德克萨斯州埃尔帕索的风成沉积物:干旱和城市来源增加了沙漠沙沉积率和粉尘浓度

IF 3.7 2区 环境科学与生态学 Q2 ENVIRONMENTAL SCIENCES Atmospheric Environment Pub Date : 2025-03-01 Epub Date: 2025-01-03 DOI:10.1016/j.atmosenv.2025.121029
Thomas E. Gill , Jose A. Rivas Jr. , Elizabeth J. Walsh
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引用次数: 0

摘要

在干旱地区,如美国德克萨斯州的埃尔帕索/墨西哥奇瓦瓦州的华雷斯城,奇瓦瓦沙漠的大都市区,风沙的沉积影响了土壤、生态系统、人类基础设施和空气质量。在埃尔帕索城市天气尺度的大风事件期间,我们使用大理石除尘器(MDCOs)监测干体沉积,这是一种被动采样器,部署在距离地面21米的大学建筑顶部,为期五年(2011-2016年)。附近的德州环境质量委员会(Texas Commission on Environmental Quality)的空气监测器不断测量颗粒物浓度。在5个天气沙尘事件季节(10 - 5月),MDCO沉积物沉积率平均为111 gm−2yr−1(范围85-164 gm−2yr−1),高于几乎所有其他北美站点,但通常低于全球沙尘带位置。这些沉积速率值仅代表天气尺度的风事件,低估了年风沙沉积总量(在非风暴条件下,对流沙尘事件和输入增加)。沉积率是埃尔帕索县农村报告的2倍,表明城市扬尘增加了总干沉积。在所有事件中沉积的沉积物的平均粒径为50 μm(沙),即使是在跳跃高度以上20 m处收集的,这表明在埃尔帕索的事件可以被认为是“吹沙”而不是“吹尘”。PM10浓度在所有收集年份平均为28 μg/m3,但在观测时间内为200 μg/m3,变化非常大,在强干旱年份显著升高。PM2.5/PM10在收集期和扬尘时段的平均比值为0.13-0.14。PM2.5浓度变化不大,显示了灰尘和干旱对埃尔帕索pm颗粒物的影响。天气事件期间的反向轨迹主要来自西南和西部,穿过沙质、可侵蚀的沙漠土壤和遥感识别的沙尘热点。MDCO沉积物主要由奇瓦瓦沙漠土壤矿物(石英、长石和方解石)组成。与全球主要和次要元素的平均风成沉降量相比,埃尔帕索样品的硅含量丰富,但铝、钛、锰以及铁(一种对生态、辐射和人类健康有重要影响的元素)含量不足。德克萨斯州的埃尔帕索似乎是北美尘土最多/沙子最多的城市之一。
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Aeolian sediment in El Paso, Texas: Elevated desert sand deposition rates and dust concentrations, enhanced by drought and urban sources
Deposition of aeolian (windblown) dust and sand in drylands, such as the El Paso, Texas, USA/Ciudad Juarez, Chihuahua, Mexico metropolitan area within the Chihuahuan Desert, impacts soils, ecosystems, human infrastructure, and air quality. We monitored dry bulk deposition using marble dust collectors (MDCOs), a passive sampler, deployed atop a university building 21m above ground level during synoptic-scale wind events in urban El Paso, for five years (2011–2016). A nearby Texas Commission on Environmental Quality air monitor continuously measured particulate matter concentrations. MDCO sediment deposition rates over five synoptic dust event seasons (October–May) averaged 111 gm−2yr−1 (range 85–164 gm−2yr−1), higher than almost all other North American sites but generally lower than Global Dust Belt locations. These deposition rate values, representing only synoptic-scale wind events, underestimate total annual aeolian deposition (augmented by convective dust events and inputs during non-windstorm conditions). Deposition rates were ∼2x those reported for rural El Paso County, suggesting urban fugitive dust enhances total dry deposition. Mean grain size of deposited sediment in all events was >50 μm (sand), even though collected ∼20 m above the height of saltation, indicating that events in El Paso can be considered “blowing sand” rather than “blowing dust.” PM10 concentrations averaged 28 μg/m3 over all collection years but 200 μg/m3 during hours dust was observed, were extremely variable, and were significantly higher during years of strong drought. PM2.5/PM10 ratios averaged 0.13–0.14 during collection periods and dust hours. PM2.5 concentrations were less strongly variable, showing the roles of dust and drought in PMcoarse in El Paso. Back trajectories during synoptic events were predominantly from the southwest and west, crossing sandy, erodible desert soils and remote-sensing-identified dust hotspots. MDCO sediments were comprised primarily of predominant Chihuahuan Desert soil minerals (quartz, feldspars, and calcite). Compared to global average aeolian deposition of major and minor elements, El Paso samples were enriched in silicon but depleted in aluminum, titanium, and manganese, as well as iron, an element with important ecological, radiative, and human health impacts. El Paso, Texas appears to be one of the dustiest/sandiest cities in North America.
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来源期刊
Atmospheric Environment
Atmospheric Environment 环境科学-环境科学
CiteScore
9.40
自引率
8.00%
发文量
458
审稿时长
53 days
期刊介绍: Atmospheric Environment has an open access mirror journal Atmospheric Environment: X, sharing the same aims and scope, editorial team, submission system and rigorous peer review. Atmospheric Environment is the international journal for scientists in different disciplines related to atmospheric composition and its impacts. The journal publishes scientific articles with atmospheric relevance of emissions and depositions of gaseous and particulate compounds, chemical processes and physical effects in the atmosphere, as well as impacts of the changing atmospheric composition on human health, air quality, climate change, and ecosystems.
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