在无线传感器网络中集成银纳米结构,增强生化传感。

IF 5.5 3区 材料科学 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY Nanoscale Research Letters Pub Date : 2025-01-13 DOI:10.1186/s11671-024-04159-6
M. Sahaya Sheela, S. Kumarganesh, Binay Kumar Pandey, Mesfin Esayas Lelisho
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引用次数: 0

摘要

事实证明,将贵金属纳米结构(特别是银纳米颗粒)集成到传感器设计中可提高传感器的性能,包括响应时间、稳定性和灵敏度等关键指标。然而,在了解各种合成参数对这些增强作用的独特贡献方面仍存在重大差距。本研究通过考察温度、生长时间和封端剂的选择等因素如何影响纳米结构的形状和尺寸,从而优化传感器在不同条件下的性能,填补了这一空白。利用硝酸银和硼氢化钠制造出银种子颗粒,然后在含有额外银离子的溶液中进行受控生长。对由此产生的纳米结构的大小和形态进行了调节,以实现无线传感器网络中生化传感的最佳性能。结果表明,将这些纳米结构嵌入聚乙烯醇(PVA)基质中可获得更高的稳定性,30 天内可保持 93% 的有效性,而在聚乙二醇(PEG)中仅能保持 70% 的有效性。性能指标显示出明显的改进:响应时间缩短(1.2 毫秒,分析物浓度为零时为 1.5 毫秒),分析物浓度较高时响应速度更快(0.2 毫秒)。这些结果证实,更高的合成温度和精确的形状控制有助于形成更大、更稳定的纳米结构。稳定性和响应性的增强凸显了贵金属纳米结构在可扩展和耐用传感器应用方面的潜力,与当前的方法相比是一大进步。
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Integration of silver nanostructures in wireless sensor networks for enhanced biochemical sensing

Integrating noble metal nanostructures, specifically silver nanoparticles, into sensor designs has proven to enhance sensor performance across key metrics, including response time, stability, and sensitivity. However, a critical gap remains in understanding the unique contributions of various synthesis parameters on these enhancements. This study addresses this gap by examining how factors such as temperature, growth time, and choice of capping agents influence nanostructure shape and size, optimizing sensor performance for diverse conditions. Using silver nitrate and sodium borohydride, silver seed particles were created, followed by controlled growth in a solution containing additional silver ions. The size and morphology of the resulting nanostructures were regulated to achieve optimal properties for biochemical sensing in wireless sensor networks. Results demonstrated that embedding these nanostructures in Polyvinyl Alcohol (PVA) matrices led to superior stability, maintaining 93% effectiveness over 30 days compared to 70% in Polyethylene Glycol (PEG). Performance metrics revealed significant improvements: reduced response times (1.2 ms vs. 1.5 ms at zero analyte concentration) and faster responses at higher analyte levels (0.2 ms). These outcomes confirm that higher synthesis temperatures and precise shape control contribute to larger, more stable nanostructures.The enhanced stability and responsiveness underscore the potential of noble metal nanostructures for scalable and durable sensor applications, offering a significant advancement over current methods.

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来源期刊
Nanoscale Research Letters
Nanoscale Research Letters 工程技术-材料科学:综合
CiteScore
11.30
自引率
0.00%
发文量
110
审稿时长
48 days
期刊介绍: Nanoscale Research Letters (NRL) provides an interdisciplinary forum for communication of scientific and technological advances in the creation and use of objects at the nanometer scale. NRL is the first nanotechnology journal from a major publisher to be published with Open Access.
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