{"title":"污水污泥化学环法制氢分析","authors":"Toshiyuki Shiraki, Satoshi Okumura, Satoshi Uehara, Hiroki Harada, Masaki Takaoka","doi":"10.1007/s10163-024-02140-0","DOIUrl":null,"url":null,"abstract":"<div><p>The objective of this study is to develop a highly efficient technology for producing hydrogen from sewage sludge using chemical-looping technology. In this study, laboratory-scale gasification experiments were conducted on sewage sludge samples. The effects of CaO as a carrier of oxygen or carbon (C) and as a gasification accelerator were evaluated. Lab-scale tests using a tube-type electric furnace showed that gasification of CaO-mixed dry sludge with steam resulted in substantial absorption of CO<sub>2</sub> by CaO at 600 ℃ and 700 ℃ and the concentration of H<sub>2</sub> in the gas reached 70 vol.%. The gasification was significantly accelerated in CaO-mixed steam gasification compared with pyrolysis gasification and steam gasification of dry sludge in the absence of the CaO mixture. The hydrogen gas (H<sub>2</sub>) recovery rate also increased, and tar with a high C weight ratio and high calorific value was recovered. Almost the entire C in the sewage sludge was gasified at 800 ℃. Therefore, this method (pyrolysis with steam and CaO) was shown to be effective as one of the hydrogen production methods from sewage sludge.</p></div>","PeriodicalId":643,"journal":{"name":"Journal of Material Cycles and Waste Management","volume":"27 1","pages":"558 - 571"},"PeriodicalIF":2.7000,"publicationDate":"2024-12-12","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://link.springer.com/content/pdf/10.1007/s10163-024-02140-0.pdf","citationCount":"0","resultStr":"{\"title\":\"Analysis of chemical-looping method for production of hydrogen gas from sewage sludge\",\"authors\":\"Toshiyuki Shiraki, Satoshi Okumura, Satoshi Uehara, Hiroki Harada, Masaki Takaoka\",\"doi\":\"10.1007/s10163-024-02140-0\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<div><p>The objective of this study is to develop a highly efficient technology for producing hydrogen from sewage sludge using chemical-looping technology. In this study, laboratory-scale gasification experiments were conducted on sewage sludge samples. The effects of CaO as a carrier of oxygen or carbon (C) and as a gasification accelerator were evaluated. Lab-scale tests using a tube-type electric furnace showed that gasification of CaO-mixed dry sludge with steam resulted in substantial absorption of CO<sub>2</sub> by CaO at 600 ℃ and 700 ℃ and the concentration of H<sub>2</sub> in the gas reached 70 vol.%. The gasification was significantly accelerated in CaO-mixed steam gasification compared with pyrolysis gasification and steam gasification of dry sludge in the absence of the CaO mixture. The hydrogen gas (H<sub>2</sub>) recovery rate also increased, and tar with a high C weight ratio and high calorific value was recovered. Almost the entire C in the sewage sludge was gasified at 800 ℃. Therefore, this method (pyrolysis with steam and CaO) was shown to be effective as one of the hydrogen production methods from sewage sludge.</p></div>\",\"PeriodicalId\":643,\"journal\":{\"name\":\"Journal of Material Cycles and Waste Management\",\"volume\":\"27 1\",\"pages\":\"558 - 571\"},\"PeriodicalIF\":2.7000,\"publicationDate\":\"2024-12-12\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"https://link.springer.com/content/pdf/10.1007/s10163-024-02140-0.pdf\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Journal of Material Cycles and Waste Management\",\"FirstCategoryId\":\"93\",\"ListUrlMain\":\"https://link.springer.com/article/10.1007/s10163-024-02140-0\",\"RegionNum\":4,\"RegionCategory\":\"环境科学与生态学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q3\",\"JCRName\":\"ENVIRONMENTAL SCIENCES\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Journal of Material Cycles and Waste Management","FirstCategoryId":"93","ListUrlMain":"https://link.springer.com/article/10.1007/s10163-024-02140-0","RegionNum":4,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q3","JCRName":"ENVIRONMENTAL SCIENCES","Score":null,"Total":0}
Analysis of chemical-looping method for production of hydrogen gas from sewage sludge
The objective of this study is to develop a highly efficient technology for producing hydrogen from sewage sludge using chemical-looping technology. In this study, laboratory-scale gasification experiments were conducted on sewage sludge samples. The effects of CaO as a carrier of oxygen or carbon (C) and as a gasification accelerator were evaluated. Lab-scale tests using a tube-type electric furnace showed that gasification of CaO-mixed dry sludge with steam resulted in substantial absorption of CO2 by CaO at 600 ℃ and 700 ℃ and the concentration of H2 in the gas reached 70 vol.%. The gasification was significantly accelerated in CaO-mixed steam gasification compared with pyrolysis gasification and steam gasification of dry sludge in the absence of the CaO mixture. The hydrogen gas (H2) recovery rate also increased, and tar with a high C weight ratio and high calorific value was recovered. Almost the entire C in the sewage sludge was gasified at 800 ℃. Therefore, this method (pyrolysis with steam and CaO) was shown to be effective as one of the hydrogen production methods from sewage sludge.
期刊介绍：
The Journal of Material Cycles and Waste Management has a twofold focus: research in technical, political, and environmental problems of material cycles and waste management; and information that contributes to the development of an interdisciplinary science of material cycles and waste management. Its aim is to develop solutions and prescriptions for material cycles.
The journal publishes original articles, reviews, and invited papers from a wide range of disciplines related to material cycles and waste management.
The journal is published in cooperation with the Japan Society of Material Cycles and Waste Management (JSMCWM) and the Korea Society of Waste Management (KSWM).
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