IF 10.8 1区 环境科学与生态学 Q1 ENGINEERING, ENVIRONMENTAL 环境科学与技术 Pub Date : 2025-03-04 DOI:10.1021/acs.est.4c07289
Qinren Shi, Philippe Ciais, Hugo Anne Denier van der Gon, Emma Julie Schoenmakers, Richard Engelen, Xinyu Dou, Piyu Ke, Biqing Zhu, Zhu Liu, Frédéric Chevallier, Marc Guevara
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摘要

二氧化碳排放网格图越来越多地应用于排放变化分析和大气研究。在本研究中,我们比较了欧洲 2019-2021 年人为二氧化碳排放量的两个高分辨率网格估算值:近实时全球网格化二氧化碳日排放量数据集(GRACED,2024 年 5 月最新更新版本)和哥白尼大气监测服务区域清单(CAMS-REG,2019-2020 年版本 6,2021 年版本 7)。两套数据的二氧化碳总排放量相当,排放量相差 2.4%,2021 年总排放量在 0.1°的空间判定系数(R)为 0.66。然而,部门排放量和空间模式却存在显著差异。在网格层面,电力、陆运和航运的跨域相对百分比差异(RPD)中位数的绝对值均达到 200%。由于 CAMS-REG 具有更高的空间分辨率,并使用了本地化数据集,因此建议用于欧洲精细尺度历史排放分析。GRACED 的最大延迟时间为 3 个月,更适合需要近实时数据的应用。对于大气建模人员来说,描述两种最先进排放地图之间差异的工作也很有价值,因为他们在对陆地和海洋二氧化碳汇进行反演计算时,需要考虑化石燃料排放的先验不确定性。
本文章由计算机程序翻译,如有差异,请以英文原文为准。

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Comparison of High-Resolution Gridded Emission Maps of Anthropogenic Carbon Dioxide in Europe: GRACED & CAMS-REG
Gridded maps of CO2 emissions are increasingly being applied in emission change analyses and atmospheric studies. In this study, we compared two high-resolution gridded estimates of anthropogenic CO2 emissions in Europe for 2019–2021: the near-real-time Global gridded daily CO2 emission data set (GRACED, latest updated version May 2024) and the Copernicus Atmosphere Monitoring Service regional inventory (CAMS-REG, v6 for 2019–2020, and v7 for 2021). Total CO2 emissions of the two data sets are comparable, with a 2.4% emission difference, and the total emissions’ spatial determination coefficient (R) at 0.1° is 0.66 in 2021. However, the sectoral emissions and spatial patterns show significant differences. At the grid level, the absolute value of the median of relative percent difference (RPD) of power, ground transportation, and shipping across the domain all reach 200%. CAMS-REG is recommended for fine-scale historical emission analysis in Europe due to its higher spatial resolution and the use of localized data sets. GRACED, with a maximum latency of 3 months, is more appropriate for applications requiring near-real-time data. This work characterizing the difference between two state-of-the-art emission maps is also valuable for atmospheric modelers who need to account for the uncertainty of a priori fossil fuel emissions when performing inverse calculations of land and ocean CO2 sinks.
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来源期刊
环境科学与技术
环境科学与技术 环境科学-工程:环境
CiteScore
17.50
自引率
9.60%
发文量
12359
审稿时长
2.8 months
期刊介绍: Environmental Science & Technology (ES&T) is a co-sponsored academic and technical magazine by the Hubei Provincial Environmental Protection Bureau and the Hubei Provincial Academy of Environmental Sciences. Environmental Science & Technology (ES&T) holds the status of Chinese core journals, scientific papers source journals of China, Chinese Science Citation Database source journals, and Chinese Academic Journal Comprehensive Evaluation Database source journals. This publication focuses on the academic field of environmental protection, featuring articles related to environmental protection and technical advancements.
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