通过分子束外延生长的高质量砷化镓同外延层

IF 1.7 4区 材料科学 Q3 CRYSTALLOGRAPHY Journal of Crystal Growth Pub Date : 2024-11-05 DOI:10.1016/j.jcrysgro.2024.127989
Hao Zhou , Yiqiao Chen , Chang Liu
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引用次数: 0

摘要

在广泛的衬底温度、As2/In 通量比和生长速率范围内,对通过分子束外延进行 InAs 同外延的生长条件进行了全面研究。研究发现,InAs 层的表面形态和整体质量受到这些参数的显著影响。最佳条件,包括较低的生长温度、较低的 As2 通量和较慢的生长速度,是获得高质量 InAs 层的关键。在评估材料质量时,采用了两种主要表征技术,即微分干涉对比显微镜和原子力显微镜。在基底温度为 455 ℃、生长速度为 0.33 单层/秒 (ML/s) 的条件下,成功生长出了高质量的砷化镓同向外延层。这些层的缺陷密度非常低,约为每平方厘米 300 个缺陷,比以前报道的低了一个数量级以上,而且均方根粗糙度也非常低,仅为 0.116 nm。在 0.33 ML/s 的生长速率下,发现 InAs 同向外延层的生长温度范围相当宽,而 As2/In 通量比则保持在较窄的范围内。这项研究强调了在分子束外延过程中精确控制生长参数对生产高质量砷化铟同外延层的关键作用。
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High-quality InAs homoepitaxial layers grown by molecular beam epitaxy
The growth conditions for InAs homoepitaxy by molecular beam epitaxy were comprehensively studied across a broad spectrum of substrate temperatures, As2/In flux ratios, and growth rates. It was found that the surface morphology and overall quality of the InAs layers were significantly influenced by these parameters. Optimal conditions, including a lower growth temperature, reduced As2 flux, and slower growth rate, were pivotal in achieving high-quality InAs layers. Two primary characterization techniques, differential interference contrast microscopy and atomic force microscopy, were employed to evaluate the material quality. High-quality InAs homoepitaxial layers were successfully grown at a substrate temperature of 455 °C and a growth rate of 0.33 monolayers per second (ML/s). These layers exhibited a remarkably low defect density of approximately 300 defects per square centimeter, which is over an order of magnitude lower than previously reported, and a notably low root-mean-square roughness of 0.116 nm. At a growth rate of 0.33 ML/s, the growth temperature range for InAs homoepitaxial layers was found to be quite broad, whereas the As2/In flux ratio remained within a narrow range. This study underscores the critical role of precise control over growth parameters in the molecular beam epitaxy process for producing high-quality InAs homoepitaxial layers.
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来源期刊
Journal of Crystal Growth
Journal of Crystal Growth 化学-晶体学
CiteScore
3.60
自引率
11.10%
发文量
373
审稿时长
65 days
期刊介绍: The journal offers a common reference and publication source for workers engaged in research on the experimental and theoretical aspects of crystal growth and its applications, e.g. in devices. Experimental and theoretical contributions are published in the following fields: theory of nucleation and growth, molecular kinetics and transport phenomena, crystallization in viscous media such as polymers and glasses; crystal growth of metals, minerals, semiconductors, superconductors, magnetics, inorganic, organic and biological substances in bulk or as thin films; molecular beam epitaxy, chemical vapor deposition, growth of III-V and II-VI and other semiconductors; characterization of single crystals by physical and chemical methods; apparatus, instrumentation and techniques for crystal growth, and purification methods; multilayer heterostructures and their characterisation with an emphasis on crystal growth and epitaxial aspects of electronic materials. A special feature of the journal is the periodic inclusion of proceedings of symposia and conferences on relevant aspects of crystal growth.
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