电子烟液体比率对重力过滤校正系数和实时测量的影响

IF 2.5 4区 环境科学与生态学 Q3 ENVIRONMENTAL SCIENCES Aerosol and Air Quality Research Pub Date : 2023-10-01 Epub Date: 2023-07-28 DOI:10.4209/aaqr.230011
Austin Close, Jane Blackerby, Heather Tunnell, Jack Pender, Eric Soule, Sinan Sousan
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引用次数: 0

摘要

电子香烟(ECIG)会产生高浓度的微粒物质(PM),通过二手接触影响人类吸入的空气质量。ECIG烟液可在市场上买到,有些用户还自己 "动手 "制作烟液,这些烟液的化学成分(包括丙二醇(PG)和植物甘油(VG))含量通常各不相同。以前的研究对含有不同 PG/VG 比率的液体产生的 ECIG 气溶胶中的 PM 浓度进行了量化。然而,这些比率对气溶胶仪器过滤校正系数的影响尚未得到评估,而这些校正系数是准确测量可吸入颗粒物浓度所必需的。因此,针对五种不同的 PG/VG 比率(1)0PG/100VG、2)15PG/85VG、3)50PG/50VG、4)72PG/28VG 和 5)90PG/10VG 以及两种不同的 PM 尺寸 PM1(1 μm 及以下)和 PM2.5(2.5 μm 及以下),确定了多种气溶胶仪器(SMPS + APS、MiniWRAS、pDR 和 SidePak)的 ECIG 气溶胶过滤校正系数。使用隔膜泵和可再充气的 ECIG 设备在受控的暴露室内产生 ECIG 气溶胶,用于所有比率。此外,还测量了所有五种 ECIG 比率的气溶胶粒度分布和质量中值直径。对于 SMPS + APS 组合数据,比率 1、2、3 和 4 的 PM2.5 校正因子(5-7.6)相似,而对于 MiniWRAS(~2)、pDR(~0.5)和 SidePak(~0.24),比率 1、2、3 相似。这些数据表明,可能需要为高 PG 含量的 ECIG 产生的气溶胶制定不同的校正系数。90PG/10VG 比率的校正因子值较高,可能是由于 PG 相对于 VG 的挥发性更大以及传感器损耗所致。PM2.5 的校正因子(比率 1-4)分别为 SMPS + APS 数据(4.96-7.62)、MiniWRAS(2.02-3.64)、pDR(0.50-1.07)和 SidePak(0.22-0.40)。这些数据有助于提高 ECIG 不同混合比气溶胶测量的准确性。
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Effects of E-Cigarette Liquid Ratios on the Gravimetric Filter Correction Factors and Real-Time Measurements.

Electronic cigarettes (ECIGs) generate high concentrations of particulate matter (PM), impacting the air quality inhaled by humans through secondhand exposure. ECIG liquids are available commercially and some users create their own "do-it-yourself" liquids, and these liquids often vary in the amounts of their chemical ingredients, including propylene glycol (PG) and vegetable glycerin (VG). Previous studies have quantified PM concentrations in ECIG aerosol generated from liquids containing different PG/VG ratios. However, the effects of these ratios on aerosol instrument filter correction factors needed to measure PM concentrations accurately have not been assessed. Thus, ECIG aerosol filter correction factors for multiple aerosol instruments (SMPS + APS, MiniWRAS, pDR, and SidePak) were determined for five different PG/VG ratios 1) 0PG/100VG, 2) 15PG/85VG, 3) 50PG/50VG, 4) 72PG/28VG, and 5) 90PG/10VG and two different PM sizes, PM1 (1 μm and smaller) and PM2.5 (2.5 μm and smaller). ECIG aerosols were generated inside a controlled exposure chamber using a diaphragm pump and a refillable ECIG device for all the ratios. In addition, the aerosol size distribution and mass median diameter were measured for all five ECIG ratios. PM2.5 correction factors (5-7.6) for ratios 1, 2, 3, and 4 were similar for the SMPS + APS combined data, and ratios 1, 2, 3 were similar for the MiniWRAS (~2), pDR (~0.5), and SidePak (~0.24). These data suggest different correction factors may need to be developed for aerosol generated from ECIGs with high PG content. The higher correction factor values for the 90PG/10VG ratio may have resulted from greater PG volatility relative to VG and sensor losses. The correction factors (ratios 1-4) for PM2.5 were SMPS + APS data (4.96-7.62), MiniWRAS (2.02-3.64), pDR (0.50-1.07), and SidePak (0.22-0.40). These data can help improve ECIG aerosol measurement accuracy for different ECIG mixture ratios.

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来源期刊
Aerosol and Air Quality Research
Aerosol and Air Quality Research ENVIRONMENTAL SCIENCES-
CiteScore
8.30
自引率
10.00%
发文量
163
审稿时长
3 months
期刊介绍: The international journal of Aerosol and Air Quality Research (AAQR) covers all aspects of aerosol science and technology, atmospheric science and air quality related issues. It encompasses a multi-disciplinary field, including: - Aerosol, air quality, atmospheric chemistry and global change; - Air toxics (hazardous air pollutants (HAPs), persistent organic pollutants (POPs)) - Sources, control, transport and fate, human exposure; - Nanoparticle and nanotechnology; - Sources, combustion, thermal decomposition, emission, properties, behavior, formation, transport, deposition, measurement and analysis; - Effects on the environments; - Air quality and human health; - Bioaerosols; - Indoor air quality; - Energy and air pollution; - Pollution control technologies; - Invention and improvement of sampling instruments and technologies; - Optical/radiative properties and remote sensing; - Carbon dioxide emission, capture, storage and utilization; novel methods for the reduction of carbon dioxide emission; - Other topics related to aerosol and air quality.
期刊最新文献
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