Hewen Niu, Shichang Kang, Xiaofei Shi, Guotao Zhang, Shijin Wang, Tao Pu
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引用次数: 17
摘要
溶解性有机碳(DOC)是空气-水碳循环系统中重要的有机污染物,对全球气候具有潜在影响。本研究于2014年6 - 9月在玉龙山地区5个采样站同步采集了204份雨水样本。对夏季降水中DOC的来源和湿沉降进行了全面研究。5个监测站DOC的平均浓度为0.74 ~ 1.31 mg / L / 1。雨水DOC质量吸收效率(MAE)在365?Nm为0.43±0.32 m2 / g / 1。反轨迹分析表明,西南平流气团占降水事件的46%,对应的雨水DOC平均浓度为1.25±0.56?mg C L?除了局地或区域贡献外,南亚和东南亚地区还输送了大量的大气污染物到玉龙山地区,对区域大气环境产生了很大的影响。首次估算了玉龙山地区DOC的年湿沉降量为1.99?2年1月1日。这是因为DOC在冰川上的沉积对积雪和冰川融化的地表反照率有很大的影响。该研究弥补了玉龙山地区与青藏高原东南部雨水DOC研究的空白,对更好地理解青藏高原东南部雨水DOC沉积与冰川收缩的关系具有重要意义。
Dissolved organic carbon in summer precipitation and its wet deposition flux in the Mt. Yulong region, southeastern Tibetan Plateau
Dissolved organic carbon (DOC) is an important organic pollutant in the air-water carbon cycle system, potentially influencing the global climate. In this study, 204 rainwater samples from five sampling stations in the Mt. Yulong region were synchronously collected from June to September in 2014. We comprehensively investigated the sources and wet deposition of DOC in summer precipitation. The average concentrations of DOC at five stations ranged from 0.74 to 1.31?mg?L?1. The mass absorption efficiency (MAE) of rainwater DOC evaluated at 365?nm was 0.43?±?0.32?m2?g?1. Backward trajectory analyses indicated that the southwest advection air parcel accounting for 46% of precipitation events, while the corresponding average concentration of rainwater DOC was 1.25?±?0.56?mg C L?1. In addition to the local or regional contribution, large amount of atmospheric pollutants were transported from South Asia and Southeast Asia to the Mt. Yulong region, both of which had exerted great influence on the regional atmospheric environment. For the first time, the annual wet deposition of DOC in the Mt. Yulong region was estimated and determined to be 1.99?g C m?2?year?1. This is significant because the deposition of DOC on glaciers has great influence on surface albedo of snow and glacier melt. This study can bridge the gap of rainwater DOC research between the Mt. Yulong region and the southeast of Tibetan Plateau (TP), which has significant implications for better understanding the relationship of DOC deposition and glacial shrink in the TP.
期刊介绍:
The Journal of Atmospheric Chemistry is devoted to the study of the chemistry of the Earth''s atmosphere, the emphasis being laid on the region below about 100 km. The strongly interdisciplinary nature of atmospheric chemistry means that it embraces a great variety of sciences, but the journal concentrates on the following topics:
Observational, interpretative and modelling studies of the composition of air and precipitation and the physiochemical processes in the Earth''s atmosphere, excluding air pollution problems of local importance only.
The role of the atmosphere in biogeochemical cycles; the chemical interaction of the oceans, land surface and biosphere with the atmosphere.
Laboratory studies of the mechanics in homogeneous and heterogeneous transformation processes in the atmosphere.
Descriptions of major advances in instrumentation developed for the measurement of atmospheric composition and chemical properties.