{"title":"peV能量尺度下的四波混频。","authors":"C Simon, D M Silevitch, T F Rosenbaum","doi":"10.1103/PhysRevLett.134.086705","DOIUrl":null,"url":null,"abstract":"<p><p>We measure the nonlinear magnetic susceptibility χ^{(3)} of the disordered quantum Ising magnet LiHo_{0.045}Y_{0.955}F_{4} and demonstrate four-wave mixing due to coherent (anti-)Stokes Raman scattering at ∼100 Hz (peV) energy scales. The temperature dependence of χ^{(3)} approximately follows a (1/T) form, with a high-T cutoff that can be linked to dissipation in the coherent spin clusters. χ^{(3)} also decreases monotonically with a transverse field, approaching a constant offset above a few kOe, suggesting the presence of both coherent and spontaneous Raman scattering.</p>","PeriodicalId":20069,"journal":{"name":"Physical review letters","volume":"134 8","pages":"086705"},"PeriodicalIF":9.0000,"publicationDate":"2025-02-28","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Four-Wave Mixing at peV Energy Scales.\",\"authors\":\"C Simon, D M Silevitch, T F Rosenbaum\",\"doi\":\"10.1103/PhysRevLett.134.086705\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<p><p>We measure the nonlinear magnetic susceptibility χ^{(3)} of the disordered quantum Ising magnet LiHo_{0.045}Y_{0.955}F_{4} and demonstrate four-wave mixing due to coherent (anti-)Stokes Raman scattering at ∼100 Hz (peV) energy scales. The temperature dependence of χ^{(3)} approximately follows a (1/T) form, with a high-T cutoff that can be linked to dissipation in the coherent spin clusters. χ^{(3)} also decreases monotonically with a transverse field, approaching a constant offset above a few kOe, suggesting the presence of both coherent and spontaneous Raman scattering.</p>\",\"PeriodicalId\":20069,\"journal\":{\"name\":\"Physical review letters\",\"volume\":\"134 8\",\"pages\":\"086705\"},\"PeriodicalIF\":9.0000,\"publicationDate\":\"2025-02-28\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Physical review letters\",\"FirstCategoryId\":\"101\",\"ListUrlMain\":\"https://doi.org/10.1103/PhysRevLett.134.086705\",\"RegionNum\":1,\"RegionCategory\":\"物理与天体物理\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q1\",\"JCRName\":\"PHYSICS, MULTIDISCIPLINARY\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Physical review letters","FirstCategoryId":"101","ListUrlMain":"https://doi.org/10.1103/PhysRevLett.134.086705","RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"PHYSICS, MULTIDISCIPLINARY","Score":null,"Total":0}
We measure the nonlinear magnetic susceptibility χ^{(3)} of the disordered quantum Ising magnet LiHo_{0.045}Y_{0.955}F_{4} and demonstrate four-wave mixing due to coherent (anti-)Stokes Raman scattering at ∼100 Hz (peV) energy scales. The temperature dependence of χ^{(3)} approximately follows a (1/T) form, with a high-T cutoff that can be linked to dissipation in the coherent spin clusters. χ^{(3)} also decreases monotonically with a transverse field, approaching a constant offset above a few kOe, suggesting the presence of both coherent and spontaneous Raman scattering.
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