不同激励脉冲对激光诱导瞬态居群光栅的影响分析

IF 16.4 1区 化学 Q1 CHEMISTRY, MULTIDISCIPLINARY Accounts of Chemical Research Pub Date : 2023-01-01 DOI:10.1117/1.JNP.17.016013
Shuanggen Zhang, Shengdong Li, Yangbo Bai, Kai Huang
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引用次数: 0

摘要

摘要在原子对不同初始相干光场响应的激励下,比较研究了连续脉冲串诱导的瞬态居群光栅。通过数值求解密度矩阵方程,得到了TPG的延时和泵浦脉冲持续时间的依赖关系。结果表明,通过选择合适的脉冲参数,可以产生和消除TPG,并得到Bloch球模型和定量验证。为了获得矩形脉冲所需的大光栅幅值,可以将允许的脉冲持续时间延长到比高斯脉冲宽一个数量级。第三次脉冲延时为脉冲宽度的一半的奇数倍,可以将填充光栅擦除到接近零,第四次脉冲延时为脉冲宽度的整数倍,也可以进一步擦除光栅,使原子组装恢复到初始状态。本文提出的不同类型脉冲激发的原子行为可能对光-物质相干相互作用过程中TPG的操纵有重要意义。
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Analysis of laser-induced transient population gratings by different types of exciting pulse
Abstract. Motivated by atomic response to different initial coherent optical fields, we comparatively studied transient population grating (TPG) induced by successive pulse train. Time delay and pump pulse duration dependence of TPG is achieved by numerically solving the density matrix equations. Results reveal that the creation and erasure of TPG is possible by choosing the appropriate pulse parameters, which is illustrated by Bloch sphere model and quantitative validation. To obtain desired large grating amplitude for rectangular pulse, the allowed pulse duration can be extended to one order wider than that of Gaussian pulse. Population grating can be erased to near zero by a third pulse with time delay by an odd multiple of half the pulse width, and it also can be erased further to recover atom assembly back to the initial state by a fourth pulse with time delay equal to an integer multiple of pulse width. Atomic behaviors excited by different types of pulse presented here may be significant to manipulate TPG during coherent light-matter interaction.
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来源期刊
Accounts of Chemical Research
Accounts of Chemical Research 化学-化学综合
CiteScore
31.40
自引率
1.10%
发文量
312
审稿时长
2 months
期刊介绍: Accounts of Chemical Research presents short, concise and critical articles offering easy-to-read overviews of basic research and applications in all areas of chemistry and biochemistry. These short reviews focus on research from the author’s own laboratory and are designed to teach the reader about a research project. In addition, Accounts of Chemical Research publishes commentaries that give an informed opinion on a current research problem. Special Issues online are devoted to a single topic of unusual activity and significance. Accounts of Chemical Research replaces the traditional article abstract with an article "Conspectus." These entries synopsize the research affording the reader a closer look at the content and significance of an article. Through this provision of a more detailed description of the article contents, the Conspectus enhances the article's discoverability by search engines and the exposure for the research.
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