飞秒激光脉冲后金属中的局部非平衡电子输运:一个多温度双曲模型

IF 2.7 3区 工程技术 Q2 ENGINEERING, MECHANICAL Nanoscale and Microscale Thermophysical Engineering Pub Date : 2021-09-30 DOI:10.1080/15567265.2021.1985022
S. Sobolev
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引用次数: 9

摘要

电子器件小型化的趋势增加了人们对纳米尺度热输运的兴趣,特别是在激光激发固体中,电子-电子热化和电子-声子耦合起着关键作用。利用考虑初始非热化电子与不同声子分支之间耦合的多温度双曲模型,我们得到了由于不同激励之间耦合的多长度和时间尺度性质而产生的电子温度的热传导方程层次。该层次预测,超短激光脉冲诱导了一个多前沿温度波传播到材料体中,其中包括各种热传递机制,从最初非热化电子的弹道运动在最短的时间尺度上传播,而不与晶格相互作用作为温度不连续,到由于各种激励之间的耦合而在中间时间尺度上产生的连续波状温度锋。最后是在最长时间尺度上的经典傅立叶输运。该模型有望用于模拟异质结构和超材料中的热波传播现象。
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Local Nonequilibrium Electron Transport in Metals after Femtosecond Laser Pulses: A Multi-Temperature Hyperbolic Model
ABSTRACT The trend toward miniaturization of electronic devices has increased the interest in nano scale heat transport, particularly, in laser-excited solids where electron–electron thermalization and electron-phonon coupling play a key role. Using a multi-temperature hyperbolic model, which takes into account the coupling between initially non-thermalized electrons and different phonon branches, we obtain a hierarchy of heat conduction equations for the electron temperature, which arises due to multi-length and time scales nature of coupling between different excitations. The hierarchy predicts that the ultrashort laser pulse induces a multi-front temperature wave propagating into the bulk of the material, which includes various heat transport regimes, ranging from the ballistic motion of the initially non-thermalized electrons propagating on the shortest time scale without interaction with the lattice as a temperature discontinuity, to the continuous wave-like temperature fronts arising on the intermediate time scale due to coupling between various excitations, and eventually to the classical Fourier transport on the longest time scale. The model is expected to be useful for modeling heat wave propagation phenomena in heterostructures and metamaterials.
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来源期刊
Nanoscale and Microscale Thermophysical Engineering
Nanoscale and Microscale Thermophysical Engineering 工程技术-材料科学:表征与测试
CiteScore
5.90
自引率
2.40%
发文量
12
审稿时长
3.3 months
期刊介绍: Nanoscale and Microscale Thermophysical Engineering is a journal covering the basic science and engineering of nanoscale and microscale energy and mass transport, conversion, and storage processes. In addition, the journal addresses the uses of these principles for device and system applications in the fields of energy, environment, information, medicine, and transportation. The journal publishes both original research articles and reviews of historical accounts, latest progresses, and future directions in this rapidly advancing field. Papers deal with such topics as: transport and interactions of electrons, phonons, photons, and spins in solids, interfacial energy transport and phase change processes, microscale and nanoscale fluid and mass transport and chemical reaction, molecular-level energy transport, storage, conversion, reaction, and phase transition, near field thermal radiation and plasmonic effects, ultrafast and high spatial resolution measurements, multi length and time scale modeling and computations, processing of nanostructured materials, including composites, micro and nanoscale manufacturing, energy conversion and storage devices and systems, thermal management devices and systems, microfluidic and nanofluidic devices and systems, molecular analysis devices and systems.
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