随着测量和分析方法的发展,对大气新粒子形成的理解是如何演变的

IF 2.9 3区 环境科学与生态学 Q2 ENGINEERING, CHEMICAL Journal of Aerosol Science Pub Date : 2025-02-01 Epub Date: 2024-11-24 DOI:10.1016/j.jaerosci.2024.106494
Katrianne Lehtipalo , Tuomo Nieminen , Siegfried Schobesberger , Mikael Ehn , Markku Kulmala , Veli-Matti Kerminen
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引用次数: 0

摘要

导致由气态前体蒸气形成新的气溶胶粒子的一系列化学和物理过程通常被称为新粒子形成(NPF)。虽然对大气NPF的首次观测可以追溯到一个多世纪以前,但该现象的许多方面及其对全球气候的重要性在很长一段时间内仍不为人所知。随着更强大的测量技术的发展,可以连续测量颗粒尺寸分布到最近形成的颗粒及其前体蒸汽的大小,NPF研究在过去的几十年里取得了飞跃。在本文中,我们回顾了新的测量方法如何使我们能够观察、分析和分类大气中的新粒子形成事件,以及这如何改变了我们对这一过程及其在大气中的意义的理解。
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How the understanding of atmospheric new particle formation has evolved along with the development of measurement and analysis methods
The chain of chemical and physical processes leading to formation of new aerosol particles from gaseous precursors vapors is often called new particle formation (NPF). Although first observations of atmospheric NPF date back to more than a century ago, many aspects of the phenomenon and its importance on global climate remained unknown for a long time. Along with the development of more robust measurement techniques enabling continuous field measurements of particle size distributions down to the size of recently formed particles and their precursors vapors, NPF research has taken leaps forward in the past decades. In this article we review how the new measurement methods has enabled us to observe, analyze and classify atmospheric new particle formation events and how this has changed our understanding of the process and its significance in the atmosphere.
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来源期刊
Journal of Aerosol Science
Journal of Aerosol Science 环境科学-工程:化工
CiteScore
8.80
自引率
8.90%
发文量
127
审稿时长
35 days
期刊介绍: Founded in 1970, the Journal of Aerosol Science considers itself the prime vehicle for the publication of original work as well as reviews related to fundamental and applied aerosol research, as well as aerosol instrumentation. Its content is directed at scientists working in engineering disciplines, as well as physics, chemistry, and environmental sciences. The editors welcome submissions of papers describing recent experimental, numerical, and theoretical research related to the following topics: 1. Fundamental Aerosol Science. 2. Applied Aerosol Science. 3. Instrumentation & Measurement Methods.
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