sub>3</sub> injection amount and the secondarily distributed NH<sub>3</sub> injection amount. Moreover, the real-time NO<sub>x</sub> flux distribution characteristics in each subzone were analysed on the basis of the operation data of the flue gas velocity and NO<sub>x</sub> concentration originating from multiple measuring points located in the flue cross-section which is in front of the AIG. The engineering application results of a 350 MW coal-fired unit revealed that 12 “critical” AIG branch-pipe valves achieved dynamic NH<sub>3</sub> injection. With a maximum fluctuation in NO<sub>x</sub> flux of 433 mol/h in the subzone of the individual flue cross-section, the opening of this AIG branch-pipe valve was subsequently adjusted by 22° to optimize the NO<sub>x</sub>/NH<sub>3</sub> matching ratio in the system in a timely manner. The ACRs (Ammonia Consumption Rates) of the A and B sides in the studied SCR system were reduced by approximately 26.70 % and 11.90 %, respectively. In addition, the average RSD (Relative Standard Deviation) of the NO<sub>x</sub> concentration at the outlet of the SCR reactor for sides A and B were approximately 11.9 % and 13.6 %, which were reduced by approximately 11.63 % and 15.47 %, respectively, owing to the application of the dynamic NH<sub>3</sub> injection strategy.</div></div>","PeriodicalId":325,"journal":{"name":"Fuel","volume":"381 ","pages":"Article 133711"},"PeriodicalIF":6.7000,"publicationDate":"2024-11-13","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"A partitioned dynamic ammonia injection strategy based on real-time NOx flux distribution characteristics in an SCR system\",\"authors\":\"Chao Zhang , Guofu Liu , Xin Zhang , Angang Song , Dan Xu , Xiaowu Jiang , Chenghong Gong , Xiaobo Zhou , Qiuping Gong , Dekui Shen\",\"doi\":\"10.1016/j.fuel.2024.133711\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<div><div>To optimize the NO<sub>x</sub>/NH<sub>3</sub> (Nitrogen Oxides/Ammonia) matching ratio for a SCR (Selective Catalytic Reduction) system, dynamic NH<sub>3</sub> injection was achieved on the basis of the constructed control rules for critical AIG (Ammonia Injection Grid) branch-pipe valves via the determination of the basic NH<sub>3</sub> injection amount and the secondarily distributed NH<sub>3</sub> injection amount. Moreover, the real-time NO<sub>x</sub> flux distribution characteristics in each subzone were analysed on the basis of the operation data of the flue gas velocity and NO<sub>x</sub> concentration originating from multiple measuring points located in the flue cross-section which is in front of the AIG. The engineering application results of a 350 MW coal-fired unit revealed that 12 “critical” AIG branch-pipe valves achieved dynamic NH<sub>3</sub> injection. With a maximum fluctuation in NO<sub>x</sub> flux of 433 mol/h in the subzone of the individual flue cross-section, the opening of this AIG branch-pipe valve was subsequently adjusted by 22° to optimize the NO<sub>x</sub>/NH<sub>3</sub> matching ratio in the system in a timely manner. The ACRs (Ammonia Consumption Rates) of the A and B sides in the studied SCR system were reduced by approximately 26.70 % and 11.90 %, respectively. In addition, the average RSD (Relative Standard Deviation) of the NO<sub>x</sub> concentration at the outlet of the SCR reactor for sides A and B were approximately 11.9 % and 13.6 %, which were reduced by approximately 11.63 % and 15.47 %, respectively, owing to the application of the dynamic NH<sub>3</sub> injection strategy.</div></div>\",\"PeriodicalId\":325,\"journal\":{\"name\":\"Fuel\",\"volume\":\"381 \",\"pages\":\"Article 133711\"},\"PeriodicalIF\":6.7000,\"publicationDate\":\"2024-11-13\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Fuel\",\"FirstCategoryId\":\"5\",\"ListUrlMain\":\"https://www.sciencedirect.com/science/article/pii/S0016236124028606\",\"RegionNum\":1,\"RegionCategory\":\"工程技术\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q2\",\"JCRName\":\"ENERGY & FUELS\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Fuel","FirstCategoryId":"5","ListUrlMain":"https://www.sciencedirect.com/science/article/pii/S0016236124028606","RegionNum":1,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q2","JCRName":"ENERGY & FUELS","Score":null,"Total":0}
A partitioned dynamic ammonia injection strategy based on real-time NOx flux distribution characteristics in an SCR system
To optimize the NOx/NH3 (Nitrogen Oxides/Ammonia) matching ratio for a SCR (Selective Catalytic Reduction) system, dynamic NH3 injection was achieved on the basis of the constructed control rules for critical AIG (Ammonia Injection Grid) branch-pipe valves via the determination of the basic NH3 injection amount and the secondarily distributed NH3 injection amount. Moreover, the real-time NOx flux distribution characteristics in each subzone were analysed on the basis of the operation data of the flue gas velocity and NOx concentration originating from multiple measuring points located in the flue cross-section which is in front of the AIG. The engineering application results of a 350 MW coal-fired unit revealed that 12 “critical” AIG branch-pipe valves achieved dynamic NH3 injection. With a maximum fluctuation in NOx flux of 433 mol/h in the subzone of the individual flue cross-section, the opening of this AIG branch-pipe valve was subsequently adjusted by 22° to optimize the NOx/NH3 matching ratio in the system in a timely manner. The ACRs (Ammonia Consumption Rates) of the A and B sides in the studied SCR system were reduced by approximately 26.70 % and 11.90 %, respectively. In addition, the average RSD (Relative Standard Deviation) of the NOx concentration at the outlet of the SCR reactor for sides A and B were approximately 11.9 % and 13.6 %, which were reduced by approximately 11.63 % and 15.47 %, respectively, owing to the application of the dynamic NH3 injection strategy.
期刊介绍:
The exploration of energy sources remains a critical matter of study. For the past nine decades, fuel has consistently held the forefront in primary research efforts within the field of energy science. This area of investigation encompasses a wide range of subjects, with a particular emphasis on emerging concerns like environmental factors and pollution.