{"title":"水热合成Mo/Zr-MOF光催化剂促进可见光下Cr6+的去除","authors":"Wenyu Ren, Yi Wang, Jin Wang, Ruixue Sun","doi":"10.1680/jgrma.22.00074","DOIUrl":null,"url":null,"abstract":"The development of highly efficient photocatalysts for the degradation of organic dyes and heavy metal ions is necessary to control pollution in the environment and further human health. We report nMo/Zr-MOFs (n=1, 2, 3, and 4, nMZMs) synthesized by a simple hydrothermal method for efficient photocatalytic Cr6+ reduction for the first time. Among all the prepared samples, 2MZMs shows the highest photocatalytic performance with a degradation rate of 94.36% for methylene blue and 91.20% for Cr6+ under visible light irradiation for 120 min and 100 min respectively. The ESR experiments reveal that •O2 − and •OH play a major role. This finding proves great potential for the design and application of MOFs nanomaterials and might bring considerable application prospects for photocatalysis of organic pollutants and heavy metal ions in polluted water.","PeriodicalId":12929,"journal":{"name":"Green Materials","volume":"1 1","pages":""},"PeriodicalIF":1.8000,"publicationDate":"2023-01-19","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Hydrothermally synthesized Mo/Zr-MOF photocatalyst for promoting the removal of Cr6+ under visible light\",\"authors\":\"Wenyu Ren, Yi Wang, Jin Wang, Ruixue Sun\",\"doi\":\"10.1680/jgrma.22.00074\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"The development of highly efficient photocatalysts for the degradation of organic dyes and heavy metal ions is necessary to control pollution in the environment and further human health. We report nMo/Zr-MOFs (n=1, 2, 3, and 4, nMZMs) synthesized by a simple hydrothermal method for efficient photocatalytic Cr6+ reduction for the first time. Among all the prepared samples, 2MZMs shows the highest photocatalytic performance with a degradation rate of 94.36% for methylene blue and 91.20% for Cr6+ under visible light irradiation for 120 min and 100 min respectively. The ESR experiments reveal that •O2 − and •OH play a major role. This finding proves great potential for the design and application of MOFs nanomaterials and might bring considerable application prospects for photocatalysis of organic pollutants and heavy metal ions in polluted water.\",\"PeriodicalId\":12929,\"journal\":{\"name\":\"Green Materials\",\"volume\":\"1 1\",\"pages\":\"\"},\"PeriodicalIF\":1.8000,\"publicationDate\":\"2023-01-19\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Green Materials\",\"FirstCategoryId\":\"88\",\"ListUrlMain\":\"https://doi.org/10.1680/jgrma.22.00074\",\"RegionNum\":4,\"RegionCategory\":\"材料科学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q4\",\"JCRName\":\"GREEN & SUSTAINABLE SCIENCE & TECHNOLOGY\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Green Materials","FirstCategoryId":"88","ListUrlMain":"https://doi.org/10.1680/jgrma.22.00074","RegionNum":4,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q4","JCRName":"GREEN & SUSTAINABLE SCIENCE & TECHNOLOGY","Score":null,"Total":0}
Hydrothermally synthesized Mo/Zr-MOF photocatalyst for promoting the removal of Cr6+ under visible light
The development of highly efficient photocatalysts for the degradation of organic dyes and heavy metal ions is necessary to control pollution in the environment and further human health. We report nMo/Zr-MOFs (n=1, 2, 3, and 4, nMZMs) synthesized by a simple hydrothermal method for efficient photocatalytic Cr6+ reduction for the first time. Among all the prepared samples, 2MZMs shows the highest photocatalytic performance with a degradation rate of 94.36% for methylene blue and 91.20% for Cr6+ under visible light irradiation for 120 min and 100 min respectively. The ESR experiments reveal that •O2 − and •OH play a major role. This finding proves great potential for the design and application of MOFs nanomaterials and might bring considerable application prospects for photocatalysis of organic pollutants and heavy metal ions in polluted water.
期刊介绍：
The focus of Green Materials relates to polymers and materials, with an emphasis on reducing the use of hazardous substances in the design, manufacture and application of products.
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