欧洲自由电子激光器的海森堡- rixs仪器。

IF 2.5 3区 物理与天体物理 Journal of Synchrotron Radiation Pub Date : 2025-01-01 DOI:10.1107/S1600577524010890
Justine Schlappa, Giacomo Ghiringhelli, Benjamin E Van Kuiken, Martin Teichmann, Piter S Miedema, Jan Torben Delitz, Natalia Gerasimova, Serguei Molodtsov, Luigi Adriano, Bernard Baranasic, Carsten Broers, Robert Carley, Patrick Gessler, Nahid Ghodrati, David Hickin, Le Phuong Hoang, Manuel Izquierdo, Laurent Mercadier, Giuseppe Mercurio, Sergii Parchenko, Marijan Stupar, Zhong Yin, Leonardo Martinelli, Giacomo Merzoni, Ying Ying Peng, Torben Reuss, Sreeju Sreekantan Nair Lalithambika, Simone Techert, Tim Laarmann, Simo Huotari, Christian Schroeter, Burkhard Langer, Tatjana Giessel, Jana Buchheim, Grzegorz Gwalt, Andrey Sokolov, Frank Siewert, Robby Buechner, Vinicius Vaz da Cruz, Sebastian Eckert, Chun Yu Liu, Christian Sohrt, Christian Weniger, Annette Pietzsch, Stefan Neppl, Friedmar Senf, Andreas Scherz, Alexander Föhlisch
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引用次数: 0

摘要

共振非弹性x射线散射(RIXS)是一种理想的x射线光谱学方法,可以将能量和时间的组合分辨率推向傅里叶变换的极限,因为它不受岩心-孔寿命能量展宽的影响。此外,在泵浦-探针实验中,相同的岩心-孔寿命使得相互作用时间非常短。RIXS非常需要光子,因此它从欧洲XFEL等高重复率脉冲x射线源中获得了很大的优势。Heisenberg RIXS仪器是专为软x射线范围的RIXS实验而设计的,其能量分辨率接近傅里叶极限和海森堡极限。它是基于一个可变线距的球面光栅和一个位置敏感的二维探测器。最初,安装了两个光栅以充分覆盖整个光子能量范围。通过优化样品光斑尺寸和小像素探测器,高分辨率(高透射)光栅在1000 eV以下的任何光子能量下,能量分辨率均优于40 meV (90 meV)。在欧洲XFEL的SCS仪器中,由于高质量地板上的空气垫,光谱仪可以很容易地定位,允许散射角在65-145°范围内连续调整。它可以耦合到两个不同的样品相互作用室,一个用于液体射流,一个用于固体,每个最先进的装备和兼容的共线几何光学激光泵浦。在探测器的能量分辨率和计数率方面,测量的性能与设计预期非常吻合。海森堡RIXS仪器从2022年夏天开始向公众开放。
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The Heisenberg-RIXS instrument at the European XFEL.

Resonant inelastic X-ray scattering (RIXS) is an ideal X-ray spectroscopy method to push the combination of energy and time resolutions to the Fourier transform ultimate limit, because it is unaffected by the core-hole lifetime energy broadening. Also, in pump-probe experiments the interaction time is made very short by the same core-hole lifetime. RIXS is very photon hungry so it takes great advantage from high-repetition-rate pulsed X-ray sources like the European XFEL. The Heisenberg RIXS instrument is designed for RIXS experiments in the soft X-ray range with energy resolution approaching the Fourier and the Heisenberg limits. It is based on a spherical grating with variable line spacing and a position-sensitive 2D detector. Initially, two gratings were installed to adequately cover the whole photon energy range. With optimized spot size on the sample and small pixel detector the energy resolution can be better than 40 meV (90 meV) at any photon energy below 1000 eV with the high-resolution (high-transmission) grating. At the SCS instrument of the European XFEL the spectrometer can be easily positioned thanks to air pads on a high-quality floor, allowing the scattering angle to be continuously adjusted over the 65-145° range. It can be coupled to two different sample interaction chambers, one for liquid jets and one for solids, each state-of-the-art equipped and compatible for optical laser pumping in collinear geometry. The measured performances, in terms of energy resolution and count rate on the detector, closely match design expectations. The Heisenberg RIXS instrument has been open to public users since the summer of 2022.

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来源期刊
Journal of Synchrotron Radiation
Journal of Synchrotron Radiation INSTRUMENTS & INSTRUMENTATIONOPTICS&-OPTICS
CiteScore
5.60
自引率
12.00%
发文量
289
审稿时长
1 months
期刊介绍: Synchrotron radiation research is rapidly expanding with many new sources of radiation being created globally. Synchrotron radiation plays a leading role in pure science and in emerging technologies. The Journal of Synchrotron Radiation provides comprehensive coverage of the entire field of synchrotron radiation and free-electron laser research including instrumentation, theory, computing and scientific applications in areas such as biology, nanoscience and materials science. Rapid publication ensures an up-to-date information resource for scientists and engineers in the field.
期刊最新文献
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