太湖污染控制与流域氮足迹的减少

IF 11.3 1区 化学 Q1 CHEMISTRY, PHYSICAL ACS Catalysis Pub Date : 2022-01-15 DOI:10.1016/j.jclepro.2021.130132
Mingqian Wu , Xiuming Zhang , Stefan Reis , Shengxiu Ge , Baojing Gu
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引用次数: 5

摘要

为了养活日益富裕的人口,全球粮食生产系统的氮投入目前是地球安全边界的两倍,导致对当地和全球环境产生不利影响。氮足迹是了解人类活动对环境影响的重要指标,但很少在流域尺度上应用。利用人与自然耦合系统(CHANS)模型发现,太湖流域的总氮输入从1995年的141.1 Gg N yr−1增加到2010年的244.3 Gg N yr−1,然后在2015年再次减少到201.2 Gg N yr−1。研究结果与太湖总氮浓度的变化一致。2010年之前,人均氮足迹稳定在30 kg N - 1左右,2010年和2015年人均氮足迹分别大幅下降至25和20 kg N - 1左右。构成氮足迹的主要氮排放源逐渐从农业生产转变为废水和化石燃料燃烧产生的氮氧化物排放。减少氮足迹有利于制定有效的氮污染控制策略,未来的政策制定应优先考虑更好的废水处理技术。
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Pollution controls in Lake Tai with the reduction of the watershed nitrogen footprint

To feed an increasingly affluent population, the nitrogen input into global food production systems is currently two times the safe planetary boundary leading to adverse impacts on the local and global environments. The nitrogen footprint is an important index to understand the impact of human activities on the environment, however, it is rarely applied at a watershed scale. By using the Coupled Human And Natural System (CHANS) model, it was found that the total nitrogen input to the Lake Tai watershed has increased from 141.1 Gg N yr−1 in 1995 to 244.3 Gg N yr−1 in 2010, and then decreased again to 201.2 Gg N yr−1 in 2015. The study findings are consistent with the change in the total nitrogen concentration observed in Lake Tai. While the per capita nitrogen footprint remained stable at around 30 kg N yr−1 before 2010, a substantial decrease to approximately 25 and 20 kg N yr−1 in 2010 and 2015, respectively, has occurred. Dominant sources of nitrogen emissions contributing to the nitrogen footprint gradually have changed from agricultural production to wastewater and nitrogen oxides emissions from fossil fuel combustion. A reduction of the nitrogen footprint is beneficial for effective nitrogen pollution control strategies and better wastewater treatment techniques should be prioritized for future policymaking.

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来源期刊
ACS Catalysis
ACS Catalysis CHEMISTRY, PHYSICAL-
CiteScore
20.80
自引率
6.20%
发文量
1253
审稿时长
1.5 months
期刊介绍: ACS Catalysis is an esteemed journal that publishes original research in the fields of heterogeneous catalysis, molecular catalysis, and biocatalysis. It offers broad coverage across diverse areas such as life sciences, organometallics and synthesis, photochemistry and electrochemistry, drug discovery and synthesis, materials science, environmental protection, polymer discovery and synthesis, and energy and fuels. The scope of the journal is to showcase innovative work in various aspects of catalysis. This includes new reactions and novel synthetic approaches utilizing known catalysts, the discovery or modification of new catalysts, elucidation of catalytic mechanisms through cutting-edge investigations, practical enhancements of existing processes, as well as conceptual advances in the field. Contributions to ACS Catalysis can encompass both experimental and theoretical research focused on catalytic molecules, macromolecules, and materials that exhibit catalytic turnover.
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