Revealing defect-induced spin disorder in nanocrystalline Ni

We use magnetic small-angle neutron scattering to study the magnetic microstructure of a nanocrystalline Ni bulk sample, which was prepared by straining via high-pressure torsion. The neutron data reveal that the scattering is strongly affected by the high density of crystal defects inside the sample, which were created by the severe plastic deformation during the sample preparation. The defects cause a significant spin-misalignment scattering contribution. The corresponding magnetic correlation length, which characterizes the spatial magnetization fluctuations in real space, indicates an average defect size of 11 nm. In the remanent state, the stray fields around the defects cause spin disorder in the surrounding ferromagnetic bulk, with a penetration depth of around 22 nm. The range and amplitude of the disorder is systematically suppressed by an increasing external magnetic field. Our findings are supported by micromagnetic simulations, which, for the particular case of nonmagnetic defects (holes) embedded in a ferromagnetic Ni phase, further highlight the role of localized spin perturbations for the magnetic microstructure of defect-rich magnets such as high-pressure torsion materials.