荒地城市界面(WUI)排放:人造建筑材料燃烧产生的气溶胶和微量气体的实验室测量

Katherine. B. Benedict*, James E. Lee, Nitin Kumar, Prakash S. Badal, Michele Barbato, Manvendra K. Dubey and Allison C. Aiken, 
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摘要

野火的强度正在增加,并且更经常威胁到建筑物和房屋与自然环境共存的荒地城市界面(WUI)。WUI排放还没有像植被排放那样得到充分的研究。因此,有必要量化在燃烧和阴燃条件下用于家庭建筑的建筑材料的排放,以研究其对人类健康、能见度、空气质量和气候的影响。在这里,在一个受控的实验室环境中,我们量化了气溶胶和微量气体的排放,包括甲醛、颗粒物和黑碳。我们关注的是传统的单一来源的木质建筑燃料的燃烧。我们的研究结果表明,与天然燃料类似,气溶胶光学性质与燃烧条件的关系比与燃料类型的关系更大。总的来说,我们观察到气体和颗粒排放的显著变化。一致的趋势包括阴燃条件下的高甲醛(HCHO)和一氧化碳(CO)排放,燃烧条件下的高二氧化碳(CO2)、氮氧化物(NOx)和黑碳排放。这些观察结果突出表明,需要更好地描述建筑环境中材料的排放特征,以评估WUI火灾对大规模气候和人类健康的影响。
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Wildland Urban Interface (WUI) Emissions: Laboratory Measurement of Aerosol and Trace Gas from Combustion of Manufactured Building Materials

Wildfires are increasing in intensity and more often threatening the wildland urban interface (WUI) where buildings and homes coexist with the natural environment. WUI emissions have not been as well-studied as emissions from vegetation. Thus, there is a need to quantify the emissions of building materials used in home construction under flaming and smoldering conditions to study their impacts to human health, visibility, air quality, and climate. Here, in a controlled laboratory setting, we quantify emissions of aerosols and trace gases including formaldehyde, particulate matter, and black carbon. We focus on the combustion of traditional single-source wood-based construction fuels. Our results indicate that, similar to natural fuels, the aerosol optical properties were more related to combustion conditions than the fuel type. Overall, we observed significant variability in the gas and particle emissions. Consistent trends include high formaldehyde (HCHO) and carbon monoxide (CO) emissions for smoldering conditions and higher carbon dioxide (CO2), nitrogen oxides (NOx), and black carbon for flaming conditions. These observations highlight the need to better characterize emissions for materials in the built environment to assess large-scale climate and human health impacts of fires at the WUI.

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