双活性NiO-Ce1-xNixO2纳米复合材料催化PET转化成H2。

IF 4.3 2区 化学 Q2 CHEMISTRY, MULTIDISCIPLINARY Chemical Communications Pub Date : 2025-04-09 DOI:10.1039/d5cc01304f
Jin Wang , Fangqi Liu , Chun Shan , Jiarui Zhu , Zengjian Guo , Xuesong Zhang , Lujia Han
{"title":"双活性NiO-Ce1-xNixO2纳米复合材料催化PET转化成H2。","authors":"Jin Wang ,&nbsp;Fangqi Liu ,&nbsp;Chun Shan ,&nbsp;Jiarui Zhu ,&nbsp;Zengjian Guo ,&nbsp;Xuesong Zhang ,&nbsp;Lujia Han","doi":"10.1039/d5cc01304f","DOIUrl":null,"url":null,"abstract":"<div><div>ANiO<sub>3</sub> (A = La, Ce, and Sr) perovskites were innovatively synthesized for catalytic steam reforming of polyethylene terephthalate (PET) following non-catalytic decomposition. CeNiO<sub>3</sub>, featuring a dual-active NiO–Ce<sub>1−<em>x</em></sub>Ni<sub><em>x</em></sub>O<sub>2</sub> nanocomposite with moderate oxygen vacancies, achieved a high H<sub>2</sub> yield of 54.58 mmol g<sub>PET</sub><sup>−1</sup> and a carbon conversion efficiency of 83.13%.</div></div>","PeriodicalId":67,"journal":{"name":"Chemical Communications","volume":"61 37","pages":"Pages 6795-6798"},"PeriodicalIF":4.3000,"publicationDate":"2025-04-09","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"A dual-active NiO–Ce1−xNixO2 nanocomposite for catalytically upcycling PET into H2†\",\"authors\":\"Jin Wang ,&nbsp;Fangqi Liu ,&nbsp;Chun Shan ,&nbsp;Jiarui Zhu ,&nbsp;Zengjian Guo ,&nbsp;Xuesong Zhang ,&nbsp;Lujia Han\",\"doi\":\"10.1039/d5cc01304f\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<div><div>ANiO<sub>3</sub> (A = La, Ce, and Sr) perovskites were innovatively synthesized for catalytic steam reforming of polyethylene terephthalate (PET) following non-catalytic decomposition. CeNiO<sub>3</sub>, featuring a dual-active NiO–Ce<sub>1−<em>x</em></sub>Ni<sub><em>x</em></sub>O<sub>2</sub> nanocomposite with moderate oxygen vacancies, achieved a high H<sub>2</sub> yield of 54.58 mmol g<sub>PET</sub><sup>−1</sup> and a carbon conversion efficiency of 83.13%.</div></div>\",\"PeriodicalId\":67,\"journal\":{\"name\":\"Chemical Communications\",\"volume\":\"61 37\",\"pages\":\"Pages 6795-6798\"},\"PeriodicalIF\":4.3000,\"publicationDate\":\"2025-04-09\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Chemical Communications\",\"FirstCategoryId\":\"92\",\"ListUrlMain\":\"https://www.sciencedirect.com/org/science/article/pii/S1359734525007074\",\"RegionNum\":2,\"RegionCategory\":\"化学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q2\",\"JCRName\":\"CHEMISTRY, MULTIDISCIPLINARY\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Chemical Communications","FirstCategoryId":"92","ListUrlMain":"https://www.sciencedirect.com/org/science/article/pii/S1359734525007074","RegionNum":2,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q2","JCRName":"CHEMISTRY, MULTIDISCIPLINARY","Score":null,"Total":0}
引用次数: 0

摘要

采用非催化分解法合成了ANiO3 (A = La, Ce, Sr)钙钛矿,用于催化蒸汽重整聚对苯二甲酸乙二醇酯(PET)。具有中等氧空位的双活性NiO-Ce1-xNixO2纳米复合材料CeNiO3的H2产率为54.58 mmol gPET-1,碳转化效率为83.13%。
本文章由计算机程序翻译,如有差异,请以英文原文为准。

摘要图片

摘要图片

查看原文
分享 分享
微信好友 朋友圈 QQ好友 复制链接
本刊更多论文
A dual-active NiO–Ce1−xNixO2 nanocomposite for catalytically upcycling PET into H2†
ANiO3 (A = La, Ce, and Sr) perovskites were innovatively synthesized for catalytic steam reforming of polyethylene terephthalate (PET) following non-catalytic decomposition. CeNiO3, featuring a dual-active NiO–Ce1−xNixO2 nanocomposite with moderate oxygen vacancies, achieved a high H2 yield of 54.58 mmol gPET−1 and a carbon conversion efficiency of 83.13%.
求助全文
通过发布文献求助,成功后即可免费获取论文全文。 去求助
来源期刊
Chemical Communications
Chemical Communications 化学-化学综合
CiteScore
8.60
自引率
4.10%
发文量
2705
审稿时长
1.4 months
期刊介绍: ChemComm (Chemical Communications) is renowned as the fastest publisher of articles providing information on new avenues of research, drawn from all the world''s major areas of chemical research.
期刊最新文献
Contributors to the Pioneering Investigators collection 2026: part 1 Degradative functionalization of perfluoro-3-methoxypropanoic acid. Ansa-methylene-substituted cobalt bis(dicarbollide) ion available via an easy click: a carbene-like mechanism. First examples of C3-, C4-, and C6-functionalized carbazoles enabling efficient near-ultraviolet electroluminescence. A hydrogen-bonding-enhanced room-temperature phosphorescent host-guest composite for highly selective detection of L-Glu.
×
引用
GB/T 7714-2015
复制
MLA
复制
APA
复制
导出至
BibTeX EndNote RefMan NoteFirst NoteExpress
×
×
提示
您的信息不完整,为了账户安全,请先补充。
现在去补充
×
提示
您因"违规操作"
具体请查看互助需知
我知道了
×
提示
现在去查看 取消
×
提示
确定
0
微信
客服QQ
Book学术公众号 扫码关注我们
反馈
×
意见反馈
请填写您的意见或建议
请填写您的手机或邮箱
已复制链接
已复制链接
快去分享给好友吧!
我知道了
×
扫码分享
扫码分享
Book学术官方微信
Book学术官方微信
Book学术文献互助
Book学术文献互助群
群 号:604180095
Book学术
文献互助 智能选刊 最新文献 互助须知 联系我们:info@booksci.cn
Book学术提供免费学术资源搜索服务,方便国内外学者检索中英文文献。致力于提供最便捷和优质的服务体验。
Copyright © 2023 Book学术 All rights reserved.
ghs 京公网安备 11010802042870号 京ICP备2023020795号-1