胺功能化纤维素作为CO2直接捕集材料的研究进展

IF 8.2 2区 材料科学 Q1 MATERIALS SCIENCE, MULTIDISCIPLINARY ACS Applied Materials & Interfaces Pub Date : 2025-03-19 Epub Date: 2025-03-04 DOI:10.1021/acsami.4c20801
Hicham Akaya, Soukaina Lamnini, Houssine Sehaqui, Johan Jacquemin
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引用次数: 0

摘要

在此,胺功能化纤维素作为一种低成本和可持续的二氧化碳捕获吸附剂的潜在用途进行了综述。本文献分析特别强调了各种先进的制备方法,用于合成具有增强吸附CO2分子亲和力的功能化纤维素载体。纤维素与不同类型的胺功能化的机制是明确详细的,考虑胺浸渍和接枝选择性化学吸收二氧化碳气体有或没有水分的存在,在不同的温度和压力。最后一节批判性地讨论了扩大胺功能化纤维素吸附剂的主要限制,特别是与胺氧化,稳定性和降解有关的问题。
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Amine-Functionalized Cellulose as Promising Materials for Direct CO2 Capture: A Review.

Herein, the potential use of amine-functionalized cellulose as a low-cost and sustainable sorbent for CO2 capture is reviewed. This literature analysis specifically highlights various advanced preparation methods used to synthesize functionalized cellulose supports with an enhanced affinity for the sorption of CO2 molecules. The mechanism of cellulose functionalization with different types of amines is explicitly detailed, considering amine impregnation and grafting to selectively chemisorb CO2 gas with or without the presence of moisture and at different temperatures and pressures. The final section critically discusses the main limitations to scaling up amine-functionalized cellulose sorbents, particularly issues related to amine oxidation, stability, and degradation.

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来源期刊
ACS Applied Materials & Interfaces
ACS Applied Materials & Interfaces 工程技术-材料科学:综合
CiteScore
16.00
自引率
6.30%
发文量
4978
审稿时长
1.8 months
期刊介绍: ACS Applied Materials & Interfaces is a leading interdisciplinary journal that brings together chemists, engineers, physicists, and biologists to explore the development and utilization of newly-discovered materials and interfacial processes for specific applications. Our journal has experienced remarkable growth since its establishment in 2009, both in terms of the number of articles published and the impact of the research showcased. We are proud to foster a truly global community, with the majority of published articles originating from outside the United States, reflecting the rapid growth of applied research worldwide.
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