{"title":"g-C3N4是否更适合于环境应用中的光催化还原或氧化?","authors":"Qiaohong Zhu , Jinlong Zhang","doi":"10.1016/j.efmat.2022.05.003","DOIUrl":null,"url":null,"abstract":"<div><p>Graphitic carbon nitride (g-C<sub>3</sub>N<sub>4</sub>), as an efficient semiconductor photocatalyst with an excellent tunable bandgap, a high physicochemical stability and a proper optical performance, has shown its non-negligible potential in multifarious photocatalytic reactions, such as hydrogen (H<sub>2</sub>) evolution, carbon dioxide (CO<sub>2</sub>) reduction, hydrogen peroxide (H<sub>2</sub>O<sub>2</sub>) production, pollutants degradation and so on. However, considering the solar light transfer efficiency, the accurate reaction mechanisms as well as the limitations of various reactions, is g-C<sub>3</sub>N<sub>4</sub> more suitable for reduction or oxidation reactions? In this perspective, we think g-C<sub>3</sub>N<sub>4</sub> might be more suitable for photocatalytic reduction reactions since the performances of single oxidation reactions maybe not ideal and sometimes the electrons are still essential during such a process.</p></div>","PeriodicalId":100481,"journal":{"name":"Environmental Functional Materials","volume":"1 1","pages":"Pages 121-125"},"PeriodicalIF":0.0000,"publicationDate":"2022-03-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.sciencedirect.com/science/article/pii/S2773058122000060/pdfft?md5=1db8be8008127378127d9c8d145b5c74&pid=1-s2.0-S2773058122000060-main.pdf","citationCount":"12","resultStr":"{\"title\":\"Is g-C3N4 more suitable for photocatalytic reduction or oxidation in environmental applications?\",\"authors\":\"Qiaohong Zhu , Jinlong Zhang\",\"doi\":\"10.1016/j.efmat.2022.05.003\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<div><p>Graphitic carbon nitride (g-C<sub>3</sub>N<sub>4</sub>), as an efficient semiconductor photocatalyst with an excellent tunable bandgap, a high physicochemical stability and a proper optical performance, has shown its non-negligible potential in multifarious photocatalytic reactions, such as hydrogen (H<sub>2</sub>) evolution, carbon dioxide (CO<sub>2</sub>) reduction, hydrogen peroxide (H<sub>2</sub>O<sub>2</sub>) production, pollutants degradation and so on. However, considering the solar light transfer efficiency, the accurate reaction mechanisms as well as the limitations of various reactions, is g-C<sub>3</sub>N<sub>4</sub> more suitable for reduction or oxidation reactions? In this perspective, we think g-C<sub>3</sub>N<sub>4</sub> might be more suitable for photocatalytic reduction reactions since the performances of single oxidation reactions maybe not ideal and sometimes the electrons are still essential during such a process.</p></div>\",\"PeriodicalId\":100481,\"journal\":{\"name\":\"Environmental Functional Materials\",\"volume\":\"1 1\",\"pages\":\"Pages 121-125\"},\"PeriodicalIF\":0.0000,\"publicationDate\":\"2022-03-01\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"https://www.sciencedirect.com/science/article/pii/S2773058122000060/pdfft?md5=1db8be8008127378127d9c8d145b5c74&pid=1-s2.0-S2773058122000060-main.pdf\",\"citationCount\":\"12\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Environmental Functional Materials\",\"FirstCategoryId\":\"1085\",\"ListUrlMain\":\"https://www.sciencedirect.com/science/article/pii/S2773058122000060\",\"RegionNum\":0,\"RegionCategory\":null,\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"\",\"JCRName\":\"\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Environmental Functional Materials","FirstCategoryId":"1085","ListUrlMain":"https://www.sciencedirect.com/science/article/pii/S2773058122000060","RegionNum":0,"RegionCategory":null,"ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"","JCRName":"","Score":null,"Total":0}
Is g-C3N4 more suitable for photocatalytic reduction or oxidation in environmental applications?
Graphitic carbon nitride (g-C3N4), as an efficient semiconductor photocatalyst with an excellent tunable bandgap, a high physicochemical stability and a proper optical performance, has shown its non-negligible potential in multifarious photocatalytic reactions, such as hydrogen (H2) evolution, carbon dioxide (CO2) reduction, hydrogen peroxide (H2O2) production, pollutants degradation and so on. However, considering the solar light transfer efficiency, the accurate reaction mechanisms as well as the limitations of various reactions, is g-C3N4 more suitable for reduction or oxidation reactions? In this perspective, we think g-C3N4 might be more suitable for photocatalytic reduction reactions since the performances of single oxidation reactions maybe not ideal and sometimes the electrons are still essential during such a process.