甲烷氧化偶联高活性单金属氧化物催化剂的研究进展

Goune Choi, B. Koo
{"title":"甲烷氧化偶联高活性单金属氧化物催化剂的研究进展","authors":"Goune Choi, B. Koo","doi":"10.31613/ceramist.2021.24.4.05","DOIUrl":null,"url":null,"abstract":"The conversion of methane to a value-added chemical is important for methane utilization and industrial demand for primary chemicals. Oxidative coupling of methane (OCM) to C2 hydrocarbons is one of the most attractive ways to use natural gas. However, it is difficult to obtain higher C2 yield in classic OCM reaction due to a favorable COx formation. Regarding this, various catalysts for OCM have been studied to fulfill desirable C2 yields. In this review, we briefly overview the single metal oxide types of OCM catalysts (alkaline-earth metal oxides and rare-earth metal oxides) and highlight the characteristics of catalysts in OCM reaction such as methane activation, surface basicity and lattice oxygen.","PeriodicalId":9738,"journal":{"name":"Ceramist","volume":null,"pages":null},"PeriodicalIF":0.0000,"publicationDate":"2021-12-31","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Research Trends in Development of Highly Active Single Metal Oxide Catalyst for Oxidative Coupling of Methane\",\"authors\":\"Goune Choi, B. Koo\",\"doi\":\"10.31613/ceramist.2021.24.4.05\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"The conversion of methane to a value-added chemical is important for methane utilization and industrial demand for primary chemicals. Oxidative coupling of methane (OCM) to C2 hydrocarbons is one of the most attractive ways to use natural gas. However, it is difficult to obtain higher C2 yield in classic OCM reaction due to a favorable COx formation. Regarding this, various catalysts for OCM have been studied to fulfill desirable C2 yields. In this review, we briefly overview the single metal oxide types of OCM catalysts (alkaline-earth metal oxides and rare-earth metal oxides) and highlight the characteristics of catalysts in OCM reaction such as methane activation, surface basicity and lattice oxygen.\",\"PeriodicalId\":9738,\"journal\":{\"name\":\"Ceramist\",\"volume\":null,\"pages\":null},\"PeriodicalIF\":0.0000,\"publicationDate\":\"2021-12-31\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Ceramist\",\"FirstCategoryId\":\"1085\",\"ListUrlMain\":\"https://doi.org/10.31613/ceramist.2021.24.4.05\",\"RegionNum\":0,\"RegionCategory\":null,\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"\",\"JCRName\":\"\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Ceramist","FirstCategoryId":"1085","ListUrlMain":"https://doi.org/10.31613/ceramist.2021.24.4.05","RegionNum":0,"RegionCategory":null,"ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"","JCRName":"","Score":null,"Total":0}
引用次数: 0

摘要

甲烷转化为增值化学品对甲烷利用和工业对初级化学品的需求具有重要意义。甲烷(OCM)与C2烃的氧化偶联是最具吸引力的天然气利用方式之一。然而,在经典的OCM反应中,由于有利于COx的形成,很难获得较高的C2产率。为此,研究了各种OCM催化剂,以实现理想的C2产率。本文简要介绍了OCM催化剂的单金属氧化物类型(碱土金属氧化物和稀土金属氧化物),重点介绍了OCM反应中催化剂的甲烷活化、表面碱度和晶格氧等特征。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
查看原文
分享 分享
微信好友 朋友圈 QQ好友 复制链接
本刊更多论文
Research Trends in Development of Highly Active Single Metal Oxide Catalyst for Oxidative Coupling of Methane
The conversion of methane to a value-added chemical is important for methane utilization and industrial demand for primary chemicals. Oxidative coupling of methane (OCM) to C2 hydrocarbons is one of the most attractive ways to use natural gas. However, it is difficult to obtain higher C2 yield in classic OCM reaction due to a favorable COx formation. Regarding this, various catalysts for OCM have been studied to fulfill desirable C2 yields. In this review, we briefly overview the single metal oxide types of OCM catalysts (alkaline-earth metal oxides and rare-earth metal oxides) and highlight the characteristics of catalysts in OCM reaction such as methane activation, surface basicity and lattice oxygen.
求助全文
通过发布文献求助,成功后即可免费获取论文全文。 去求助
来源期刊
自引率
0.00%
发文量
0
期刊最新文献
Perspectives on the development of advanced lithium metal anode Short Review of Flash Sintering: Mechanisms, Microstructures, and Mechanical Properties Research Trends on the Influence of Oxygen Vacancies in Post BaTiO3 (BT) Ceramics for Next-Generation MLCCs Resent Progress of LiNi1-x-yCoxMnyO2 for Lithium-ion batteries Recent progress in all-solid-state Li-ion battery anodes
×
引用
GB/T 7714-2015
复制
MLA
复制
APA
复制
导出至
BibTeX EndNote RefMan NoteFirst NoteExpress
×
×
提示
您的信息不完整,为了账户安全,请先补充。
现在去补充
×
提示
您因"违规操作"
具体请查看互助需知
我知道了
×
提示
现在去查看 取消
×
提示
确定
0
微信
客服QQ
Book学术公众号 扫码关注我们
反馈
×
意见反馈
请填写您的意见或建议
请填写您的手机或邮箱
已复制链接
已复制链接
快去分享给好友吧!
我知道了
×
扫码分享
扫码分享
Book学术官方微信
Book学术文献互助
Book学术文献互助群
群 号:481959085
Book学术
文献互助 智能选刊 最新文献 互助须知 联系我们:info@booksci.cn
Book学术提供免费学术资源搜索服务,方便国内外学者检索中英文文献。致力于提供最便捷和优质的服务体验。
Copyright © 2023 Book学术 All rights reserved.
ghs 京公网安备 11010802042870号 京ICP备2023020795号-1