用 252Cf 混合放射性核素辐照混凝土掺杂磁铁矿的剂量评估和辐射屏蔽特性:瓦特裂变方法和多普勒效应

IF 2.8 3区 物理与天体物理 Q3 CHEMISTRY, PHYSICAL Radiation Physics and Chemistry Pub Date : 2024-11-04 DOI:10.1016/j.radphyschem.2024.112364
Roya Boudaghi Malidarreh , N. Almousa , Iskender Akkurt , Shams A.M. Issa , Hesham M.H. Zakaly
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引用次数: 0

摘要

核聚变反应堆、核电站和医疗机构发出的核辐射对生物体人员构成潜在风险,因此必须采取防护措施。为了加强对患者工作人员的辐射防护,可以使用各种材料。添加了各种添加剂的混凝土历来是一种屏蔽材料。因此,近期的研究主要集中在通过改变混凝土的成分来增强其衰减核源发射的有害能量的能力。因此,本研究采用 MCNPX 蒙特卡洛(MC)方法和 252Cf 混合辐射放射性核素的理论计算,分析了 CM-0(对照样本)、CM-25、CM-50、CM-75 和 CM-100 等一系列混凝土磁铁矿(CM)配方的剂量评估和辐射屏蔽特性。在这项工作中,采用了瓦特裂变分布来推导 CM 样品的中子谱,并彻底阐明了在存在和不存在指定样品时的结果。然后,利用多普勒效应,提取并描述了暴露于自发裂变 252Cf 源的屏蔽材料中的伽马光子谱。半值厚度(HVT)和平均自由路径(MFP)的估算适用于广泛的能级谱。分析证实了新型混凝土磁铁矿(CM)样品的成功开发,与对照样品相比,该样品的辐照度更低。这项研究为利用混凝土屏蔽混合辐射放射性核素提供了有价值的见解,并为今后涉及类似材料的研究打开了大门。具体来说,CM-100 样品的半值厚度(HVT)最低,能最有效地减少中子和伽马辐射。研究结果表明,提高混凝土中磁铁矿的浓度可大大增强其屏蔽中子-伽马混合辐射的能力。这一创新在辐射防护领域,尤其是核反应堆和医疗设施中的应用前景广阔。CM-100 样品显示出明显的改进,HVT 达到 0.012 厘米,剂量率降低了 2.95 × 10-9 Sv.h-1,而对照样品(CM-0)的 HVT 为 10.358 厘米,等效剂量率为 2.84 × 10-9 Sv.h-1。这些结果表明,掺磁铁矿的混凝土配方具有卓越的屏蔽性能。
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A closer look to dose assessment and radiation shielding characteristics of concrete doped magnetite irradiated with 252Cf mixed radiation radionuclide: A Watt Fission approach and Doppler effect
Nuclear radiation emitted by fusion reactors, nuclear power plants, and medical establishments presents potential risks to living organisms personnel, necessitating the implementation of protective measures. To enhance radiation protection for patients workers, various materials can be utilized. Concrete, augmented with various additives, has historically acted as a shielding material. Hence, recent research has predominantly focused on enhancing concrete's ability to attenuate the harmful energy emitted by nuclear sources through modifications to its composition. Accordingly, in the present work, the dose evaluation and radiation shielding characteristics of a range of concrete magnetite (CM) formulations designated as CM-0 (control sample), CM-25, CM-50, CM-75, and CM-100 have been analyzed using MCNPX Monte Carlo (MC) approach and theoretical computations concerning 252Cf mixed radiation radionuclide. In this work, the Watt Fission distribution was employed to derive the neutron spectrum of CM samples, and findings have been thoroughly elucidated in the presence and absence of the specified samples. Then, utilizing the Doppler Effect, the gamma photon spectrum within shielding materials exposed to a spontaneous fission 252Cf source is extracted and characterized. Estimation of Half Value Thickness (HVT) and Mean Free Path (MFP) are provided across a broad spectrum of energy levels. The analysis confirms the successful development of a new type of concrete magnetite (CM) sample that exhibits lower radiation exposure compared to the control sample. This study offers valuable insights into the use of concrete in shielding against mixed radiation radionuclides and opens the door for future research involving similar materials. Specifically, the CM-100 sample demonstrated the lowest half-value thickness (HVT) and provided the most effective reduction of both neutron and gamma radiation. The findings suggest that increasing the concentration of magnetite in concrete greatly enhances its ability to shield against mixed neutron-gamma radiation. This innovation has promising potential for applications in radiation protection, particularly within nuclear reactors and medical facilities. The CM-100 sample showed a notable improvement, achieving an HVT of 0.012 cm and a dose rate reduction of 2.95 × 10−9 Sv.h−1, in contrast to the control sample (CM-0), which had an HVT of 10.358 cm and an equivalent dose rate of 2.84 × 10−9 Sv.h−1. These results underscore the superior shielding properties of the magnetite-doped concrete formulations.
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来源期刊
Radiation Physics and Chemistry
Radiation Physics and Chemistry 化学-核科学技术
CiteScore
5.60
自引率
17.20%
发文量
574
审稿时长
12 weeks
期刊介绍: Radiation Physics and Chemistry is a multidisciplinary journal that provides a medium for publication of substantial and original papers, reviews, and short communications which focus on research and developments involving ionizing radiation in radiation physics, radiation chemistry and radiation processing. The journal aims to publish papers with significance to an international audience, containing substantial novelty and scientific impact. The Editors reserve the rights to reject, with or without external review, papers that do not meet these criteria. This could include papers that are very similar to previous publications, only with changed target substrates, employed materials, analyzed sites and experimental methods, report results without presenting new insights and/or hypothesis testing, or do not focus on the radiation effects.
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