[自由水面人工湿地对洱海上游水体微塑料赋存特征的影响]。

Q2 Environmental Science 环境科学 Pub Date : 2024-11-08 DOI:10.13227/j.hjkx.202312273
Hua Wang, Qi-Bin Liang, Liu-Yun Dai, Yan-Xia Wang, Xiao-Lin Li, Lei Hou
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引用次数: 0

摘要

微塑料是一种新兴的污染物,广泛存在于水、沉积物、土壤和大气等环境介质中。探索MPs在不同环境中的发生和迁移特征是准确评价其生态环境效应的必要条件。然而,自由水面人工湿地(FWS)在多大程度上改变了MPs在水中的发生特征,目前还没有明确的研究。因此,选取洱海上游罗石江流域的5个FWS人工湿地作为研究对象。从湿地进出口的MPs丰度、形态、粒径、聚合物类型等方面探讨了FWS人工湿地对水体MPs特性的影响。结果表明:①罗石江流域FWS人工湿地水体中MPs的数量丰度为10 375 ~ 21 000 n·m-3,质量丰度为5.5 ~ 9.8mg·m-3,其平均丰度分别为(14 115±2 790)mg·m-3和(7.6±2.3)mg·m-3。FWS人工湿地水体中高分子聚合物以粒径小(0.2-1 mm, 73.8%±7.5%)、颜色透明(64.0%±12.2%)、纤维状(98.9%±1.7%)为主,主要为玻璃膜(CP, 58.5%±13.9%)、聚对苯二甲酸乙二醇酯(PET, 22.1%±11.4%)和聚酯(PES, 12.8%±16.8%)。该流域FWS人工湿地水体MPs丰度较高,污染负荷指数和生态风险指数均处于较低水平(一级)。②水经过FWS人工湿地后,膜状和碎片状MPs消失,主色(透明、黑色和白色)和聚合物型(PET)的比例分别下降1.4%和4.1%。大尺寸和少数色(红、黄、绿、紫等)MPs的比例增加,1-2 mm、2-5 mm和少数色分别增加了3.0%、2.2%和5.4%,并检测到湿地入口不存在的人造丝和PES聚合物类型。③罗石江流域FWS人工湿地入口和出口MPs的数量和质量丰度差异均不显著(P>0.05), FWS人工湿地对水体中MPs的滞留也不显著。然而,FWS人工湿地削弱了水体中不同MPs特征之间的相关性。结果表明,FWS人工湿地可以改变水体中MPs的粒度、形状、颜色和聚合物类型等存在特征,并表现出MPs的源汇双重作用。
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[Effect of Free Water Surface Constructed Wetland on the Occurrence Characteristics of Microplastics in Water in the Upper Reaches of the Erhai Lake].

Microplastics (MPs), an emerging contaminant, have been widely detected in environmental media including water, sediment, soil, and atmosphere. Exploring the occurrence and transport characteristics of MPs in different environments is essential for accurately evaluating its ecological and environmental effects. However, the extent to which a free water surface (FWS) constructed wetland alters the occurrence characteristics of MPs in water has not been clearly elucidated. Therefore, five FWS constructed wetlands in the Luoshijiang Watershed located in the upper reaches of the Erhai Lake were selected as the research objects. The effects of these FWS constructed wetlands on MPs characteristics in water bodies were explored based on their abundance, shape, particle size, and polymer type in the wetland inlet and outlet. The results showed that: ① The quantity and mass abundance of MPs in the water of the FWS constructed wetland in the Luoshijiang Watershed were in the range of 10 375-21 000 n·m-3 and 5.5-9.8mg·m-3, and the corresponding average abundances were (14 115±2 790) n·m-3 and (7.6±2.3)mg·m-3, respectively. MPs with small particle size (0.2-1 mm, 73.8%±7.5%), transparent color (64.0%±12.2%), and fiber shape (98.9%±1.7%) were dominant in water bodies of the FWS constructed wetland, while cellophane (CP, 58.5%±13.9%), polyethylene terephthalate (PET, 22.1%±11.4%), and polyester (PES, 12.8%±16.8%) were the main polymer types. The MPs abundance in the water of FWS constructed wetland in this watershed was relatively high, whereas the pollution load index and ecological risk index were both in low levels (Level I). ② After water flowing through the FWS constructed wetland, the film- and fragment-shaped MPs disappeared, and the proportions of dominant color (transparent, black, and white) and polymer type (PET) decreased by 1.4% and 4.1%, respectively. By contrast, the proportions of large size and minority-color (red, yellow, green, purple, etc.) MPs increased, with 1-2 mm, 2-5 mm, and minority-color increasing by 3.0%, 2.2%, and 5.4%, respectively, and polymer types of rayon and PES, which did not exist in the wetland inlet, were detected. ③ The quantity and mass abundance of MPs differences between the inlet and outlet of the FWS constructed wetland in the Luoshijiang Watershed were both insignificant (P>0.05), and the retention of MPs in water bodies by the FWS constructed wetland was also insignificant. However, the FWS constructed wetland weakened the correlations among different MPs characteristics in water bodies. The results indicated that the FWS constructed wetland could alter the occurrence characteristics of MPs in water bodies, including particle size, shape, color, and polymer type, and exhibited the dual roles of source and sink of MPs.

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来源期刊
环境科学
环境科学 Environmental Science-Environmental Science (all)
CiteScore
4.40
自引率
0.00%
发文量
15329
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