Sr2RuO4中以Ru dxy轨道为主导的手性超导的隐藏异常霍尔效应

Jia-Long Zhang, Yu Li, Wen Huang, Fu-Chun Zhang
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引用次数: 5

摘要

超导材料Sr$_2$RuO$_4$中的极性克尔效应意味着有限交流异常霍尔电导率。由于在单个Ru $d_{xy}$轨道上发展的手性超导对不存在本征异常霍尔效应,因此提出了积极涉及Ru $d_{xz}$和$d_{yz}$轨道的多轨道手性对作为一种潜在的机制。在这里,我们提出即使手性超导主要是由$d_{xy}$轨道驱动,AHE仍然可能产生。这是通过两个单独的模型来证明的,它们考虑了库珀对中的亚优势轨道,一个涉及到RuO$_2$平面上的氧$p_x$和$p_y$轨道,另一个涉及到$d_{xz}$和$d_{yz}$轨道。在这两种模型中,占主导地位的$d_{xy}$和其他轨道之间的有限轨道混合可能导致它们之间的轨道间配对,并且所得到的态支持本然AHE,克尔旋转角可能与实验观测相一致。因此,我们的建议为Sr$_2$RuO$_4$的微观配对提供了新的思路。本征霍尔效应在$\mathcal{S}+i\mathcal{D}$、$\mathcal{D}+i\mathcal{P}$和$\mathcal{D}+i\mathcal{G}$等非手性态中普遍不存在,这为该材料超导序的对称性提供了明确的约束。
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Hidden anomalous Hall effect in Sr2RuO4 with chiral superconductivity dominated by the Ru dxy orbital
The polar Kerr effect in superconducting Sr$_2$RuO$_4$ implies finite ac anomalous Hall conductivity. Since intrinsic anomalous Hall effect (AHE) is not expected for a chiral superconducting pairing developed on the single Ru $d_{xy}$ orbital, multiorbital chiral pairing actively involving the Ru $d_{xz}$ and $d_{yz}$ orbitals has been proposed as a potential mechanism. Here we propose that AHE could still arise even if the chiral superconductivity is predominantly driven by the $d_{xy}$ orbital. This is demonstrated through two separate models which take into account subdominant orbitals in the Cooper pairing, one involving the oxygen $p_x$ and $p_y$ orbitals in the RuO$_2$ plane, and another the $d_{xz}$ and $d_{yz}$ orbitals. In both models, finite orbital mixing between the dominant $d_{xy}$ and the other orbitals may induce inter-orbital pairing between them, and the resultant states support intrinsic AHE, with Kerr rotation angles that could potentially reconcile with the experimental observation. Our proposal therefore sheds new light on the microscopic pairing in Sr$_2$RuO$_4$. We also show that intrinsic Hall effect is generally absent for non-chiral states such as $\mathcal{S}+i\mathcal{D}$, $\mathcal{D}+i\mathcal{P}$ and $\mathcal{D}+i\mathcal{G}$, which provides a clear constraint on the symmetry of the superconducting order in this material.
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