激光与二氧化钛相互作用的研究进展-图像化、结晶和烧蚀过程

IF 9.1 2区 化学 Q1 CHEMISTRY, INORGANIC & NUCLEAR Progress in Solid State Chemistry Pub Date : 2021-06-01 DOI:10.1016/j.progsolidstchem.2020.100297
Katarzyna Siuzdak, Łukasz Haryński, Jakub Wawrzyniak, Katarzyna Grochowska
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引用次数: 5

摘要

二氧化钛被认为是一种非常有前途的半导体材料,广泛应用于许多日常使用的产品、设备和工艺中。一般来说,这些应用可分为能源或环境类别,其中高转换率和能量和功率密度特别令人感兴趣。因此,人们正在努力探索新的生产路线,改善材料的光吸收和电荷集中等性能,以及开发表面积以提高特定工艺的效率。通常,可以区分大块掺杂和表面修饰,在掺杂前体存在的情况下,应用一些溶胶-凝胶、化学气相沉积和水热工艺。然而,废物处理的发展和许多扩大规模的优化路线必须执行,以考虑建议的路径值得广泛的商业用途。与湿化学方法相比,激光技术通过特定波长、影响和脉冲重复率的光提供独特的材料处理。因此,这些变化可以影响整体结构或仅影响其表面。这种方法在不使用任何化学产品的情况下提供了广泛的可能改性,因此避免了任何副产物的形成。此外,了解激光治疗的快速扩展,达到更高的技术准备水平,我们相信这种方法从首先在小烧瓶中使用少量基板进行的合成和/或修饰中脱颖而出。在这篇综述中,我们想强调一些研究的结果,这些研究表明激光束和二氧化钛的相互作用可能会改变表面区域或深入内部结构。这里的工作表明,这种强大的技术可以提供二氧化钛纳米管的轻微表面熔化,它们的相从无定形固体转变为锐钛矿,或者,当影响超过一定的阈值时,从二氧化钛靶中烧蚀材料。
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Review on robust laser light interaction with titania – Patterning, crystallisation and ablation processes

Titanium dioxide is regarded as a very promising semiconducting material that is widely applied in many everyday-use products, devices, and processes. In general, those applications can be divided into energy or environmental categories, where a high conversion rate, and energy and power density are of particular interest. Therefore, many efforts are being put towards the elaboration of novel production routes, and improving the material's properties such as light absorption, and charge concentration, as well as development of the surface area to improve the efficiency of particular process. Typically, bulk doping and surface modifications can be distinguished, applying some sol-gel, chemical vapour deposition, and hydrothermal processes in the presence of dopant precursors. However, development of waste disposal and many up-scaling optimisation routes have to be performed to consider the proposed path worthy of wide scale, commercial use. In contrast to the wet-chemistry methods, laser technology offers unique material treatment by light of a particular wavelength, fluence, and pulse repetition rate. In consequence, the changes can affect the bulk structure or only its surface. Such an approach provides a wide range of possible modifications without the use of any chemical products, and therefore avoids the formation of any by-products. Moreover, knowing the facile scaling up of laser treatment towards a higher technology readiness level, we believe such an approach stands out from synthesis and/or modification carried out first in small flasks and using small amounts of substrates. In this review, we would like to emphasize the results of selected studies presenting possible laser beam and titania interactions ensuring changes in the surface zone or deeply in the internal structure. The works evoked here indicate that this powerful technique can, among other things, provide slight surface melting of titania nanotubes, their phase transition from an amorphous solid to anatase or, when the fluence exceeds a certain threshold, the ablation of material out of the titania target.

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来源期刊
Progress in Solid State Chemistry
Progress in Solid State Chemistry 化学-无机化学与核化学
CiteScore
14.10
自引率
3.30%
发文量
12
期刊介绍: Progress in Solid State Chemistry offers critical reviews and specialized articles written by leading experts in the field, providing a comprehensive view of solid-state chemistry. It addresses the challenge of dispersed literature by offering up-to-date assessments of research progress and recent developments. Emphasis is placed on the relationship between physical properties and structural chemistry, particularly imperfections like vacancies and dislocations. The reviews published in Progress in Solid State Chemistry emphasize critical evaluation of the field, along with indications of current problems and future directions. Papers are not intended to be bibliographic in nature but rather to inform a broad range of readers in an inherently multidisciplinary field by providing expert treatises oriented both towards specialists in different areas of the solid state and towards nonspecialists. The authorship is international, and the subject matter will be of interest to chemists, materials scientists, physicists, metallurgists, crystallographers, ceramists, and engineers interested in the solid state.
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