中国中部城市秋冬季空气污染特征、健康风险和典型污染过程

IF 2.9 4区 环境科学与生态学 Q3 ENVIRONMENTAL SCIENCES Air Quality Atmosphere and Health Pub Date : 2023-05-10 DOI:10.1007/s11869-023-01371-8
Qianheng Wang, Sen Yao, Jie Tao, Yifei Xu, Huijiao Yan, Hanyu Zhang, Shushen Yang, Fengjuan Fan
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引用次数: 0

摘要

结合大气环境观测资料,利用特征雷达图、潜在污染源贡献因子分析和浓度加权轨迹分析,阐述了郑州市大气污染的特征、类型和潜在污染源区域。我们还计算了过量空气污染物导致死亡的超额风险(ER),并探索了一个典型的污染过程。结果显示,秋季(2020年10月和11月)PM2.5平均浓度(55.5微克/立方米)低于冬季(2020年12月和2021年1月)(83.5微克/m3),1月是受扬尘污染影响最严重的月份。二次污染主要集中在12月和1月,扬尘污染主要集中于10月和1月份。沙尘污染主要受西北长途运输影响,其余污染(除综合污染外)主要受东部城市(济宁、徐州)短途运输影响。ER值主要归因于PM10、PM2.5和NO2超标。二次污染和扬尘污染是造成ER的主要原因。在典型的污染过程中,在沙尘期(第一阶段),气团主要受西北部长途运输的影响,表现出较高的风速和较低的相对湿度。此外,PM2.5/PM10值低于0.4。在PM2.5重污染期(第三阶段),气团主要受东北局地输送的影响,表现出较低的风速和较高的相对湿度。这一时期表现出明显的二次污染和更严重的机动车排放。
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Air pollution characteristics, health risks, and typical pollution processes in autumn and winter in a central city of China

By combining atmospheric environment observational data, we expounded the characteristics, types, and potential source regions of air pollution in Zhengzhou using the characteristic radar chart, potential source contribution factor analysis, and concentration weighted trajectory analysis. We also calculated the excess risk (ER) of death caused by excessive air pollutants and explored a typical pollution process. The results showed that the average PM2.5 concentration in autumn (October and November 2020) (55.5 μg/m3) was lower than that in winter (December 2020 and January 2021) (83.5 μg/m3), and January was the month most seriously affected by dust pollution. Secondary pollution was mainly concentrated in December and January, while dust pollution was mainly concentrated in October and January. Dust pollution was mainly affected by long-distance transport in the northwest, and the remaining pollution (except comprehensive pollution) was mainly affected by short-distance transport in the eastern cities (Jining and Xuzhou). The ER values were mainly attributed to excessive PM10, PM2.5, and NO2. Secondary pollution and dust pollution were the main contributors to ER. During the typical pollution process, in the dust period (stage I), air masses were mainly affected by long-distance transport in the northwest, which displayed higher wind speed and lower relative humidity. Moreover, the PM2.5/PM10 value was below 0.4. During the heavy PM2.5 pollution period (stage III), air masses were mainly affected by local transport in the northeast, which displayed lower wind speed and higher relative humidity. This period showed clear secondary pollution and more severe motor vehicle emissions.

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来源期刊
Air Quality Atmosphere and Health
Air Quality Atmosphere and Health ENVIRONMENTAL SCIENCES-
CiteScore
8.80
自引率
2.00%
发文量
146
审稿时长
>12 weeks
期刊介绍: Air Quality, Atmosphere, and Health is a multidisciplinary journal which, by its very name, illustrates the broad range of work it publishes and which focuses on atmospheric consequences of human activities and their implications for human and ecological health. It offers research papers, critical literature reviews and commentaries, as well as special issues devoted to topical subjects or themes. International in scope, the journal presents papers that inform and stimulate a global readership, as the topic addressed are global in their import. Consequently, we do not encourage submission of papers involving local data that relate to local problems. Unless they demonstrate wide applicability, these are better submitted to national or regional journals. Air Quality, Atmosphere & Health addresses such topics as acid precipitation; airborne particulate matter; air quality monitoring and management; exposure assessment; risk assessment; indoor air quality; atmospheric chemistry; atmospheric modeling and prediction; air pollution climatology; climate change and air quality; air pollution measurement; atmospheric impact assessment; forest-fire emissions; atmospheric science; greenhouse gases; health and ecological effects; clean air technology; regional and global change and satellite measurements. This journal benefits a diverse audience of researchers, public health officials and policy makers addressing problems that call for solutions based in evidence from atmospheric and exposure assessment scientists, epidemiologists, and risk assessors. Publication in the journal affords the opportunity to reach beyond defined disciplinary niches to this broader readership.
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