西非Lamto地区CO2、CH4和CO浓度的时间变异分析

Toure Dro Tiemoko, M. Ramonet, Fidèle Yoroba, K. B. Kouassi, K. Kouadio, V. Kazan, C. Kaiser, F. Truong, C. Vuillemin, M. Delmotte, B. Wastine, P. Ciais
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引用次数: 7

摘要

摘要利用位于Côte科特迪瓦的Lamto (LTO)站(6°31 N和5°02 W)的高精度测量数据,分析了西非地区10年大气CO2、CH4和CO的摩尔分数。在日尺度上,CO2和CH4的高浓度出现在夜间,在当地时间早上7点左右达到峰值,下午浓度最低。CO浓度在8 h和20 h出现两个峰值,对应于距离站点14 km的北部高速公路的道路交通最大值。Lamto的CH4 (~ 7 ppb - 1年)和CO2 (~ 2.24 ppm - 1年)的长期增长率非常接近全球趋势。3种气体的浓度变化均表现出较强的季节性,其中CO2和CH4在1月达到峰值,CO2和CH4在9月达到最低点,CO在6月达到最低点。CO的变化表明,12月至2月枯水期林火对Lamto地区CO、CO2和CH4异常有显著影响。CO和CH4在1月(r = 0.84)、2月(r = 0.90)、4月(r = 0.74)、11月(r = 0.79)和12月(r = 0.72)表现出较强的相关性(在天气尺度和月基础上),反映出两种气体的排放源相似。LTO受污染气团的轨迹也显示了与哈马丹风有关的大陆排放源。
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Analysis of the temporal variability of CO2, CH4 and CO concentrations at Lamto, West Africa
Abstract The 10-year observations of the atmospheric molar fractions of CO2, CH4 and CO in West Africa were analyzed using a high precision measurement of the Lamto (LTO) station (6°31 N and 5°02 W) in Côte d’Ivoire. At daily scale, high concentrations appear at night with significant peaks around 7 a.m. local time and minimum concentrations in the afternoon for CO2 and CH4. The CO concentrations show two peaks around 8 h and 20 h corresponding to the maximum in road traffic of a northern motorway located 14 km from the station. The long-term increase rates of CH4 (∼7 ppb year−1) and CO2 (∼2.24 ppm year−1) at Lamto are very close to global trends. The variations of the concentrations of the three gases show strong seasonality with a peak in January for all gases and minima in September for CO2 and CH4, and in June for CO. The CO variation suggests a significant impact of fires on the CO, CO2 and CH4 anomalies in the Lamto region during the dry season (December to February). CO and CH4 show strong correlations (at synoptic-scale and monthly based) in January (r = 0.84), February (r = 0.90), April (r = 0.74), November (r = 0.79) and December (r = 0.72) reflecting similar sources of emission for both gases. The trajectories of polluted air masses at LTO, also indicate continental sources of emission associated with Harmattan winds.
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