用于连续太阳能海水淡化的低成本、环保、高性能三维激光诱导石墨烯蒸发器。

IF 15.8 1区 材料科学 Q1 CHEMISTRY, MULTIDISCIPLINARY ACS Nano Pub Date : 2024-11-18 DOI:10.1021/acsnano.4c12553
Truong-Son Dinh Le, Dongwook Yang, Han Ku Nam, Younggeun Lee, Chwee Teck Lim, Bong Jae Lee, Seung-Woo Kim, Young-Jin Kim
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引用次数: 0

摘要

由于气候变化、森林砍伐、人口增长和水资源需求增加,水资源短缺已成为全球性挑战。虽然先进的制水厂在城市地区很普遍,但偏远岛屿和人口稀少地区在建立此类技术方面却面临着巨大障碍。因此,这些地区迫切需要高效、经济、可持续的制水技术。在本文中,我们介绍了一种利用超短脉冲激光在环境条件下直接将棉织物转化为石墨烯的简便方法。由此产生的激光诱导石墨烯(LIG)具有最高的光吸收率(99.0%)和宽广的吸收范围(250-2500 nm)。作为一种优异的太阳能吸收剂,棉织物上的石墨烯可有效吸收 98.6% 的太阳总辐照度,其表面温度在阳光照射下可达到 84.5 °C,且无需光学浓缩。此外,我们还提出了一种经济高效的三维 LIG 蒸发器(LIGE),用于连续太阳能海水淡化。这一创新设计有效缓解了盐形成问题,并提高了蒸汽产生效率。经测量,水蒸发率和太阳能到水蒸气的转换效率分别约为 1.709 kg m-2 h-1 和 95.1%,超过了以往研究的结果。三维 LIGE 的简易性、耐用性和连续运行能力为应对全球水资源短缺日益严峻的挑战提供了广阔的前景。
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Low-Cost, Eco-Friendly, and High-Performance 3D Laser-Induced Graphene Evaporator for Continuous Solar-Powered Water Desalination.

Water scarcity has become a global challenge attributed to climate change, deforestation, population growth, and increasing water demand. While advanced water production plants are prevalent in urban areas, remote islands and sparsely populated regions face significant obstacles in establishing such technologies. Consequently, there is an urgent need for efficient, affordable, and sustainable water production technologies in these areas. Herein, we present a facile approach utilizing an ultrashort-pulsed laser to directly convert cotton fabric into graphene under ambient conditions. The resulting laser-induced graphene (LIG) demonstrates the highest light absorption efficiency of 99.0% and a broad absorption range (250-2500 nm). As an excellent solar absorber, LIG on cotton fabric can efficiently absorb 98.6% of the total solar irradiance and its surface temperature can reach 84.5 °C under sunlight without optical concentration. Moreover, we propose a cost-effective 3D LIG evaporator (LIGE) for continuous solar-powered desalination. This innovative design effectively mitigates salt formation issues and enhances the steam generation efficiency. The water evaporation rate and the solar-to-vapor conversion efficiency are measured to be around 1.709 kg m-2 h-1 and 95.1%, respectively, which surpass those reported in previous studies. The simplicity, durability, and continuous operational capability of the 3D LIGE offer promising prospects to address the growing challenges in global water scarcity.

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来源期刊
ACS Nano
ACS Nano 工程技术-材料科学:综合
CiteScore
26.00
自引率
4.10%
发文量
1627
审稿时长
1.7 months
期刊介绍: ACS Nano, published monthly, serves as an international forum for comprehensive articles on nanoscience and nanotechnology research at the intersections of chemistry, biology, materials science, physics, and engineering. The journal fosters communication among scientists in these communities, facilitating collaboration, new research opportunities, and advancements through discoveries. ACS Nano covers synthesis, assembly, characterization, theory, and simulation of nanostructures, nanobiotechnology, nanofabrication, methods and tools for nanoscience and nanotechnology, and self- and directed-assembly. Alongside original research articles, it offers thorough reviews, perspectives on cutting-edge research, and discussions envisioning the future of nanoscience and nanotechnology.
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