综述了电化学CO2还原反应中单原子催化剂合理设计的研究进展

IF 5.8 3区 材料科学 Q2 CHEMISTRY, MULTIDISCIPLINARY Carbon Letters Pub Date : 2025-03-01 DOI:10.1007/s42823-025-00874-x
Jinuk Choi, Seoyeon Yoo, Gnanaprakasam Janani, Subramani Surendran, Sathyanarayanan Shanmugapriya, Heechae Choi, Gibum Kwon, Kyoungsuk Jin, Uk Sim
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引用次数: 0

摘要

二氧化碳的电化学还原是一种至关重要的能量转换方案,涉及两个重要过程:将二氧化碳(一种温室气体)转化为增值产品和减少化石燃料的使用以生产燃料或化学产品。此外,由于二氧化碳还原反应是一个双质子/电子反应,因此二氧化碳还原反应产生的CO量很大,并且在化学,冶金和制药工业中也有潜在的应用。在各类电催化材料中,单原子催化剂因其高原子利用率而备受关注。本文综述了二氧化碳电还原制一氧化碳用单原子电催化剂的最新研究进展。
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Recent research trends in the rational designing of single atom catalysts for electrochemical CO2 reduction reaction to CO—a mini review

Electrochemical reduction of carbon dioxide is a crucial energy conversion protocol involving two significant processes: converting CO2, a greenhouse gas, into value-added products and reducing fossil fuel usage to produce fuels or chemical products. Moreover, the production of CO from the carbon dioxide reduction reaction is highly substantial since it is a two-proton/electron reaction, and it also finds potential applications in chemical, metallurgical, and pharmaceutical industries. Among the various classes of electrocatalytic materials, single-atom catalysts have attracted great attention because of their high atom utilization. Here, we survey the recent research trends involved in the preparation of single atom-based electrocatalysts for the generation of carbon monoxide from the electroreduction of carbon dioxide.

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来源期刊
Carbon Letters
Carbon Letters CHEMISTRY, MULTIDISCIPLINARY-MATERIALS SCIENCE, MULTIDISCIPLINARY
CiteScore
7.30
自引率
20.00%
发文量
118
期刊介绍: Carbon Letters aims to be a comprehensive journal with complete coverage of carbon materials and carbon-rich molecules. These materials range from, but are not limited to, diamond and graphite through chars, semicokes, mesophase substances, carbon fibers, carbon nanotubes, graphenes, carbon blacks, activated carbons, pyrolytic carbons, glass-like carbons, etc. Papers on the secondary production of new carbon and composite materials from the above mentioned various carbons are within the scope of the journal. Papers on organic substances, including coals, will be considered only if the research has close relation to the resulting carbon materials. Carbon Letters also seeks to keep abreast of new developments in their specialist fields and to unite in finding alternative energy solutions to current issues such as the greenhouse effect and the depletion of the ozone layer. The renewable energy basics, energy storage and conversion, solar energy, wind energy, water energy, nuclear energy, biomass energy, hydrogen production technology, and other clean energy technologies are also within the scope of the journal. Carbon Letters invites original reports of fundamental research in all branches of the theory and practice of carbon science and technology.
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