Quanyou Liu, Yongbo Wei, Pengpeng Li, Xiaowei Huang, Qingqiang Meng, Xiaoqi Wu, Dongya Zhu, Huiyuan Xu, Yin Fu, Di Zhu, Wang Zhang, Zhijun Jin
{"title":"含火山沉积盆地中的天然氢：起源、转化和产量。","authors":"Quanyou Liu, Yongbo Wei, Pengpeng Li, Xiaowei Huang, Qingqiang Meng, Xiaoqi Wu, Dongya Zhu, Huiyuan Xu, Yin Fu, Di Zhu, Wang Zhang, Zhijun Jin","doi":"10.1126/sciadv.adr6771","DOIUrl":null,"url":null,"abstract":"<div >The origins of natural hydrogen in natural gas systems of sedimentary basins and the capacity of these systems to store hydrogen remain inadequately understood, posing crucial questions for the large-scale exploration of natural hydrogen. This study reports on the natural gas composition, stable carbon and hydrogen isotopic values, and helium isotopic values of gas samples collected from the Qingshen gas deposit within volcanic rocks of the Songliao Basin. Natural hydrogen primarily originates from water radiolysis, water-rock interactions (WRI), and mantle. The Qingshen gas deposit contains 95.23 × 10<sup>9</sup> cubic meters of abiotic CH<sub>4</sub>, of which 15.24 × 10<sup>9</sup> cubic meters was generated through hydrogen conversion via Fischer-Tropsch synthesis, with the maximum original hydrogen reserves calculated to be approximately 61.9 × 10<sup>9</sup> cubic meters. We estimated that the study area has generated a maximum total of 572 × 10<sup>9</sup> cubic meters of radiolytic hydrogen, 248 × 10<sup>9</sup> cubic meters of WRI hydrogen, and 127 × 10<sup>9</sup> cubic meters of mantle-derived hydrogen.</div>","PeriodicalId":21609,"journal":{"name":"Science Advances","volume":"11 4","pages":""},"PeriodicalIF":12.5000,"publicationDate":"2025-01-24","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.ncbi.nlm.nih.gov/pmc/articles/PMC11759049/pdf/","citationCount":"0","resultStr":"{\"title\":\"Natural hydrogen in the volcanic-bearing sedimentary basin: Origin, conversion, and production rates\",\"authors\":\"Quanyou Liu, Yongbo Wei, Pengpeng Li, Xiaowei Huang, Qingqiang Meng, Xiaoqi Wu, Dongya Zhu, Huiyuan Xu, Yin Fu, Di Zhu, Wang Zhang, Zhijun Jin\",\"doi\":\"10.1126/sciadv.adr6771\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<div >The origins of natural hydrogen in natural gas systems of sedimentary basins and the capacity of these systems to store hydrogen remain inadequately understood, posing crucial questions for the large-scale exploration of natural hydrogen. This study reports on the natural gas composition, stable carbon and hydrogen isotopic values, and helium isotopic values of gas samples collected from the Qingshen gas deposit within volcanic rocks of the Songliao Basin. Natural hydrogen primarily originates from water radiolysis, water-rock interactions (WRI), and mantle. The Qingshen gas deposit contains 95.23 × 10<sup>9</sup> cubic meters of abiotic CH<sub>4</sub>, of which 15.24 × 10<sup>9</sup> cubic meters was generated through hydrogen conversion via Fischer-Tropsch synthesis, with the maximum original hydrogen reserves calculated to be approximately 61.9 × 10<sup>9</sup> cubic meters. We estimated that the study area has generated a maximum total of 572 × 10<sup>9</sup> cubic meters of radiolytic hydrogen, 248 × 10<sup>9</sup> cubic meters of WRI hydrogen, and 127 × 10<sup>9</sup> cubic meters of mantle-derived hydrogen.</div>\",\"PeriodicalId\":21609,\"journal\":{\"name\":\"Science Advances\",\"volume\":\"11 4\",\"pages\":\"\"},\"PeriodicalIF\":12.5000,\"publicationDate\":\"2025-01-24\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"https://www.ncbi.nlm.nih.gov/pmc/articles/PMC11759049/pdf/\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Science Advances\",\"FirstCategoryId\":\"103\",\"ListUrlMain\":\"https://www.science.org/doi/10.1126/sciadv.adr6771\",\"RegionNum\":1,\"RegionCategory\":\"综合性期刊\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q1\",\"JCRName\":\"MULTIDISCIPLINARY SCIENCES\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Science Advances","FirstCategoryId":"103","ListUrlMain":"https://www.science.org/doi/10.1126/sciadv.adr6771","RegionNum":1,"RegionCategory":"综合性期刊","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"MULTIDISCIPLINARY SCIENCES","Score":null,"Total":0}
Natural hydrogen in the volcanic-bearing sedimentary basin: Origin, conversion, and production rates
The origins of natural hydrogen in natural gas systems of sedimentary basins and the capacity of these systems to store hydrogen remain inadequately understood, posing crucial questions for the large-scale exploration of natural hydrogen. This study reports on the natural gas composition, stable carbon and hydrogen isotopic values, and helium isotopic values of gas samples collected from the Qingshen gas deposit within volcanic rocks of the Songliao Basin. Natural hydrogen primarily originates from water radiolysis, water-rock interactions (WRI), and mantle. The Qingshen gas deposit contains 95.23 × 109 cubic meters of abiotic CH4, of which 15.24 × 109 cubic meters was generated through hydrogen conversion via Fischer-Tropsch synthesis, with the maximum original hydrogen reserves calculated to be approximately 61.9 × 109 cubic meters. We estimated that the study area has generated a maximum total of 572 × 109 cubic meters of radiolytic hydrogen, 248 × 109 cubic meters of WRI hydrogen, and 127 × 109 cubic meters of mantle-derived hydrogen.
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Science Advances, an open-access journal by AAAS, publishes impactful research in diverse scientific areas. It aims for fair, fast, and expert peer review, providing freely accessible research to readers. Led by distinguished scientists, the journal supports AAAS's mission by extending Science magazine's capacity to identify and promote significant advances. Evolving digital publishing technologies play a crucial role in advancing AAAS's global mission for science communication and benefitting humankind.
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