包覆可可逆切换铁(II)自旋跃迁纳米粒子的光波导有机纳米棒

Supratim Basak, Ajay Kumar Botcha, M. Ansari, Rajadurai Chandrasekar
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引用次数: 1

摘要

通过“自下而上”的自组装方法,成功制备了具有光子和磁性质的双功能纳米杂化物体。该方法原位生成了自旋跃迁铁(II)配位纳米粒子和光波导有机纳米棒,并通过自组装成功地集成在一个锅中。包覆在有机纳米棒(纳米杂化体)上的Fe(II)纳米颗粒显示出温度依赖的可逆自旋跃迁(顺磁性;抗磁性。的行为。这些纳米杂化物表现出高效的光波引导行为,这表明在单自旋跃迁纳米粒子水平上进行光诱导激发自旋态捕获(LIESST)实验是可能的。这些光子和磁性的“纳米杂化体”为利用温度和远程激光从外部操纵自旋跃迁纳米粒子的自旋态提供了有希望的选择。
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Optical Waveguiding Organic Nanorods Coated with Reversibly Switchable Fe(II) Spin Transition Nanoparticles
A dual functional nanohybrid object combining photonic and magnetic properties was successfully prepared through a “bottom-up” self-assembly approach. In this method, spin transition Fe(II) coordination nanoparticles and optical wave guiding organic nanorods were generated in situ and successfully integrated together in a single pot through self-assembly. The Fe(II) nanoparticles coated on organic nanorods (nanohybrids) display temperature dependent reversible spin transition (Paramagnetic; diamagnetic; ) behavior. The nano-hybrids show efficient optical wave guiding behavior, which demonstrates the future possibility to perform light induced excited spin state trapping (LIESST) experiments on a single spin transition nanoparticle level. These photonic and magnetic “nanohybrids” offer promising option to externally manipulate spin state of the spin transition nanoparticles using temperature as well as remote laser light.
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