同轴电弧等离子沉积法制备聚合物电解质膜燃料电池用Pt/C催化剂

Y. Agawa, M. Kunimatsu, T. Ito, Yasutaka Kuwahara, H. Yamashita
{"title":"同轴电弧等离子沉积法制备聚合物电解质膜燃料电池用Pt/C催化剂","authors":"Y. Agawa, M. Kunimatsu, T. Ito, Yasutaka Kuwahara, H. Yamashita","doi":"10.1149/2.0091510EEL","DOIUrl":null,"url":null,"abstract":"A coaxial arc plasma deposition (CAPD) source was developed to generate metallic nanoparticles (NPs) with sizes from sub-nanometer to several nanometers. Pt NPs were deposited on a carbon support by CAPD for use as a polymer electrolyte membrane fuel cell (PEMFC) electrode catalyst. The principle of catalyst formation and the mechanism for control of the particle size by CAPD were investigated. Transmission electron microscopy observations were performed for Pt/C catalysts with various Pt contents. Single PEMFCs were fabricated using 1, 5, and 10 wt% Pt/C catalysts, of which the best cell performance was obtained with the 10 wt% Pt/C catalyst.","PeriodicalId":11470,"journal":{"name":"ECS Electrochemistry Letters","volume":null,"pages":null},"PeriodicalIF":0.0000,"publicationDate":"2015-01-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://sci-hub-pdf.com/10.1149/2.0091510EEL","citationCount":"8","resultStr":"{\"title\":\"Preparation of Pt/C Catalyst by Coaxial Arc Plasma Deposition for Polymer Electrolyte Membrane Fuel Cells\",\"authors\":\"Y. Agawa, M. Kunimatsu, T. Ito, Yasutaka Kuwahara, H. Yamashita\",\"doi\":\"10.1149/2.0091510EEL\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"A coaxial arc plasma deposition (CAPD) source was developed to generate metallic nanoparticles (NPs) with sizes from sub-nanometer to several nanometers. Pt NPs were deposited on a carbon support by CAPD for use as a polymer electrolyte membrane fuel cell (PEMFC) electrode catalyst. The principle of catalyst formation and the mechanism for control of the particle size by CAPD were investigated. Transmission electron microscopy observations were performed for Pt/C catalysts with various Pt contents. Single PEMFCs were fabricated using 1, 5, and 10 wt% Pt/C catalysts, of which the best cell performance was obtained with the 10 wt% Pt/C catalyst.\",\"PeriodicalId\":11470,\"journal\":{\"name\":\"ECS Electrochemistry Letters\",\"volume\":null,\"pages\":null},\"PeriodicalIF\":0.0000,\"publicationDate\":\"2015-01-01\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"https://sci-hub-pdf.com/10.1149/2.0091510EEL\",\"citationCount\":\"8\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"ECS Electrochemistry Letters\",\"FirstCategoryId\":\"1085\",\"ListUrlMain\":\"https://doi.org/10.1149/2.0091510EEL\",\"RegionNum\":0,\"RegionCategory\":null,\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"\",\"JCRName\":\"\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"ECS Electrochemistry Letters","FirstCategoryId":"1085","ListUrlMain":"https://doi.org/10.1149/2.0091510EEL","RegionNum":0,"RegionCategory":null,"ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"","JCRName":"","Score":null,"Total":0}
引用次数: 8

摘要

研究了一种同轴电弧等离子体沉积(CAPD)源,用于制备亚纳米到几纳米尺寸的金属纳米颗粒。采用CAPD技术在碳载体上沉积Pt纳米粒子,作为聚合物电解质膜燃料电池(PEMFC)电极催化剂。研究了催化剂的形成原理和CAPD控制颗粒大小的机理。对不同Pt含量的Pt/C催化剂进行了透射电镜观察。分别用1、5、10 wt% Pt/C催化剂制备了单体pemfc,其中10 wt% Pt/C催化剂的电池性能最好。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
查看原文
分享 分享
微信好友 朋友圈 QQ好友 复制链接
本刊更多论文
Preparation of Pt/C Catalyst by Coaxial Arc Plasma Deposition for Polymer Electrolyte Membrane Fuel Cells
A coaxial arc plasma deposition (CAPD) source was developed to generate metallic nanoparticles (NPs) with sizes from sub-nanometer to several nanometers. Pt NPs were deposited on a carbon support by CAPD for use as a polymer electrolyte membrane fuel cell (PEMFC) electrode catalyst. The principle of catalyst formation and the mechanism for control of the particle size by CAPD were investigated. Transmission electron microscopy observations were performed for Pt/C catalysts with various Pt contents. Single PEMFCs were fabricated using 1, 5, and 10 wt% Pt/C catalysts, of which the best cell performance was obtained with the 10 wt% Pt/C catalyst.
求助全文
通过发布文献求助,成功后即可免费获取论文全文。 去求助
来源期刊
ECS Electrochemistry Letters
ECS Electrochemistry Letters ELECTROCHEMISTRY-MATERIALS SCIENCE, MULTIDISCIPLINARY
自引率
0.00%
发文量
0
期刊最新文献
Preparation of Mesoporous Si@PAN Electrodes for Li-Ion Batteries via the In-Situ Polymerization of PAN Effect of Clamping Pressure and Temperature on the Performance of a CuCl(aq)/HCl(aq) Electrolyzer Carbon-Free AZO/Ru Cathode for Li-Air Batteries Electrochemical Characterization of Iodide Ions Adsorption Kinetics at Bi(111) Electrode from Three-Component Ionic Liquids Mixtures Redox Behavior of Dopamine in the Presence of Ferritin
×
引用
GB/T 7714-2015
复制
MLA
复制
APA
复制
导出至
BibTeX EndNote RefMan NoteFirst NoteExpress
×
×
提示
您的信息不完整,为了账户安全,请先补充。
现在去补充
×
提示
您因"违规操作"
具体请查看互助需知
我知道了
×
提示
现在去查看 取消
×
提示
确定
0
微信
客服QQ
Book学术公众号 扫码关注我们
反馈
×
意见反馈
请填写您的意见或建议
请填写您的手机或邮箱
已复制链接
已复制链接
快去分享给好友吧!
我知道了
×
扫码分享
扫码分享
Book学术官方微信
Book学术文献互助
Book学术文献互助群
群 号:481959085
Book学术
文献互助 智能选刊 最新文献 互助须知 联系我们:info@booksci.cn
Book学术提供免费学术资源搜索服务,方便国内外学者检索中英文文献。致力于提供最便捷和优质的服务体验。
Copyright © 2023 Book学术 All rights reserved.
ghs 京公网安备 11010802042870号 京ICP备2023020795号-1