强场驱动固体的原子科学

IF 44.8 1区 物理与天体物理 Q1 PHYSICS, APPLIED Nature Reviews Physics Pub Date : 2024-12-16 DOI:10.1038/s42254-024-00784-3
Stefano M. Cavaletto, Katarzyna M. Kowalczyk, Francisco O. Navarrete, Javier Rivera-Dean
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摘要

近年来,由于在产生从飞秒到阿秒持续时间的短激光脉冲方面的技术进步,固态系统中电子的超快动力学引起了相当大的关注。高次谐波产生(HHG)和阿秒瞬态吸收 ;和 ;反射光谱(ATAS ;和 ;ATRS)等技术为亚周期动力学提供了有价值的见解,使固体与强激光场的相互作用成为研究的关键领域。然而,对潜在机制的解释仍然存在差异,需要进一步分析。本展望着重于上述技术之间的关系,强调了它们在探测强激光脉冲在固态系统中引起的电荷动力学方面的有效性。我们强调统一的理论框架对于促进我们对固体强场力学的理解的重要性,同时认识到理论描述和实验结果之间的差异。通过引起人们对HHG与atas和ATRS的互补性的关注,并通过说明它们所实现的关键应用,本展望旨在激发更强的合作和共同努力,弥合理论与实验之间的现有差距,推动该领域向前发展。本展望探讨固体中的阿秒物理,重点是高谐波产生和阿秒瞬态吸收和反射光谱。结合物理实现和理论概念是未来发展的挑战。
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The attoscience of strong-field-driven solids
The ultrafast dynamics of electrons in solid-state systems have garnered considerable attention recently, driven by technological advancements in the generation of short laser pulses from femtosecond down to attosecond durations. Techniques such as high-order harmonic generation (HHG) and attosecond transient absorption and reflection spectroscopy (ATAS and ATRS) provide valuable insights into sub-cycle dynamics, rendering the interaction of solids with intense laser fields a pivotal area of research. However, discrepancies in the explanation of the underlying mechanisms remain, requiring further analysis. This Perspective focuses on the relationship between the above techniques, highlighting their efficacy in probing charge dynamics induced by intense laser pulses in solid-state systems. We emphasize the importance of unified theoretical frameworks to advance our understanding of the strong-field attoscience of solids, while recognizing points of disparity between theoretical descriptions and experimental findings. By drawing attention to the complementary nature of HHG and both ATAS and ATRS, and by illustrating the key applications enabled by them, this Perspective aims to motivate stronger collaborations and concerted efforts to bridge the existing gaps between theory and experiment and propel the field forward. This Perspective explores attosecond physics in solids, focussing on high harmonic generation and attosecond transient absorption and reflection spectroscopy. Combining physical realizations and theoretical concepts is a challenge for future progress.
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来源期刊
CiteScore
47.80
自引率
0.50%
发文量
122
期刊介绍: Nature Reviews Physics is an online-only reviews journal, part of the Nature Reviews portfolio of journals. It publishes high-quality technical reference, review, and commentary articles in all areas of fundamental and applied physics. The journal offers a range of content types, including Reviews, Perspectives, Roadmaps, Technical Reviews, Expert Recommendations, Comments, Editorials, Research Highlights, Features, and News & Views, which cover significant advances in the field and topical issues. Nature Reviews Physics is published monthly from January 2019 and does not have external, academic editors. Instead, all editorial decisions are made by a dedicated team of full-time professional editors.
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