自旋轨道耦合对菱形石墨烯超导性的影响

IF 38.5 1区 材料科学 Q1 CHEMISTRY, PHYSICAL Nature Materials Pub Date : 2025-03-19 DOI:10.1038/s41563-025-02156-3
Jixiang Yang, Xiaoyan Shi, Shenyong Ye, Chiho Yoon, Zhengguang Lu, Vivek Kakani, Tonghang Han, Junseok Seo, Lihan Shi, Kenji Watanabe, Takashi Taniguchi, Fan Zhang, Long Ju
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引用次数: 0

摘要

自旋轨道耦合(SOC)在许多拓扑和相关电子材料中起着重要的作用。在基于石墨烯的体系中,由过渡金属二硫化物近距离诱导的SOC已被证明可以驱动拓扑状态并增强超导性。然而,在菱面体多层石墨烯中,一个强大的电子相关和拓扑平台,超导性和SOC的作用仍然很大程度上未被探索。在这里,我们报告了过渡金属二硫化物-近方面体三层石墨烯的输运测量。我们观察到一个临界温度为234 mK的空穴掺杂超导态SC4。在电子掺杂侧,我们注意到一个同位旋对称破缺的四分之三金属相,并观察到附近的弱超导态SC3得到了显著增强。令人惊讶的是,裸菱形三层石墨烯中的原始超导态SC1在过渡金属二硫化物的存在下被强烈抑制,这与SOC对所有其他石墨烯超导性的影响相反。我们的观察结果为探索菱形石墨烯器件中的超导性和非阿贝尔准粒子奠定了基础。
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Impact of spin–orbit coupling on superconductivity in rhombohedral graphene
Spin–orbit coupling (SOC) has played an important role in many topological and correlated electron materials. In graphene-based systems, SOC induced by a transition metal dichalcogenide at close proximity has been shown to drive topological states and strengthen superconductivity. However, in rhombohedral multilayer graphene, a robust platform for electron correlation and topology, superconductivity and the role of SOC remain largely unexplored. Here we report transport measurements of transition metal dichalcogenide-proximitized rhombohedral trilayer graphene. We observed a hole-doped superconducting state SC4 with a critical temperature of 234 mK. On the electron-doped side, we noted an isospin-symmetry-breaking three-quarter-metal phase and observed that the nearby weak superconducting state SC3 is substantially enhanced. Surprisingly, the original superconducting state SC1 in bare rhombohedral trilayer graphene is strongly suppressed in the presence of transition metal dichalcogenide—opposite to the effect of SOC on all other graphene superconductivities. Our observations form the basis of exploring superconductivity and non-Abelian quasiparticles in rhombohedral graphene devices. The authors present transport measurements of rhombohedral trilayer graphene proximitized by transition metal dichalcogenides. They find that the presence of transition metal dichalcogenides enables the emergence of new superconducting and metallic phases and affects the superconducting states present in bare rhombohedral trilayer graphene.
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来源期刊
Nature Materials
Nature Materials 工程技术-材料科学:综合
CiteScore
62.20
自引率
0.70%
发文量
221
审稿时长
3.2 months
期刊介绍: Nature Materials is a monthly multi-disciplinary journal aimed at bringing together cutting-edge research across the entire spectrum of materials science and engineering. It covers all applied and fundamental aspects of the synthesis/processing, structure/composition, properties, and performance of materials. The journal recognizes that materials research has an increasing impact on classical disciplines such as physics, chemistry, and biology. Additionally, Nature Materials provides a forum for the development of a common identity among materials scientists and encourages interdisciplinary collaboration. It takes an integrated and balanced approach to all areas of materials research, fostering the exchange of ideas between scientists involved in different disciplines. Nature Materials is an invaluable resource for scientists in academia and industry who are active in discovering and developing materials and materials-related concepts. It offers engaging and informative papers of exceptional significance and quality, with the aim of influencing the development of society in the future.
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