大型燃煤活动引发的工业干热岛和空气污染物扩散

IF 10.8 1区 环境科学与生态学 Q1 ENGINEERING, ENVIRONMENTAL 环境科学与技术 Pub Date : 2024-11-21 DOI:10.1021/acs.est.4c02300
Jinyuan Xin, Xinbing Ren, Yongjing Ma, Dandan Zhao, Yonghong Wang, Jianhuai Ye, Zifa Wang, Junji Cao, Jordi Vilà-Guerau de Arellano, Scot T. Martin
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引用次数: 0

摘要

燃煤电厂等显著的人为热源会改变大气边界层结构和污染物扩散,从而影响当地环境和小气候。在此,我们于 2021 年 5 月 21 日至 6 月 21 日在中国山西省运城市利用多个先进的激光雷达对一个燃煤钢铁厂进行了实地测量。与邻近的气象观测点相比,我们发现工厂上空有一个突出的夜间干热岛,温度比周围地区高 3-10 °C,干燥度高 30%-60%。在测量到的热对比约束下进行的大涡度模拟表明,热岛引起的环流可以向上输送工厂排放的污染物,并将其水平扩散到残余层顶部以下,形成蘑菇状云团。云的形状、大小和污染物负荷在很大程度上取决于热力学变量,如空气动力风和人为热通量。此外,这些残留的残留层污染物会在日出后通过熏蒸效应向下对流到地面,造成地面上的峰值现象。据统计,这些峰值在中国主要城市群中很常见。该研究为残留层污染物的来源提供了新的见解,并强调了在中尺度空气质量模型中对燃煤热力排放进行编程表示的必要性。
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Industrial Dry Heat Island and Dispersion of Air Pollutants Induced by Large Coal-Fired Activities
Notable anthropogenic heat sources such as coal-fired plants can alter the atmospheric boundary layer structure and the pollutant dispersion, thereby affecting the local environment and microclimate. Herein, in situ measurements inside a coal-fired steel plant were performed by multiple advanced lidars from 21 May to 21 June of 2021 in Yuncheng, Shanxi Province, China. Comparing with an adjacent meteorological site, we found a prominent nighttime dry heat island overhead of the factory, which was 3–10 °C hotter and 30%–60% drier than the surrounding fields. Large-eddy simulations constrained by the measured thermal contrast suggested that the heat-island-induced circulation could upward transport factory-discharged pollutants and horizontally spread them below the residual layer top, forming a mushroom-shaped cloud. The shape, size, and pollutant loading of the cloud were highly determined by thermodynamic variables such as aerodynamic wind and anthropogenic heat flux. Furthermore, these retained residual-layer pollutants can be convected downward to the ground after sunrise through the fumigation effect, causing the peaking phenomena aboveground. These peaks were statistically evidenced to be common in major urban agglomerations in China. The study provides a new insight regarding the origins of residual-layer pollutants and highlights the needs for programming representations of coal-fired heat emissions in mesoscale air-quality models.
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来源期刊
环境科学与技术
环境科学与技术 环境科学-工程:环境
CiteScore
17.50
自引率
9.60%
发文量
12359
审稿时长
2.8 months
期刊介绍: Environmental Science & Technology (ES&T) is a co-sponsored academic and technical magazine by the Hubei Provincial Environmental Protection Bureau and the Hubei Provincial Academy of Environmental Sciences. Environmental Science & Technology (ES&T) holds the status of Chinese core journals, scientific papers source journals of China, Chinese Science Citation Database source journals, and Chinese Academic Journal Comprehensive Evaluation Database source journals. This publication focuses on the academic field of environmental protection, featuring articles related to environmental protection and technical advancements.
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