B. Franco, L. Clarisse, M. Van Damme, J. Hadji-Lazaro, C. Clerbaux, P. Coheur
{"title":"基于卫星的大型人为 NMVOC 排放源识别","authors":"B. Franco, L. Clarisse, M. Van Damme, J. Hadji-Lazaro, C. Clerbaux, P. Coheur","doi":"10.1029/2024JD042047","DOIUrl":null,"url":null,"abstract":"<p>Nonmethane volatile organic compounds (NMVOCs) emitted in excess from anthropogenic sources significantly contribute to the formation of harmful pollutants, thereby degrading air quality. While satellite measurements have become valuable tools for tracking anthropogenic emitters, they have primarily targeted inorganic species and methane (<span></span><math>\n <semantics>\n <mrow>\n <msub>\n <mtext>CH</mtext>\n <mn>4</mn>\n </msub>\n </mrow>\n <annotation> ${\\text{CH}}_{4}$</annotation>\n </semantics></math>). This study demonstrates the potential of infrared atmospheric sounding interferometers (IASI) to detect anthropogenic NMVOC point sources on a global scale. Using an advanced oversampling technique, we enhance the spatial resolution of IASI measurements to identify emitters of three major NMVOCs: methanol (<span></span><math>\n <semantics>\n <mrow>\n <msub>\n <mtext>CH</mtext>\n <mn>3</mn>\n </msub>\n </mrow>\n <annotation> ${\\text{CH}}_{3}$</annotation>\n </semantics></math>OH), acetylene (<span></span><math>\n <semantics>\n <mrow>\n <msub>\n <mi>C</mi>\n <mn>2</mn>\n </msub>\n <msub>\n <mi>H</mi>\n <mn>2</mn>\n </msub>\n </mrow>\n <annotation> ${\\mathrm{C}}_{2}{\\mathrm{H}}_{2}$</annotation>\n </semantics></math>), and propylene (<span></span><math>\n <semantics>\n <mrow>\n <msub>\n <mi>C</mi>\n <mn>3</mn>\n </msub>\n <msub>\n <mi>H</mi>\n <mn>6</mn>\n </msub>\n </mrow>\n <annotation> ${\\mathrm{C}}_{3}{\\mathrm{H}}_{6}$</annotation>\n </semantics></math>). These point sources are primarily associated with chemical and petrochemical facilities, coal-burning activities, metallurgy, pharmaceutical manufacturing sites, and megacities. We also highlight the value of combining IASI measurements of NMVOCs with those of the inorganic species, such as sulfur dioxide (<span></span><math>\n <semantics>\n <mrow>\n <msub>\n <mtext>SO</mtext>\n <mn>2</mn>\n </msub>\n </mrow>\n <annotation> ${\\text{SO}}_{2}$</annotation>\n </semantics></math>) and ammonia (<span></span><math>\n <semantics>\n <mrow>\n <msub>\n <mtext>NH</mtext>\n <mn>3</mn>\n </msub>\n </mrow>\n <annotation> ${\\text{NH}}_{3}$</annotation>\n </semantics></math>), to aid in the identification of anthropogenic point sources.</p>","PeriodicalId":15986,"journal":{"name":"Journal of Geophysical Research: Atmospheres","volume":"129 22","pages":""},"PeriodicalIF":3.8000,"publicationDate":"2024-11-16","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1029/2024JD042047","citationCount":"0","resultStr":"{\"title\":\"Satellite-Based Identification of Large Anthropogenic NMVOC Emission Sources\",\"authors\":\"B. Franco, L. Clarisse, M. Van Damme, J. Hadji-Lazaro, C. Clerbaux, P. Coheur\",\"doi\":\"10.1029/2024JD042047\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<p>Nonmethane volatile organic compounds (NMVOCs) emitted in excess from anthropogenic sources significantly contribute to the formation of harmful pollutants, thereby degrading air quality. While satellite measurements have become valuable tools for tracking anthropogenic emitters, they have primarily targeted inorganic species and methane (<span></span><math>\\n <semantics>\\n <mrow>\\n <msub>\\n <mtext>CH</mtext>\\n <mn>4</mn>\\n </msub>\\n </mrow>\\n <annotation> ${\\\\text{CH}}_{4}$</annotation>\\n </semantics></math>). This study demonstrates the potential of infrared atmospheric sounding interferometers (IASI) to detect anthropogenic NMVOC point sources on a global scale. Using an advanced oversampling technique, we enhance the spatial resolution of IASI measurements to identify emitters of three major NMVOCs: methanol (<span></span><math>\\n <semantics>\\n <mrow>\\n <msub>\\n <mtext>CH</mtext>\\n <mn>3</mn>\\n </msub>\\n </mrow>\\n <annotation> ${\\\\text{CH}}_{3}$</annotation>\\n </semantics></math>OH), acetylene (<span></span><math>\\n <semantics>\\n <mrow>\\n <msub>\\n <mi>C</mi>\\n <mn>2</mn>\\n </msub>\\n <msub>\\n <mi>H</mi>\\n <mn>2</mn>\\n </msub>\\n </mrow>\\n <annotation> ${\\\\mathrm{C}}_{2}{\\\\mathrm{H}}_{2}$</annotation>\\n </semantics></math>), and propylene (<span></span><math>\\n <semantics>\\n <mrow>\\n <msub>\\n <mi>C</mi>\\n <mn>3</mn>\\n </msub>\\n <msub>\\n <mi>H</mi>\\n <mn>6</mn>\\n </msub>\\n </mrow>\\n <annotation> ${\\\\mathrm{C}}_{3}{\\\\mathrm{H}}_{6}$</annotation>\\n </semantics></math>). These point sources are primarily associated with chemical and petrochemical facilities, coal-burning activities, metallurgy, pharmaceutical manufacturing sites, and megacities. We also highlight the value of combining IASI measurements of NMVOCs with those of the inorganic species, such as sulfur dioxide (<span></span><math>\\n <semantics>\\n <mrow>\\n <msub>\\n <mtext>SO</mtext>\\n <mn>2</mn>\\n </msub>\\n </mrow>\\n <annotation> ${\\\\text{SO}}_{2}$</annotation>\\n </semantics></math>) and ammonia (<span></span><math>\\n <semantics>\\n <mrow>\\n <msub>\\n <mtext>NH</mtext>\\n <mn>3</mn>\\n </msub>\\n </mrow>\\n <annotation> ${\\\\text{NH}}_{3}$</annotation>\\n </semantics></math>), to aid in the identification of anthropogenic point sources.</p>\",\"PeriodicalId\":15986,\"journal\":{\"name\":\"Journal of Geophysical Research: Atmospheres\",\"volume\":\"129 22\",\"pages\":\"\"},\"PeriodicalIF\":3.8000,\"publicationDate\":\"2024-11-16\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"https://onlinelibrary.wiley.com/doi/epdf/10.1029/2024JD042047\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Journal of Geophysical Research: Atmospheres\",\"FirstCategoryId\":\"89\",\"ListUrlMain\":\"https://onlinelibrary.wiley.com/doi/10.1029/2024JD042047\",\"RegionNum\":2,\"RegionCategory\":\"地球科学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q2\",\"JCRName\":\"METEOROLOGY & ATMOSPHERIC SCIENCES\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Journal of Geophysical Research: Atmospheres","FirstCategoryId":"89","ListUrlMain":"https://onlinelibrary.wiley.com/doi/10.1029/2024JD042047","RegionNum":2,"RegionCategory":"地球科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q2","JCRName":"METEOROLOGY & ATMOSPHERIC SCIENCES","Score":null,"Total":0}
Satellite-Based Identification of Large Anthropogenic NMVOC Emission Sources
Nonmethane volatile organic compounds (NMVOCs) emitted in excess from anthropogenic sources significantly contribute to the formation of harmful pollutants, thereby degrading air quality. While satellite measurements have become valuable tools for tracking anthropogenic emitters, they have primarily targeted inorganic species and methane (). This study demonstrates the potential of infrared atmospheric sounding interferometers (IASI) to detect anthropogenic NMVOC point sources on a global scale. Using an advanced oversampling technique, we enhance the spatial resolution of IASI measurements to identify emitters of three major NMVOCs: methanol (OH), acetylene (), and propylene (). These point sources are primarily associated with chemical and petrochemical facilities, coal-burning activities, metallurgy, pharmaceutical manufacturing sites, and megacities. We also highlight the value of combining IASI measurements of NMVOCs with those of the inorganic species, such as sulfur dioxide () and ammonia (), to aid in the identification of anthropogenic point sources.
期刊介绍:
JGR: Atmospheres publishes articles that advance and improve understanding of atmospheric properties and processes, including the interaction of the atmosphere with other components of the Earth system.