北极两个峡湾(霍恩松湾和康斯峡湾)冰川海湾对海洋沉积物的重金属排放增加

IF 4.6 Q2 MATERIALS SCIENCE, BIOMATERIALS ACS Applied Bio Materials Pub Date : 2023-07-11 DOI:10.1016/j.jmarsys.2023.103915
Paulina Rudnicka-Kępa , Magdalena Bełdowska , Agata Zaborska
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引用次数: 2

摘要

气候变化正在以影响污染物运输和积累的方式改变北极生态系统。研究了两个斯匹次卑尔根峡湾Kongsfjorden和Hornsund重金属分布的时空变异性。2018年至2019年,收集了Kongsfjorden五个站和Hornsund六个站的沉积物岩芯,用于测量重金属浓度(Hg、Pb、Cd、Cu和Zn)。沉积物层采用210Pb法测年,以揭示污染历史。利用同位素铅组分研究了铅的来源。重金属对峡湾沉积物的负荷是根据大量沉积物积累率计算的。重金属负荷在空间上变化,汞达到0.3 mg m−2 yr−1,铅达到57.6 mg m−1 yr−2,镉达到0.5 mg m−3 yr−3,铜达到101 mg m−4 yr−4,锌达到117 mg m−5 yr−6。从冰川到冰川湾的重金属排放量比峡湾中部和外部的排放量高得多。这可能表明冰川可能是峡湾污染物的重要次生来源。
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Enhanced heavy metal discharges to marine deposits in glacial bays of two Arctic fjords (Hornsund and Kongsfjorden)

Climate change is transforming Arctic ecosystems in ways that are influencing the transport and accumulation of contaminants. The spatial and temporal variability of heavy metal distribution was studied in two Spitsbergen fjords – Kongsfjorden and Hornsund. Sediment cores from five stations in Kongsfjorden and six in Hornsund were collected in 2018–2019 and used for measurement of heavy metal concentrations (Hg, Pb, Cd, Cu, and Zn). Sediment layers were dated by the 210Pb method to reveal the history of contamination. Isotopic lead composition was used to study sources of Pb. Loads of heavy metals to fjord deposits were calculated based on mass sediment accumulation rates. The heavy metal loads varied spatially and reached ranged 0.3 mg m−2 yr−1 for Hg, 57.6 mg m−2 yr−1 for Pb, 0.5 mg m−2 yr−1 for Cd, 101 mg m−2 yr−1 for Cu, and 117 mg m−2 yr−1 for Zn. Heavy metal discharge from the glaciers to the glacial bays were much higher compared to discharge in central and outer fjord parts. This may suggest that glaciers can be important secondary sources of pollutants to fjords.

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来源期刊
ACS Applied Bio Materials
ACS Applied Bio Materials Chemistry-Chemistry (all)
CiteScore
9.40
自引率
2.10%
发文量
464
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