利用氮氧化物和氮化物在可见光下减少二氧化碳

IF 9.1 2区 化学 Q1 CHEMISTRY, INORGANIC & NUCLEAR Progress in Solid State Chemistry Pub Date : 2018-09-01 DOI:10.1016/j.progsolidstchem.2017.11.003
Kazuhiko Maeda
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引用次数: 20

摘要

在可见光下使用多相光催化剂减少二氧化碳已被研究作为解决全球变暖和化石燃料枯竭问题的潜在手段。最近,由金属配合物和微粒半导体构成的混合光催化剂受到了特别的关注,因为金属配合物具有出色的电化学(和/或光催化)能力来还原CO2,而半导体在氧化反应中的效率很高,其中氧化反应的最终目标是水氧化形成分子O2。本文综述了近年来用于可见光CO2还原的金属-配合物/半导体杂化材料的研究进展,重点介绍了氮化氧材料和氮化氮材料的半导体成分。
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CO2 reduction using oxynitrides and nitrides under visible light

Reduction of CO2 using a heterogeneous photocatalyst under visible light has been studied as a potential means to address the problems of global warming and the depletion of fossil fuels. Recently, hybrid photocatalysts constructed with a metal complex and a particulate semiconductor are of particular interest because of the excellent electrochemical (and/or photocatalytic) ability of the metal complexes for CO2 reduction and the high efficiency of the semiconductors for oxidation reactions, where the ultimate target of oxidation reaction is water oxidation to form molecular O2. This review article highlights our recent progress in the development of metal-complex/semiconductor hybrid materials for visible-light CO2 reduction with a focus on oxynitride and nitride materials as the semiconductor component.

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来源期刊
Progress in Solid State Chemistry
Progress in Solid State Chemistry 化学-无机化学与核化学
CiteScore
14.10
自引率
3.30%
发文量
12
期刊介绍: Progress in Solid State Chemistry offers critical reviews and specialized articles written by leading experts in the field, providing a comprehensive view of solid-state chemistry. It addresses the challenge of dispersed literature by offering up-to-date assessments of research progress and recent developments. Emphasis is placed on the relationship between physical properties and structural chemistry, particularly imperfections like vacancies and dislocations. The reviews published in Progress in Solid State Chemistry emphasize critical evaluation of the field, along with indications of current problems and future directions. Papers are not intended to be bibliographic in nature but rather to inform a broad range of readers in an inherently multidisciplinary field by providing expert treatises oriented both towards specialists in different areas of the solid state and towards nonspecialists. The authorship is international, and the subject matter will be of interest to chemists, materials scientists, physicists, metallurgists, crystallographers, ceramists, and engineers interested in the solid state.
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