单向电荷密度波材料中沿纳米褶皱受限的一维电子气体

IF 16 1区 材料科学 Q1 CHEMISTRY, MULTIDISCIPLINARY ACS Nano Pub Date : 2025-04-19 DOI:10.1021/acsnano.4c18943
Eunseo Kim, Sanghun Lee, Hyungryul Yang, Makoto Hashimoto, Donghui Lu, Jongho Park, Changyoung Kim, Dirk Wulferding, Sunghun Kim, Doohee Cho
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引用次数: 0

摘要

二维(2D)材料固有地表现出不稳定性。在结构上,这可能导致沿第三维的调制,例如褶皱。电子上,二维不稳定性可以表现为电荷密度波(cdw)。虽然褶皱可以改变易形成cdw的各向异性电子结构,但对它们对破对称基态的影响知之甚少。本文利用扫描隧道显微镜和光谱学技术,研究了DyTe3皱褶表面的CDW态。我们发现细长的,平行的纳米级皱纹稳定的带状缺陷。有趣的是,CDW顺序在纳米皱纹中持续存在,并逐渐发生相移,但在缺陷附近被局部抑制,在缺陷附近发生相绕组。此外,这些缺陷沿纳米皱褶方向诱导量子约束效应,表明存在一维金属态,具有类似空穴的色散,而角分辨光电发射光谱在皱褶方向上发现了一个间隙。我们将这种差异归因于费米表面的应变引起的变化,这导致纳米皱纹位置的间隙关闭。综上所述,我们的结果强调了结构特征和费米表面拓扑之间复杂的相互作用,允许通过局部晶体变形故意操纵强相关系统中的量子态。
本文章由计算机程序翻译,如有差异,请以英文原文为准。

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One-Dimensional Electron Gas Confined along Nanowrinkles in a Unidirectional Charge Density Wave Material
Two-dimensional (2D) materials inherently exhibit instabilities. Structurally, this may lead to modulations along the third dimension, e.g., wrinkles. Electronically, 2D instabilities can manifest themselves as charge density waves (CDWs). Although wrinkles can alter anisotropic electronic structures susceptible to forming CDWs, less is known about their impact on broken-symmetry ground states. Here, using scanning tunneling microscopy and spectroscopy, we investigate the CDW states on the wrinkled surface of DyTe3. We identify elongated, parallel nanoscale wrinkles stabilized by ribbon-shaped defects. Interestingly, the CDW order persists across the nanowrinkles with a gradual phase shift but is locally suppressed near the defects, where phase windings occur. In addition, these defects induce quantum confinement effects along the nanowrinkles, indicating the presence of one-dimensional metallic states with hole-like dispersion, while angle-resolved photoemission spectroscopy identifies a gap along the wrinkle direction. We ascribe this discrepancy to strain-induced changes in the Fermi surface, which lead to the closure of the gap at the sites of the nanowrinkles. Taken together, our results underscore the complex interplay between structural features and Fermi surface topology, allowing for the deliberate manipulation of quantum states in strongly correlated systems via local crystal deformations.
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来源期刊
ACS Nano
ACS Nano 工程技术-材料科学:综合
CiteScore
26.00
自引率
4.10%
发文量
1627
审稿时长
1.7 months
期刊介绍: ACS Nano, published monthly, serves as an international forum for comprehensive articles on nanoscience and nanotechnology research at the intersections of chemistry, biology, materials science, physics, and engineering. The journal fosters communication among scientists in these communities, facilitating collaboration, new research opportunities, and advancements through discoveries. ACS Nano covers synthesis, assembly, characterization, theory, and simulation of nanostructures, nanobiotechnology, nanofabrication, methods and tools for nanoscience and nanotechnology, and self- and directed-assembly. Alongside original research articles, it offers thorough reviews, perspectives on cutting-edge research, and discussions envisioning the future of nanoscience and nanotechnology.
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