辐照密度为4.8 gU/cm3的U3Si2-Al时裂变气泡和相互作用层的研究

Juan Carlos Sihotang, M. K. Ajiriyanto, Anditania Sari Dwi Putri, E. Nurlaily, J. Junaedi, Aslina Br Ginting, Supardjo Supardjo
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摘要

辐照密度为4.8 gU/cm3的U3Si2-Al时裂变气泡和相互作用层的研究。分散在铝基中的铀硅化物复合燃料(U3Si2-Al)由于其优异的辐照性能,已在世界范围内大量应用于研究堆中。该燃料还提供了高铀密度,典型燃料负荷高达4.8 gU/cm3,以弥补低浓铀中裂变量的减少。为了提高印度尼西亚GA siwessy多用途研究堆中使用的U3Si2-Al的密度(2.96 gU/cm3),密度为4.8 gU/cm3 (U235 ~ 19.75%)的U3Si2-Al分散燃料板在RSG GAS中以15 MW功率照射175天,使燃耗水平约为40%。利用SEM-EDS和光学显微镜对辐照后燃料的微观结构进行了表征,主要是裂变气泡和U3Si2燃料与Al基体之间的相互作用层。直径为0.06 ~ 0.55µm的气泡平均直径为0.21µm。相互作用层为U(Al,Si)2,3,厚度约为1.5µm。相对较小的裂变气泡和相互作用层没有引起燃料膨胀,燃料板的整体性能很好。关键词:低浓缩铀,硅化铀,辐照后检测,相互作用层,裂变气泡。
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STUDY OF FISSION GAS BUBBLES AND INTERACTION LAYER ON IRRADIATED U3Si2-Al DENSITY OF 4.8 gU/cm3
STUDY OF FISSION GAS BUBBLES AND INTERACTION LAYER ON IRRADIATED U3Si2-Al DENSITY OF 4.8 gU/cm3. Uranium-silicide compound fuel dispersed in aluminium matrix (U3Si2-Al) have been used in a large number of research reactors around the world because of its excellent behavior under irradiation. This fuel also provides high uranium density with typical fuel loading up to 4.8 gU/cm3 to compensate for the reduced fissile amount in LEU. To improve the density of current U3Si2-Al (2.96 gU/cm3) used in Indonesian GA Siwabessy Multipurpose Research Reactor, U3Si2-Al dispersion fuel plate with density of 4.8 gU/cm3 (U235 ∼19.75%) had been irradiated in RSG GAS for 175 days at 15 MW power to burnup level of approximately 40%. The characterization was performed using SEM-EDS and optical microscope to study microstructure of the irradiatted fuel, largely the fission gas bubbles and the interaction layer between U3Si2 fuel and Al matrix. The average diameter of the bubbles with diameter from 0.06 to 0.55 µm was 0.21 µm. The interaction layer was identified as U(Al,Si)2,3 with thickness of approximately 1.5 µm. The relatively small fission gas bubbles and the interaction layer didn’t cause swelling on the fuel and the overall performance of the fuel plate was very good.Keyword:  LEU, uranium-silicide, post-irradiation examination, interaction layer, fission gas bubbles.
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